A chronicle of titanium niobium oxide materials for high-performance lithium-ion batteries: From laboratory to industry

Cancan Peng, Suzhe Liang, Ying Yu, Longhao Cao, Chao Yang, Xiaosong Liu, Kunkun Guo, Peter Müller-Buschbaum, Ya-Jun Cheng, Changhong Wang
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Abstract

Titanium niobium oxide (TiNbxO2 + 2.5x) is emerging as a promising electrode material for rechargeable lithium-ion batteries (LIBs) due to its exceptional safety characteristics, high electrochemical properties (e.g., cycling stability and rate performance), and eco-friendliness. However, several intrinsic critical drawbacks, such as relatively low electrical conductivity, significantly hinder its practical applications. Developing reliable strategies is crucial to accelerating the practical use of TiNbxO2 + 2.5x-based materials in LIBs, especially high-power LIBs. Here, we provide a chronicle review of the research progress on TiNbxO2 + 2.5x-based anodes from the early 1950s to the present, which is classified into early stage (before 2008), emerging stage (2008–2012), explosive stage (2013–2017), commercialization (2018), steady development (2018–2022), and new breakthrough stage (since 2022). In each stage, the advancements in the fundamental science and application of the TiNbxO2 + 2.5x-based anodes are reviewed, and the corresponding developing trends of TiNbxO2 + 2.5x-based anodes are summarized. Moreover, several future research directions to propel the practical use of TiNbxO2 + 2.5x anodes are suggested based on reviewing the history. This review is expected to pave the way for developing the fabrication and application of high-performance TiNbxO2 + 2.5x-based anodes for LIBs.

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用于高性能锂离子电池的钛铌氧化物材料编年史:从实验室到工业
钛铌氧化物(TiNbxO2 + 2.5x)因其卓越的安全特性、高电化学性能(如循环稳定性和速率性能)以及环保性,正逐渐成为可充电锂离子电池(LIB)的一种前景广阔的电极材料。然而,一些固有的关键缺点,如相对较低的导电性,严重阻碍了其实际应用。开发可靠的策略对于加速基于 TiNbxO2 + 2.5x 的材料在 LIB(尤其是大功率 LIB)中的实际应用至关重要。在此,我们对 20 世纪 50 年代初至今基于 TiNbxO2 + 2.5x 阳极材料的研究进展进行了编年史式的回顾,分为早期阶段(2008 年以前)、新兴阶段(2008-2012 年)、爆发阶段(2013-2017 年)、商业化阶段(2018 年)、稳定发展阶段(2018-2022 年)和新突破阶段(2022 年以后)。在每个阶段,回顾了 TiNbxO2 + 2.5x 基阳极的基础科学和应用进展,并总结了 TiNbxO2 + 2.5x 基阳极的相应发展趋势。此外,在回顾历史的基础上,还提出了推动 TiNbxO2 + 2.5x 阳极实际应用的几个未来研究方向。本综述有望为开发用于 LIB 的高性能 TiNbxO2 + 2.5x 基阳极的制造和应用铺平道路。
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Issue Information Front Cover: Carbon Neutralization, Volume 3, Issue 6, November 2024 Inside Back Cover Image: Carbon Neutralization, Volume 3, Issue 6, November 2024 Back Cover Image: Carbon Neutralization, Volume 3, Issue 6, November 2024 A chronicle of titanium niobium oxide materials for high-performance lithium-ion batteries: From laboratory to industry
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