Exploring mechanical properties and long-term environmental impact of ceramsites derived from diverse solid wastes

IF 7.1 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Waste management Pub Date : 2024-10-24 DOI:10.1016/j.wasman.2024.10.012
Yunjie Wan, Xinyu Wu, Houhu Zhang, Yueqing Xu, Chengyan Li, Yifan Xu
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Abstract

The escalating global issue of soil pollution by heavy metals, particularly incinerated municipal solid waste fly ash (IMSWFA), necessitates effective remediation strategies. The prevailing approach for safely disposing and utilization of IMSWFA involves high-temperature sintering. In this work, we propose a cost-effective method to produce ceramsites by utilizing IMSWFA, municipal sludge (MS), contaminated soil (CS), and iron tail slag (ITS). After conducting a comprehensive analysis and comparison of outcomes obtained from orthogonal experiments and single-factor experiments, it was determined that the optimal preparation conditions for achieving desirable results are preheating at a temperature of 400 °C for 15 min followed by sintering at a temperature of 1150 °C for 10 min. The optimal ratio of raw materials for ceramsites is 15 % IMSWFA, 15 % MS, 58 % CS, and 12 % ITS. The ceramsites, prepared in accordance with the specified process and raw material ratio, exhibit remarkable properties including robust stability, minimal water absorption, reduced weight, and elevated cylindrical compressive strength. The ceramsites demonstrate an exceptionally high heavy metal loss ratio ranging from 91 % to 100 %, while exhibiting significantly lower leaching quantities of these metals compared to the raw materials. Additionally, aging tests of ceramsites were performed under UV light and acid/alkaline etching to simulate the real-world environment. This work can be utilized to investigate the long-term environmental impact of ceramsites derived from municipal solid waste (MSW), thereby making a valuable contribution to the advancement of solid waste management technology.
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探索从各种固体废物中提取的陶瓷的机械性能和长期环境影响。
重金属(尤其是焚烧过的城市固体废弃物飞灰)造成的土壤污染问题在全球范围内日益严重,因此有必要采取有效的补救策略。安全处置和利用 IMSWFA 的主流方法是高温烧结。在这项工作中,我们提出了一种利用 IMSWFA、市政污泥(MS)、污染土壤(CS)和铁尾渣(ITS)生产陶瓷石的经济有效的方法。在对正交实验和单因素实验的结果进行综合分析和比较后,确定了获得理想结果的最佳制备条件是在 400 °C 温度下预热 15 分钟,然后在 1150 °C 温度下烧结 10 分钟。陶瓷石原料的最佳比例为 15 % IMSWFA、15 % MS、58 % CS 和 12 % ITS。按照规定的工艺和原料配比制备的陶瓷石具有卓越的性能,包括稳定性强、吸水性小、重量轻和圆柱抗压强度高。陶瓷的重金属损耗率极高,从 91% 到 100%不等,同时与原材料相比,这些金属的沥滤量明显降低。此外,还在紫外线和酸碱腐蚀条件下对陶瓷石进行了老化测试,以模拟真实世界的环境。这项工作可用于研究从城市固体废物(MSW)中提取的陶瓷石料对环境的长期影响,从而为固体废物管理技术的进步做出宝贵贡献。
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来源期刊
Waste management
Waste management 环境科学-工程:环境
CiteScore
15.60
自引率
6.20%
发文量
492
审稿时长
39 days
期刊介绍: Waste Management is devoted to the presentation and discussion of information on solid wastes,it covers the entire lifecycle of solid. wastes. Scope: Addresses solid wastes in both industrialized and economically developing countries Covers various types of solid wastes, including: Municipal (e.g., residential, institutional, commercial, light industrial) Agricultural Special (e.g., C and D, healthcare, household hazardous wastes, sewage sludge)
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