High discrimination ratio, broadband circularly polarized light photodetector using dielectric achiral nanostructures

IF 3.5 3区 医学 Q2 CHEMISTRY, MEDICINAL ACS Medicinal Chemistry Letters Pub Date : 2024-09-27 DOI:10.1038/s41377-024-01634-8
Guanyu Zhang, Xiaying Lyu, Yulu Qin, Yaolong Li, Zipu Fan, Xianghan Meng, Yuqing Cheng, Zini Cao, Yixuan Xu, Dong Sun, Yunan Gao, Qihuang Gong, Guowei Lyu
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Abstract

The on-chip measurement of polarization states plays an increasingly crucial role in modern sensing and imaging applications. While high-performance monolithic linearly polarized photodetectors have been extensively studied, integrated circularly polarized light (CPL) photodetectors are still hindered by inadequate discrimination capability. This study presents a broadband CPL photodetector utilizing achiral all-dielectric nanostructures, achieving an impressive discrimination ratio of ~107 at a wavelength of 405 nm. Our device shows outstanding CPL discrimination capability across the visible band without requiring intensity calibration. It functions based on the CPL-dependent near-field modes within achiral structures: under left or right CPL illumination, distinct near-field modes are excited, resulting in asymmetric irradiation of the two electrodes and generating a photovoltage with directions determined by the chirality of the incident light field. The proposed design strategy facilitates ultra-compact CPL detection across diverse materials, structures, and spectral ranges, presenting a novel avenue for achieving high-performance monolithic CPL detection.

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使用介电非手性纳米结构的高分辨比、宽带圆偏振光光电探测器
片上偏振态测量在现代传感和成像应用中发挥着越来越重要的作用。虽然高性能单片线性偏振光检测器已被广泛研究,但集成的圆偏振光(CPL)光检测器仍然受到分辨能力不足的阻碍。本研究提出了一种利用非手性全介电纳米结构的宽带 CPL 光电探测器,在波长为 405 纳米时实现了 ~107 的惊人分辨比。我们的器件在整个可见光波段都具有出色的 CPL 分辨能力,无需进行强度校准。它的功能基于非手性结构中依赖于 CPL 的近场模式:在左侧或右侧 CPL 照射下,不同的近场模式被激发,导致两个电极受到不对称照射,并产生光电压,其方向由入射光场的手性决定。所提出的设计策略有助于在各种材料、结构和光谱范围内进行超紧凑型 CPL 检测,为实现高性能单片 CPL 检测提供了一条新途径。
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来源期刊
ACS Medicinal Chemistry Letters
ACS Medicinal Chemistry Letters CHEMISTRY, MEDICINAL-
CiteScore
7.30
自引率
2.40%
发文量
328
审稿时长
1 months
期刊介绍: ACS Medicinal Chemistry Letters is interested in receiving manuscripts that discuss various aspects of medicinal chemistry. The journal will publish studies that pertain to a broad range of subject matter, including compound design and optimization, biological evaluation, drug delivery, imaging agents, and pharmacology of both small and large bioactive molecules. Specific areas include but are not limited to: Identification, synthesis, and optimization of lead biologically active molecules and drugs (small molecules and biologics) Biological characterization of new molecular entities in the context of drug discovery Computational, cheminformatics, and structural studies for the identification or SAR analysis of bioactive molecules, ligands and their targets, etc. Novel and improved methodologies, including radiation biochemistry, with broad application to medicinal chemistry Discovery technologies for biologically active molecules from both synthetic and natural (plant and other) sources Pharmacokinetic/pharmacodynamic studies that address mechanisms underlying drug disposition and response Pharmacogenetic and pharmacogenomic studies used to enhance drug design and the translation of medicinal chemistry into the clinic Mechanistic drug metabolism and regulation of metabolic enzyme gene expression Chemistry patents relevant to the medicinal chemistry field.
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