Flash sintering glass–ceramic treatment of Sr-contaminated soil waste

IF 5.6 2区 材料科学 Q1 MATERIALS SCIENCE, CERAMICS Ceramics International Pub Date : 2024-12-15 DOI:10.1016/j.ceramint.2024.10.136
Guilin Wei , Xiaoyan Shu , Jiahong Wang , Shibing Zuo , Kuan Wu , Guoliang Zhao , Fen Luo , Wenhong Han , Chen Xu , Xirui Lu
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Abstract

Effective disposal of radioactive waste is crucial for safe development of nuclear energy. In this study, flash sintering technology is used for the first time to quickly solidify simulated Sr-contaminated soil waste. The waste can be converted into a glass–ceramic phase by heating the waste at 1100 °C for 1 min during flash sintering. The phase evolution during flash sintering as a function of density and amorphous fraction was systematically investigated. Additionally, the microstructural evolution of the matrices and the leaching behavior of simulated waste elements (e.g., Sr) were evaluated. This study explores the feasibility of using flash sintering for treating radioactive contamination waste.

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闪速烧结玻璃陶瓷处理锶污染土壤废弃物
有效处置放射性废物对核能的安全发展至关重要。本研究首次采用闪速烧结技术来快速固化模拟锶污染土壤废物。在闪速烧结过程中,通过在 1100 °C 下加热 1 分钟,可将废料转化为玻璃陶瓷相。系统研究了闪速烧结过程中相的演变与密度和无定形部分的函数关系。此外,还评估了基质的微观结构演变和模拟废物元素(如锶)的浸出行为。这项研究探讨了利用闪速烧结处理放射性污染废物的可行性。
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产品信息
阿拉丁
SrSO4
来源期刊
Ceramics International
Ceramics International 工程技术-材料科学:硅酸盐
CiteScore
9.40
自引率
15.40%
发文量
4558
审稿时长
25 days
期刊介绍: Ceramics International covers the science of advanced ceramic materials. The journal encourages contributions that demonstrate how an understanding of the basic chemical and physical phenomena may direct materials design and stimulate ideas for new or improved processing techniques, in order to obtain materials with desired structural features and properties. Ceramics International covers oxide and non-oxide ceramics, functional glasses, glass ceramics, amorphous inorganic non-metallic materials (and their combinations with metal and organic materials), in the form of particulates, dense or porous bodies, thin/thick films and laminated, graded and composite structures. Process related topics such as ceramic-ceramic joints or joining ceramics with dissimilar materials, as well as surface finishing and conditioning are also covered. Besides traditional processing techniques, manufacturing routes of interest include innovative procedures benefiting from externally applied stresses, electromagnetic fields and energetic beams, as well as top-down and self-assembly nanotechnology approaches. In addition, the journal welcomes submissions on bio-inspired and bio-enabled materials designs, experimentally validated multi scale modelling and simulation for materials design, and the use of the most advanced chemical and physical characterization techniques of structure, properties and behaviour. Technologically relevant low-dimensional systems are a particular focus of Ceramics International. These include 0, 1 and 2-D nanomaterials (also covering CNTs, graphene and related materials, and diamond-like carbons), their nanocomposites, as well as nano-hybrids and hierarchical multifunctional nanostructures that might integrate molecular, biological and electronic components.
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