Activation cross-sections of proton-induced nuclear reactions on natural zinc in the energy range of 4–30 MeV

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Radiation Physics and Chemistry Pub Date : 2024-09-30 DOI:10.1016/j.radphyschem.2024.112272
Mayeen Uddin Khandaker , Hiromitsu Haba , Ahmed Rufai Usman , Mustafa Mahmoud , Naohiko Otuka , Samer K.I. Ali
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Abstract

In the present work, the excitation functions for the proton-induced nuclear reactions on natural zinc were measured in the energy range of 4–30 MeV using the well-established stacked-foil activation procedure. The activation products were measured based on their characteristic gamma lines using HPGe γ-ray spectrometry. The radioactivities determined were used for the calculation of cross-sections of the radionuclides of interest, i.e., 61Cu, 62,65,69mZn, 57Co and 66,67,68Ga. The cross-sections have also been compared with the available literature data and the theoretical prediction of the TALYS code via its latest TENDL-2023 library as well as the prediction of EMPIRE-3.2.2 model code. The results show a reasonable agreement when compared with the available literature data. This work, however, shows that the theoretical data extracted from the TENDL-2023 library and EMPIRE-3.2.2 default calculation significantly underestimate the experimental cross-sections of 57Co nuclide while they overestimate those of 69mZn. The present result has potential applications to improve the predicting capability of the model codes as well as to serve as additional data for the nuclear reaction cross-section database.
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4-30 MeV 能量范围内天然锌上质子诱导核反应的活化截面
在本研究中,利用成熟的叠片活化程序测量了天然锌上质子诱导核反应在 4-30 MeV 能量范围内的激发函数。使用 HPGe γ 射线光谱法根据活化产物的特征伽玛线对其进行了测量。测定的放射性活度用于计算相关放射性核素(即 61Cu、62,65,69mZn、57Co 和 66,67,68Ga)的横截面。横截面还与现有的文献数据、TALYS 代码通过其最新的 TENDL-2023 库进行的理论预测以及 EMPIRE-3.2.2 模型代码的预测进行了比较。与现有文献数据相比,结果显示出合理的一致性。然而,这项工作表明,从 TENDL-2023 库和 EMPIRE-3.2.2 默认计算中提取的理论数据明显低估了 57Co 核素的实验截面,而高估了 69mZn 核素的实验截面。本结果具有潜在的应用价值,不仅可以提高模型代码的预测能力,还可以作为核反应截面数据库的补充数据。
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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