Minggang Zheng , Han Liang , Wenxie Bu , Cheng Qu , Xiaoxu Hu , Zhihu Zhang
{"title":"Porosity and permeability optimization of PEMFC cathode gas diffusion layer based on topology algorithm","authors":"Minggang Zheng , Han Liang , Wenxie Bu , Cheng Qu , Xiaoxu Hu , Zhihu Zhang","doi":"10.1016/j.ijoes.2024.100803","DOIUrl":null,"url":null,"abstract":"<div><div>The gas diffusion layer (GDL) is a crucial component in proton exchange membrane fuel cells (PEMFCs), significantly affecting mass transport and overall cell performance. Due to the pronounced pressure gradients and uneven mass transfer between the inlet and outlet of the serpentine flow field, this study proposes the design of a GDL with a concentration gradient to optimize performance. Leveraging topological optimization algorithms, the research focuses on enhancing the mass transport properties and improving cell efficiency. The optimization process considers the pressure distribution, oxygen concentration, and water content within the serpentine flow field as boundary conditions. By optimizing the porosity and permeability of the GDL in different regions, the study aims to enhance the GDL's mass transport capabilities. Simulation results demonstrate that initializing the porosity at 1 provides superior optimization, significantly enhancing mass transfer and overall cell performance. Although increased permeability contributes to improved mass transport, its impact is less significant compared to porosity optimization. Therefore, GDL porosity is identified as the dominant factor in enhancing cell performance, while permeability adjustments play a secondary role.</div></div>","PeriodicalId":13872,"journal":{"name":"International Journal of Electrochemical Science","volume":"19 11","pages":"Article 100803"},"PeriodicalIF":1.3000,"publicationDate":"2024-09-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"International Journal of Electrochemical Science","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1452398124003456","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"ELECTROCHEMISTRY","Score":null,"Total":0}
引用次数: 0
Abstract
The gas diffusion layer (GDL) is a crucial component in proton exchange membrane fuel cells (PEMFCs), significantly affecting mass transport and overall cell performance. Due to the pronounced pressure gradients and uneven mass transfer between the inlet and outlet of the serpentine flow field, this study proposes the design of a GDL with a concentration gradient to optimize performance. Leveraging topological optimization algorithms, the research focuses on enhancing the mass transport properties and improving cell efficiency. The optimization process considers the pressure distribution, oxygen concentration, and water content within the serpentine flow field as boundary conditions. By optimizing the porosity and permeability of the GDL in different regions, the study aims to enhance the GDL's mass transport capabilities. Simulation results demonstrate that initializing the porosity at 1 provides superior optimization, significantly enhancing mass transfer and overall cell performance. Although increased permeability contributes to improved mass transport, its impact is less significant compared to porosity optimization. Therefore, GDL porosity is identified as the dominant factor in enhancing cell performance, while permeability adjustments play a secondary role.
期刊介绍:
International Journal of Electrochemical Science is a peer-reviewed, open access journal that publishes original research articles, short communications as well as review articles in all areas of electrochemistry: Scope - Theoretical and Computational Electrochemistry - Processes on Electrodes - Electroanalytical Chemistry and Sensor Science - Corrosion - Electrochemical Energy Conversion and Storage - Electrochemical Engineering - Coatings - Electrochemical Synthesis - Bioelectrochemistry - Molecular Electrochemistry