Bright compact ultrabroadband source by orthogonal laser-sustained plasma

IF 3.5 3区 医学 Q2 CHEMISTRY, MEDICINAL ACS Medicinal Chemistry Letters Pub Date : 2024-09-26 DOI:10.1038/s41377-024-01602-2
Zhaojiang Shi, Shichao Yang, He Hu, Haodong Lei, Zhaohua Yang, Xia Yu
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Abstract

Laser-sustained plasma (LSP) source featuring high brightness and broadband spectral coverage is found to be powerful in various fields of scientific and industrial applications. However, the fundamental limit of low conversion efficiency constrains the system compactness and widespread applications of such broadband light sources. In this paper, we propose an innovative orthogonal LSP to break through the conversion efficiency limitation. Driven by the elevated conversion efficiency from absorbed laser power to ultraviolet (UV) emission, a compact broadband source (250–1650 nm) with UV spectral radiance exceeding 210 \({mW}/({{mm}}^{2}\,\cdot\, {sr}\,\cdot\, {nm})\) is achieved with >100 W pump laser. With the plot of a two-dimensional refractive index model, we report an important conceptual advance that the orthogonal design eliminates the influence of the negative lensing effect on laser power density. Experimental results unambiguously demonstrate that we achieve a bright compact UV-VIS-NIR source with negligible thermal loss and the highest conversion efficiency to our knowledge. Significant enhancement of 4 dB contrast-to-noise ratio (CNR) in spectral single-pixel imaging has been demonstrated using the proposed ultrabroadband source. By establishing the quantitative link between pumping optics design and plasma absorption, this work presents a compact broadband source that combines superior conversion efficiency and unprecedented brightness, which is essential to high-speed inspection and spectroscopy applications.

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通过正交激光维持等离子体实现明亮紧凑的超宽带源
激光维持等离子体(LSP)光源具有高亮度和宽带光谱覆盖的特点,在科学和工业应用的各个领域都具有强大的功能。然而,低转换效率这一基本限制制约了此类宽带光源的系统紧凑性和广泛应用。在本文中,我们提出了一种创新的正交 LSP,以突破转换效率的限制。在从吸收激光功率到紫外线(UV)发射的转换效率提高的驱动下,在使用100 W泵浦激光的情况下,紧凑型宽带光源(250-1650 nm)的紫外光谱辐射率超过了210 \({mW}/({{mm}}^{2}\,{sr}\,\cdot\,{nm})\)。通过绘制二维折射率模型,我们报告了一个重要的概念进步,即正交设计消除了负透镜效应对激光功率密度的影响。实验结果清楚地表明,我们实现了一种明亮紧凑的紫外-可见-近红外光源,其热损耗可以忽略不计,转换效率也是我们目前所知最高的。利用所提出的超宽带光源,光谱单像素成像的对比噪声比(CNR)显著提高了 4 dB。通过建立泵浦光学设计与等离子体吸收之间的定量联系,这项研究提出了一种紧凑型宽带光源,它结合了卓越的转换效率和前所未有的亮度,这对高速检测和光谱学应用至关重要。
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来源期刊
ACS Medicinal Chemistry Letters
ACS Medicinal Chemistry Letters CHEMISTRY, MEDICINAL-
CiteScore
7.30
自引率
2.40%
发文量
328
审稿时长
1 months
期刊介绍: ACS Medicinal Chemistry Letters is interested in receiving manuscripts that discuss various aspects of medicinal chemistry. The journal will publish studies that pertain to a broad range of subject matter, including compound design and optimization, biological evaluation, drug delivery, imaging agents, and pharmacology of both small and large bioactive molecules. Specific areas include but are not limited to: Identification, synthesis, and optimization of lead biologically active molecules and drugs (small molecules and biologics) Biological characterization of new molecular entities in the context of drug discovery Computational, cheminformatics, and structural studies for the identification or SAR analysis of bioactive molecules, ligands and their targets, etc. Novel and improved methodologies, including radiation biochemistry, with broad application to medicinal chemistry Discovery technologies for biologically active molecules from both synthetic and natural (plant and other) sources Pharmacokinetic/pharmacodynamic studies that address mechanisms underlying drug disposition and response Pharmacogenetic and pharmacogenomic studies used to enhance drug design and the translation of medicinal chemistry into the clinic Mechanistic drug metabolism and regulation of metabolic enzyme gene expression Chemistry patents relevant to the medicinal chemistry field.
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