Yu Gao, Guangyuan Liang, Huanhuan Liang, Lijing Wang, Hongfang Du, Dezheng Liu, Liangxu Lin
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引用次数: 0
Abstract
The advancement of various energy conversion and storage technologies hinges on the development of efficient and stable electrocatalysts for the oxygen reduction reaction (ORR). In this study, we report the enhancement of carbon cloth (CC) for robust ORR through an FeCl3intercalation reaction. Utilizing a thermal annealing method, FeCl3was intercalated into the graphite structure on the surface of CC, resulting in the creation of numerous defects and the incorporation of Fe species. These newly introduced defects play a pivotal role in activating the ORR via a two-electron pathway. The presence of Fe species further stabilizes the catalytic activity, leading to efficient and stable ORR performance. Our findings highlight the significance of defect engineering and Fe species incorporation in carbon-based materials for improved ORR catalysis and pave the way for the development of advanced electrocatalysts for energy-related applications.
期刊介绍：
The journal aims to publish papers at the forefront of nanoscale science and technology and especially those of an interdisciplinary nature. Here, nanotechnology is taken to include the ability to individually address, control, and modify structures, materials and devices with nanometre precision, and the synthesis of such structures into systems of micro- and macroscopic dimensions such as MEMS based devices. It encompasses the understanding of the fundamental physics, chemistry, biology and technology of nanometre-scale objects and how such objects can be used in the areas of computation, sensors, nanostructured materials and nano-biotechnology.
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