Liquid Metal-Based Elastomer Composite with Selective Switchable Adhesion to Solids

IF 8.2 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2024-10-23 DOI:10.1021/acsami.4c15780
Xiaofeng Liu, Lei Jia, Jiawei Li, Ruoxi Zhao, Chao Wu, Zhongjun Cheng, Yuyan Liu, Zhenxing Lin, Zhimin Xie, Sibo Kang, Dongjie Zhang
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Abstract

Selective switchable adhesion has recently attracted much attention due to its wide applications in transfer printing, information transfer, and flexible electronics. However, selective adhesive materials often have a complex adhesion or preparation process, which limits their use. To overcome this problem, this study prepares a composite of liquid metal foam and polydimethylsiloxane (PDMS) with selective photocontrolled adhesion, which can directly adhere to solids at room temperature. Utilizing the photoinduced phase transition of liquid metals, solid adhesion can be regulated by changing the backing layer modulus of the adhesive layer. Since the phase transition process is gradually completed by heat transfer from the illuminated side to the backlight side that adheres to the solid, the melting area on the backlight side can be regulated by controlling the light time, which determines the adhesion regulation area. Therefore, the accuracy of the adhesion regulation can reach less than 0.9 mm without relying on the accuracy of the infrared light. Moreover, based on the selective switchable adhesion, the selective transfer of solids with different scales can be achieved at room temperature. The findings of this study may provide strategies for the simple preparation of selective adhesive materials and the improvement of control accuracy.

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对固体具有选择性可切换粘附力的液态金属基弹性体复合材料
最近,选择性可切换粘合剂因其在转移印刷、信息传输和柔性电子产品中的广泛应用而备受关注。然而,选择性粘合材料通常具有复杂的粘合或制备过程,从而限制了其应用。为了克服这一问题,本研究制备了一种具有选择性光控粘附力的液态金属泡沫和聚二甲基硅氧烷(PDMS)复合材料,它可以在室温下直接粘附到固体上。利用液态金属的光诱导相变,可以通过改变粘合剂层的背层模量来调节固体粘合力。由于相变过程是通过热量从照明侧传到粘附固体的背光侧而逐渐完成的,因此可以通过控制照明时间来调节背光侧的熔化面积,从而决定粘附调节面积。因此,无需依赖红外光的精确度,粘附调节的精确度就能达到小于 0.9 毫米。此外,基于选择性可切换附着力,可在室温下实现不同尺度固体的选择性转移。本研究的发现可为选择性粘合材料的简单制备和控制精度的提高提供策略。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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