Zhao Liu, Zelong Fan, Wenliang Li, Yuan Cao, Feihong Zhang, Zuoyan Qin, Zhenhua Sun, Baikui Li and Honglei Wu
{"title":"Self-powered solar-blind photodetectors based on AlN/a-Ga2O3 heterojunctions with a nanocolumnar structure on various substrates","authors":"Zhao Liu, Zelong Fan, Wenliang Li, Yuan Cao, Feihong Zhang, Zuoyan Qin, Zhenhua Sun, Baikui Li and Honglei Wu","doi":"10.1039/D4CE00826J","DOIUrl":null,"url":null,"abstract":"<p >AlN/amorphous Ga<small><sub>2</sub></small>O<small><sub>3</sub></small> heterojunction photodetectors were fabricated to achieve solar-blind UV detection. The responsivity and detectivity of the photodetector on a native substrate are 150% and 21.8% higher than those on a heterogeneous substrate at a 20 V bias, reaching 8.31 A W<small><sup>−1</sup></small> and 3.24 × 10<small><sup>14</sup></small> Jones, respectively. The built-in electric field enables self-powered UV detection without an external power supply. The addition of a nanocolumnar AlN structure significantly improved the performance of the photodetector, achieving a photo-to-dark current ratio and responsivity up to 2.11 × 10<small><sup>7</sup></small> and 9.17 mA W<small><sup>−1</sup></small> at 0 V bias. The fabricated photodetector has demonstrated self-powered and high-sensitivity UV detection.</p>","PeriodicalId":70,"journal":{"name":"CrystEngComm","volume":" 42","pages":" 6017-6024"},"PeriodicalIF":2.6000,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"CrystEngComm","FirstCategoryId":"92","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2024/ce/d4ce00826j","RegionNum":3,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
AlN/amorphous Ga2O3 heterojunction photodetectors were fabricated to achieve solar-blind UV detection. The responsivity and detectivity of the photodetector on a native substrate are 150% and 21.8% higher than those on a heterogeneous substrate at a 20 V bias, reaching 8.31 A W−1 and 3.24 × 1014 Jones, respectively. The built-in electric field enables self-powered UV detection without an external power supply. The addition of a nanocolumnar AlN structure significantly improved the performance of the photodetector, achieving a photo-to-dark current ratio and responsivity up to 2.11 × 107 and 9.17 mA W−1 at 0 V bias. The fabricated photodetector has demonstrated self-powered and high-sensitivity UV detection.