{"title":"Insight into Fluoride Additives to Enhance Ammonia Production from Lithium-Mediated Electrochemical Nitrogen Reduction Reaction (Small 40/2024)","authors":"Dongwoo Shin, Yeongbae Jeon, Vy Thuy Nguyen, Shinmyeong Kang, Yewon Hong, Chaeeun Lim, Kijung Yong, Hyeyoung Shin, Yun Jeong Hwang","doi":"10.1002/smll.202470299","DOIUrl":null,"url":null,"abstract":"<p><b>Nitrogen Reduction Reaction</b></p><p>Adding F-additives with low lowest occupied molecular orbital energy during the electrochemical Li-mediated N<sub>2</sub> reduction reaction results in the formation of LiF solid electrolyte interphases. This process effectively reduces the energy barrier for the hydrogenation of Li<sub>3</sub>N on the surface, thereby enhancing the efficient production of NH<sub>3</sub>. More in article number 2404525, Hyeyoung Shin, Yun Jeong Hwang, and co-workers.\n\n <figure>\n <div><picture>\n <source></source></picture><p></p>\n </div>\n </figure></p>","PeriodicalId":228,"journal":{"name":"Small","volume":"20 40","pages":""},"PeriodicalIF":12.1000,"publicationDate":"2024-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://onlinelibrary.wiley.com/doi/epdf/10.1002/smll.202470299","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Small","FirstCategoryId":"88","ListUrlMain":"https://onlinelibrary.wiley.com/doi/10.1002/smll.202470299","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
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Abstract
Nitrogen Reduction Reaction
Adding F-additives with low lowest occupied molecular orbital energy during the electrochemical Li-mediated N2 reduction reaction results in the formation of LiF solid electrolyte interphases. This process effectively reduces the energy barrier for the hydrogenation of Li3N on the surface, thereby enhancing the efficient production of NH3. More in article number 2404525, Hyeyoung Shin, Yun Jeong Hwang, and co-workers.
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Small serves as an exceptional platform for both experimental and theoretical studies in fundamental and applied interdisciplinary research at the nano- and microscale. The journal offers a compelling mix of peer-reviewed Research Articles, Reviews, Perspectives, and Comments.
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