Preparation and application of organic hydrogels incorporating polyacrylamide/sodium alginate/DMSO for enhanced anti-drying, anti-freezing, and self-healing properties

Abstract

The double-network hydrogel comprises two asymmetrically structured cross-linked networks, demonstrating exceptional mechanical properties and possessing significant potential for application in the field of flexible sensors. However, conventional hydrogels primarily disperse in water as a medium and continuously lose moisture in natural environments, rendering them incapable of retaining hydration over extended periods and unsuitable for utilization under low-temperature conditions. In this study, we devised an organic hydrogel based on polyacrylamide (PAM), sodium alginate (SA), and dimethyl sulfoxide (DMSO). Through hydrogen bonding interactions among DMSO molecules, polyacrylamide, and sodium alginate, this organic hydrogel not only exhibits anti-drying and anti-freezing properties but also demonstrates self-healing characteristics. Moreover, the organic hydrogel showcases remarkable mechanical properties and conductivity capabilities that render it suitable for constructing flexible strain sensors to monitor human movements such as finger bending, elbow flexion, knee joint bending, and ankle extension. Additionally, the sensor exhibits excellent stability and durability.