Recent advances in luminescent metal-organic frameworks (L-MOFs) as sustainable materials for sensing of potentially toxic environmental ubiquitous explosive contaminants

IF 8.6 2区 工程技术 Q1 ENERGY & FUELS Sustainable Materials and Technologies Pub Date : 2024-10-24 DOI:10.1016/j.susmat.2024.e01155
Muhammad Asad , Muhammad Imran Anwar , Baoji Miao , Ansar Abbas , Saadat Majeed , Irshad Ahmad Mir , Muhammad Saqib Rabbani , Sameer Hussain , Sankui Xu , Mohammed A. Al-Tahan , Chuxiao Shao , Shuanghu Wang , Ayesha Younas
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Abstract

Although, the explosive materials are crucial for homeland safety and defense systems, they impose severe side effects on the environment and human health. The residues or byproducts of these hazardous materials can contaminate the environment and implies acute chronic effects on humans as well as animals. Hence, the ultrasensitive, low cost and convenient detection of widely used explosive compounds is highly desirable considering environmental pollution and increasing human health issues. Owing to their numerous features, luminescent metal-organic frameworks (L-MOFs) have gained much attention during the past few decades in the field of sensing with focus on national security, environmental monitoring, and forensic science. In this review, we have systematically described the detection of six kinds of widely used hazardous explosive compounds (nitroaromatics, nitramines, nitroalkanes, nitrate esters, peroxides and acid salts) using luminescent MOFs as the primary sensing material. The origin of fluorescence in MOFs, factors affecting the fluorescence, synthetic methods as well as various sensing mechanisms involved during the detection are discussed. Besides, most of the MOF based fluorescent probes reported in past decade for the detection of various explosive chemicals through diverse coordination interactions are summarized in tabular forms. Finally, the existing challenges and future prospects in the relevant research area are also discussed.

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将发光金属有机框架(L-MOFs)作为可持续材料用于传感具有潜在毒性的环境隐爆污染物的最新进展
尽管爆炸材料对国土安全和防御系统至关重要,但它们也对环境和人类健康造成了严重的副作用。这些危险材料的残留物或副产品会污染环境,并对人类和动物造成急性慢性影响。因此,考虑到环境污染和日益严重的人类健康问题,对广泛使用的爆炸性化合物进行超灵敏、低成本和便捷的检测是非常必要的。过去几十年来,发光金属有机框架(L-MOFs)凭借其众多特性,在以国家安全、环境监测和法医学为重点的传感领域备受关注。在这篇综述中,我们系统地介绍了以发光 MOFs 为主要传感材料检测六种广泛使用的危险爆炸性化合物(硝基芳烃、硝胺、硝基烷烃、硝酸酯、过氧化物和酸盐)的方法。本文讨论了 MOFs 荧光的起源、影响荧光的因素、合成方法以及检测过程中涉及的各种传感机制。此外,还以表格形式总结了过去十年中报道的大多数基于 MOF 的荧光探针,这些探针通过不同的配位相互作用来检测各种爆炸性化学物质。最后,还讨论了相关研究领域的现有挑战和未来前景。
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来源期刊
Sustainable Materials and Technologies
Sustainable Materials and Technologies Energy-Renewable Energy, Sustainability and the Environment
CiteScore
13.40
自引率
4.20%
发文量
158
审稿时长
45 days
期刊介绍: Sustainable Materials and Technologies (SM&T), an international, cross-disciplinary, fully open access journal published by Elsevier, focuses on original full-length research articles and reviews. It covers applied or fundamental science of nano-, micro-, meso-, and macro-scale aspects of materials and technologies for sustainable development. SM&T gives special attention to contributions that bridge the knowledge gap between materials and system designs.
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