Improving the photoswitching performance of a transistor with amorphous metal oxide semiconductor thin film by a gradient annealing approach

IF 3.8 3区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Optical Materials Pub Date : 2024-10-22 DOI:10.1016/j.optmat.2024.116305
Gergely Tarsoly , Jae-Yun Lee , Sung-Jin Kim
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Abstract

Metal oxides are attracting attention as electronic mate rials in research and industry. Thin films of amorphous indium gallium zinc oxide (a-IGZO) exhibit low absorbance in the visible spectrum, making them ideal components in transparent electronics. To widen the scope of use for thin film transistor (TFT) devices based on a-IGZO in on-chip sensing applications, photoresponsive behavior has been achieved by proper engineering of the active layers by either introducing a photosensitive top layer or using a method to generate localized states inside the band gap. In this paper, we propose a bilayer structured with the use of thermal annealing of a-IGZO film at different temperatures. Thermal annealing has been shown to improve the electrical performance of the TFT devices because of the improved film quality but negatively affects the photoresponsivity by removing tarp sites that play an important role in both charge generation and photomultiplication via the photogating effect. Therefore, here we propose an a-IGZO film with a high temperature-annealed bottom layer and pristine top layer. The bottom layer plays a vital role in the charge transport behavior, resulting in a low threshold voltage and subthreshold swing similar to the device with a fully annealed film, while the photoresponse of the device is driven by the higher density of gap states in the pristine top layer. This proposed method is advantageous to previously published procedures due to the simplicity of using no additional materials and complex steps to introduce trap sites into the photoactive layer, but only differential annealing temperature.

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用梯度退火法提高非晶态金属氧化物半导体薄膜晶体管的光开关性能
金属氧化物作为电子元件在科研和工业领域备受关注。非晶铟镓锌氧化物(a-IGZO)薄膜在可见光谱中的吸光率很低,是透明电子器件的理想元件。为了拓宽基于 a-IGZO 的薄膜晶体管 (TFT) 器件在片上传感应用中的使用范围,我们通过引入光敏顶层或使用在带隙内产生局部态的方法对有源层进行适当的工程设计,从而实现了光致发光行为。在本文中,我们提出了一种在不同温度下对 a-IGZO 薄膜进行热退火的双层结构。事实证明,热退火可以提高薄膜质量,从而改善 TFT 器件的电气性能,但会对光发射率产生负面影响,因为热退火会去除在电荷生成和光放大中通过光ogating 效应发挥重要作用的 tarp 位点。因此,我们提出了一种具有高温退火底层和原始表层的 a-IGZO 薄膜。底层在电荷传输行为中起着至关重要的作用,因此阈值电压和阈下摆动较低,与完全退火薄膜的器件相似,而器件的光响应则由原始顶层中更高密度的间隙态驱动。由于无需使用额外材料和复杂步骤在光活性层中引入陷阱位点,而只需不同的退火温度,因此与之前公布的程序相比,所提出的方法更具优势。
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来源期刊
Optical Materials
Optical Materials 工程技术-材料科学:综合
CiteScore
6.60
自引率
12.80%
发文量
1265
审稿时长
38 days
期刊介绍: Optical Materials has an open access mirror journal Optical Materials: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. The purpose of Optical Materials is to provide a means of communication and technology transfer between researchers who are interested in materials for potential device applications. The journal publishes original papers and review articles on the design, synthesis, characterisation and applications of optical materials. OPTICAL MATERIALS focuses on: • Optical Properties of Material Systems; • The Materials Aspects of Optical Phenomena; • The Materials Aspects of Devices and Applications. Authors can submit separate research elements describing their data to Data in Brief and methods to Methods X.
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