A comprehensive review of covalent organic frameworks (COFs) and their derivatives in environmental pollution control

IF 40.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Chemical Society Reviews Pub Date : 2024-10-30 DOI:10.1039/d4cs00521j
Shengbo Ge, Kexin Wei, Wanxi Peng, Runzhou Huang, Esther Akinlabi, Hongyan Xia, Muhammad Wakil Shahzad, Xuehua Zhang, Ben Bin Xu, Jianchun Jiang
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Abstract

Covalent organic frameworks (COFs) have gained considerable attention due to their design possibilities as the molecular organic building blocks that can stack in an atomically precise spatial arrangement. Since the inception of COFs in 2005, there has been a continuous expansion in the product range of COFs and their derivatives. This expansion has led to the evolution of three-dimensional structures and various synthetic routes, propelling the field towards large-scale preparation of COFs and their derivatives. This review will offer a holistic analysis and comparison of the spatial structure and synthesis techniques of COFs and their derivatives. The conventional methods of COF synthesis (i.e., ultrasonic chemical, microwave, and solvothermal) are discussed alongside the synthesis strategies of new COFs and their derivatives. Furthermore, the applications of COFs and their derived materials are demonstrated in air, water, and soil pollution management such as gas capture, catalytic conversion, adsorption, and pollutant removal. Finally, this review highlights the current challenges and prospects for large-scale preparation and application of new COFs and the derived materials. In line with the United Nations Sustainable Development Goals (SDGs) and the needs of digital-enabled technologies (AI and machine learning), this review will encompass the future technical trends for COFs in environmental pollution control.

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共价有机框架(COF)及其衍生物在环境污染控制中的应用综述
共价有机框架(COFs)作为分子有机构件,能以原子精度的空间排列方式堆叠,其设计可能性已引起广泛关注。自 2005 年 COF 问世以来,COF 及其衍生物的产品范围不断扩大。这种扩展导致了三维结构和各种合成路线的演变,推动了 COFs 及其衍生物的大规模制备。本综述将对 COF 及其衍生物的空间结构和合成技术进行整体分析和比较。在讨论 COF 合成的传统方法(即超声化学法、微波法和溶热法)的同时,还将讨论新型 COF 及其衍生物的合成策略。此外,还展示了 COFs 及其衍生材料在空气、水和土壤污染治理方面的应用,如气体捕获、催化转化、吸附和污染物去除。最后,本综述强调了当前大规模制备和应用新型 COFs 及其衍生材料所面临的挑战和前景。根据联合国可持续发展目标(SDGs)和数字技术(人工智能和机器学习)的需求,本综述将涵盖 COFs 在环境污染控制方面的未来技术趋势。
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来源期刊
Chemical Society Reviews
Chemical Society Reviews 化学-化学综合
CiteScore
80.80
自引率
1.10%
发文量
345
审稿时长
6.0 months
期刊介绍: Chemical Society Reviews is published by: Royal Society of Chemistry. Focus: Review articles on topics of current interest in chemistry; Predecessors: Quarterly Reviews, Chemical Society (1947–1971); Current title: Since 1971; Impact factor: 60.615 (2021); Themed issues: Occasional themed issues on new and emerging areas of research in the chemical sciences
期刊最新文献
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