Dynamic control and manipulation of near-fields using direct feedback

IF 3.5 3区 医学 Q2 CHEMISTRY, MEDICINAL ACS Medicinal Chemistry Letters Pub Date : 2024-10-24 DOI:10.1038/s41377-024-01610-2
Jacob Kher-Aldeen, Kobi Cohen, Stav Lotan, Kobi Frischwasser, Bergin Gjonaj, Shai Tsesses, Guy Bartal
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Abstract

Shaping and controlling electromagnetic fields at the nanoscale is vital for advancing efficient and compact devices used in optical communications, sensing and metrology, as well as for the exploration of fundamental properties of light-matter interaction and optical nonlinearity. Real-time feedback for active control over light can provide a significant advantage in these endeavors, compensating for ever-changing experimental conditions and inherent or accumulated device flaws. Scanning nearfield microscopy, being slow in essence, cannot provide such a real-time feedback that was thus far possible only by scattering-based microscopy. Here, we present active control over nanophotonic near-fields with direct feedback facilitated by real-time near-field imaging. We use far-field wavefront shaping to control nanophotonic patterns in surface waves, demonstrating translation and splitting of near-field focal spots at nanometer-scale precision, active toggling of different near-field angular momenta and correction of patterns damaged by structural defects using feedback enabled by the real-time operation. The ability to simultaneously shape and observe nanophotonic fields can significantly impact various applications such as nanoscale optical manipulation, optical addressing of integrated quantum emitters and near-field adaptive optics.

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利用直接反馈对近场进行动态控制和操纵
在纳米尺度上塑造和控制电磁场,对于推动光通信、传感和计量领域使用的高效紧凑型设备,以及探索光物质相互作用和光学非线性的基本特性至关重要。对光进行主动控制的实时反馈可为这些工作提供显著优势,弥补不断变化的实验条件和固有或累积的设备缺陷。扫描近场显微镜本质上速度较慢,无法提供这种实时反馈,而迄今为止只有基于散射的显微镜才能做到这一点。在这里,我们提出了纳米光子近场主动控制,并通过实时近场成像提供直接反馈。我们利用远场波前整形来控制表面波中的纳米光子图案,展示了纳米级精度的近场焦斑平移和分割、不同近场角矩的主动切换,以及利用实时操作实现的反馈来校正受结构缺陷破坏的图案。同时塑造和观察纳米光子场的能力会对各种应用产生重大影响,如纳米级光学操纵、集成量子发射器的光学寻址和近场自适应光学。
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来源期刊
ACS Medicinal Chemistry Letters
ACS Medicinal Chemistry Letters CHEMISTRY, MEDICINAL-
CiteScore
7.30
自引率
2.40%
发文量
328
审稿时长
1 months
期刊介绍: ACS Medicinal Chemistry Letters is interested in receiving manuscripts that discuss various aspects of medicinal chemistry. The journal will publish studies that pertain to a broad range of subject matter, including compound design and optimization, biological evaluation, drug delivery, imaging agents, and pharmacology of both small and large bioactive molecules. Specific areas include but are not limited to: Identification, synthesis, and optimization of lead biologically active molecules and drugs (small molecules and biologics) Biological characterization of new molecular entities in the context of drug discovery Computational, cheminformatics, and structural studies for the identification or SAR analysis of bioactive molecules, ligands and their targets, etc. Novel and improved methodologies, including radiation biochemistry, with broad application to medicinal chemistry Discovery technologies for biologically active molecules from both synthetic and natural (plant and other) sources Pharmacokinetic/pharmacodynamic studies that address mechanisms underlying drug disposition and response Pharmacogenetic and pharmacogenomic studies used to enhance drug design and the translation of medicinal chemistry into the clinic Mechanistic drug metabolism and regulation of metabolic enzyme gene expression Chemistry patents relevant to the medicinal chemistry field.
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