High-risk nuclide screening and parameter sensitivity analysis based on numerical simulation and machine learning

IF 12.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2024-09-30 DOI:10.1016/j.jhazmat.2024.136002
Xin Zhang, Yanjun Zhang, Yu Zhang, Yuxiang Cheng, Qiangbin Liu, Hao Deng, Yongjie Ma, Lin Bai, Lei Liu
{"title":"High-risk nuclide screening and parameter sensitivity analysis based on numerical simulation and machine learning","authors":"Xin Zhang, Yanjun Zhang, Yu Zhang, Yuxiang Cheng, Qiangbin Liu, Hao Deng, Yongjie Ma, Lin Bai, Lei Liu","doi":"10.1016/j.jhazmat.2024.136002","DOIUrl":null,"url":null,"abstract":"During nuclear accidents, large quantities of radionuclides will be released into the environment, posing serious health hazards to local residents. The screening of high-risk nuclides is critical for the development of subsequent nuclear emergency response measures. In order to overcome the shortcomings of traditional screening methods, a machine learning method was proposed to screen high-risk nuclides and predict their contamination to groundwater more effectively. The performances of Support Vector Machine (SVM), Random Forest (RF) and Back Propagation Neural Network (BPNN) algorithms were compared, and sensitivity analyses of the initial leakage concentration ratio (<em>C</em><sub><em>0</em></sub><em>/C</em><sub><em>p</em></sub>), distribution coefficient (<em>K</em><sub><em>d</em></sub>) and decay coefficient (<span><math><mi is=\"true\" mathvariant=\"bold-italic\">λ</mi></math></span>) on the model outputs were performed. Results showed that RF classification model achieved the highest prediction accuracy for screening high-risk nuclides. The contribution of the input parameters ranked as <em>K</em><sub><em>d</em></sub> &gt; <span><math><mi is=\"true\">λ</mi></math></span> &gt; <em>C</em><sub><em>0</em></sub><em>/C</em><sub><em>p</em></sub>. BPNN regression model was found to be the best for predicting when high-risk nuclides would pollute groundwater. The output was negatively correlated with <em>C</em><sub><em>0</em></sub><em>/C</em><sub><em>p</em></sub> and positively correlated with <em>K</em><sub><em>d</em></sub> and <span><math><mi is=\"true\">λ</mi></math></span>, with the parameter influence ranking as <em>K</em><sub><em>d</em></sub> &gt; <em>C</em><sub><em>0</em></sub><em>/C</em><sub><em>p</em></sub> &gt; <span><math><mi is=\"true\">λ</mi></math></span>. The contribution of <em>K</em><sub><em>d</em></sub> mainly came from itself, and the contribution of <em>C</em><sub><em>0</em></sub><em>/C</em><sub><em>p</em></sub> and <span><math><mi is=\"true\">λ</mi></math></span> mainly due to their interaction with other parameters.","PeriodicalId":361,"journal":{"name":"Journal of Hazardous Materials","volume":null,"pages":null},"PeriodicalIF":12.2000,"publicationDate":"2024-09-30","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Hazardous Materials","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1016/j.jhazmat.2024.136002","RegionNum":1,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0

Abstract

During nuclear accidents, large quantities of radionuclides will be released into the environment, posing serious health hazards to local residents. The screening of high-risk nuclides is critical for the development of subsequent nuclear emergency response measures. In order to overcome the shortcomings of traditional screening methods, a machine learning method was proposed to screen high-risk nuclides and predict their contamination to groundwater more effectively. The performances of Support Vector Machine (SVM), Random Forest (RF) and Back Propagation Neural Network (BPNN) algorithms were compared, and sensitivity analyses of the initial leakage concentration ratio (C0/Cp), distribution coefficient (Kd) and decay coefficient (λ) on the model outputs were performed. Results showed that RF classification model achieved the highest prediction accuracy for screening high-risk nuclides. The contribution of the input parameters ranked as Kd > λ > C0/Cp. BPNN regression model was found to be the best for predicting when high-risk nuclides would pollute groundwater. The output was negatively correlated with C0/Cp and positively correlated with Kd and λ, with the parameter influence ranking as Kd > C0/Cp > λ. The contribution of Kd mainly came from itself, and the contribution of C0/Cp and λ mainly due to their interaction with other parameters.

Abstract Image

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
基于数值模拟和机器学习的高风险核素筛选和参数敏感性分析
核事故发生时,大量放射性核素会释放到环境中,严重危害当地居民的健康。高风险核素的筛选对于后续核应急措施的制定至关重要。为了克服传统筛选方法的不足,提出了一种机器学习方法来筛选高风险核素,并更有效地预测其对地下水的污染。比较了支持向量机(SVM)、随机森林(RF)和反向传播神经网络(BPNN)算法的性能,并分析了初始泄漏浓度比(C0/Cp)、分布系数(Kd)和衰变系数(λ)对模型输出结果的敏感性。结果表明,射频分类模型在筛选高风险核素方面的预测准确率最高。输入参数的贡献排序为 Kd > λ > C0/Cp。BPNN 回归模型被认为是预测高风险核素何时会污染地下水的最佳模型。输出结果与 C0/Cp 呈负相关,与 Kd 和 λ 呈正相关,参数影响程度排序为 Kd > C0/Cp > λ。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
期刊最新文献
Comparative QSAR and q-RASAR Modeling for Aquatic Toxicity of Organic Chemicals to Three Trout Species: O. Clarkii, S. Namaycush, and S. Fontinalis Shortening the early diagnostic window of Hg2+-induced liver injury with a H2O2-activated fluorescence/afterglow imaging assay Cyanobacterial blooms prediction in China’s large hypereutrophic lakes based on MODIS observations and Bayesian theory Assessment of Drinking Water Quality and Identifying Pollution Sources in a Chromite Mining Region Rapid Detection of Microfibres in Environmental Samples Using Open-Source Visual Recognition Models
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1