Universal synthesis of pure-phase IB-group Sn-based alloys with modulable electrocatalytic CO2 reduction products†

IF 4.2 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY Chemical Communications Pub Date : 2024-10-21 Epub Date: 2024-10-22 DOI:10.1039/d4cc05317f
Luyao Yang , Wenqing Zhang , Ximei Lv , Qianqian Zhao , Xiaojing Liu , Shulin Zhao , Yuhui Chen
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Abstract

We present a universal preparation method for synthesizing a range of pure-phase IB-group Sn-based alloy catalysts (Cu3Sn, Ag4Sn, and AuSn) for electrochemical reduction of CO2 to C1 product. The selectivity can be widely adjusted by altering metal composition and potential, improving the understanding of the structure–activity relationship in various Sn-based alloys.

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具有可调节的电催化二氧化碳还原产物的纯相 IB 族 Sn 基合金的通用合成方法
我们提出了一种合成一系列纯相 IB 族锡基合金催化剂(Cu3Sn、Ag4Sn 和 AuSn)的通用方法,用于将 CO2 电化学还原为 C1 产物。根据金属成分和应用电位的变化,选择性可进行广泛调整。这项研究有助于更好地理解各种锡基合金中成分与性能之间的结构-活性关系。
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来源期刊
Chemical Communications
Chemical Communications 化学-化学综合
CiteScore
8.60
自引率
4.10%
发文量
2705
审稿时长
1.4 months
期刊介绍: ChemComm (Chemical Communications) is renowned as the fastest publisher of articles providing information on new avenues of research, drawn from all the world''s major areas of chemical research.
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