Enhance optically stimulated luminescence sensitivity and improve fading of newly developed LiMgPO4:Er phosphor

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Radiation Physics and Chemistry Pub Date : 2024-10-15 DOI:10.1016/j.radphyschem.2024.112297
Kaiyong Tang , Li Fu , Siyuan Zhang , Mo Zhou , Haijun Fan , Yan Zeng
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Abstract

To avoid fading, the readout time of the old LiMgPO4:Er in the previous study had to be taken to be at least 20 s. The readout time is up to 20 s, which not only contradicts the fast OSL readout, but also eliminates too many OSL signals per readout and is not favourable to the requirement that the OSL can be read multiple times. The primary objective of this study is to reduce readout time under conditions where the OSL signal of LiMgPO4:Er phosphor stabilizes after irradiation. The OSL properties were investigated. To achieve OSL fading of about 5% within 30 d after irradiation, the shortest integration time for new LiMgPO4:Er in this study was 1 s, whereas old LiMgPO4:Er required 20 s. When the integration time was 1 s, the OSL sensitivity of the new LiMgPO4:Er samples in this study was about 2.4 times that of the old LiMgPO4:Er samples. A new LiMgPO4:Er phosphor with an OSL signal loss of about 5% for the shortest integration time of 1 s within 30 days after irradiation, a sensitivity comparable to that of TLD-500k, and an MMD as low as 38 μGy was successfully prepared, which will meet the fast read out and the multiple readings requirements.
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提高新开发的 LiMgPO4:Er 荧光粉的光激发发光灵敏度并改善褪色情况
为了避免衰减,之前研究中旧的 LiMgPO4:Er 的读出时间必须至少达到 20 秒。读出时间长达 20 秒,这不仅与快速 OSL 读出相矛盾,而且每次读出会消除过多的 OSL 信号,不利于 OSL 可以多次读出的要求。本研究的主要目的是在锂镁磷酸盐:铒荧光粉的 OSL 信号在辐照后趋于稳定的条件下缩短读出时间。对 OSL 特性进行了研究。为了在辐照后 30 d 内使 OSL 衰减约为 5%,本研究中新 LiMgPO4:Er 的最短积分时间为 1 s,而旧 LiMgPO4:Er 则需要 20 s。当积分时间为 1 s 时,本研究中新 LiMgPO4:Er 样品的 OSL 灵敏度约为旧 LiMgPO4:Er 样品的 2.4 倍。成功制备了一种新的 LiMgPO4:Er 荧光粉,在辐照后 30 天内,最短积分时间为 1 秒时,OSL 信号损失约为 5%,灵敏度与 TLD-500k 相当,MMD 低至 38 μGy,可满足快速读出和多次读取的要求。
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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