Evidence of Different Charging Behavior of Conductive and Dielectric Materials in Low-Temperature Plasmas and a New Diagnostic for Low-Energy Electron Absorption

IF 8.1 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Physical review letters Pub Date : 2024-10-28 DOI:10.1103/physrevlett.133.185301
Armin Mengel, Franz X. Bronold, Franko Greiner
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For dielectrics, it could previously only be measured for high energies (<mjx-container ctxtmenu_counter=\"27\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(10 (6 5 0 1) 2 3 4)\"><mjx-mrow data-semantic-children=\"6,2,3,4\" data-semantic-collapsed=\"(10 (c 7 8 9) 6 2 3 4)\" data-semantic- data-semantic-owns=\"6 2 3 4\" data-semantic-role=\"text\" data-semantic-speech=\"greater than 100 e upper V\" data-semantic-type=\"punctuated\"><mjx-mrow data-semantic-added=\"true\" data-semantic-children=\"5,1\" data-semantic-content=\"0\" data-semantic- data-semantic-owns=\"5 0 1\" data-semantic-parent=\"10\" data-semantic-role=\"inequality\" data-semantic-type=\"relseq\"><mjx-mrow data-semantic-added=\"true\" data-semantic- data-semantic-parent=\"6\" data-semantic-role=\"unknown\" data-semantic-type=\"empty\"></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\"relseq,&gt;\" data-semantic-parent=\"6\" data-semantic-role=\"inequality\" data-semantic-type=\"relation\"><mjx-c>&gt;</mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"6\" data-semantic-role=\"integer\" data-semantic-type=\"number\" space=\"4\"><mjx-c noic=\"true\" style=\"padding-top: 0.642em;\">1</mjx-c><mjx-c noic=\"true\" style=\"padding-top: 0.642em;\">0</mjx-c><mjx-c style=\"padding-top: 0.642em;\">0</mjx-c></mjx-mn></mjx-mrow><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic- data-semantic-parent=\"10\" data-semantic-role=\"space\" data-semantic-type=\"text\" style='font-family: MJX-STX-ZERO, \"Helvetica Neue\", Helvetica, Roboto, Arial, sans-serif;'><mjx-utext style=\"font-size: 90.6%; padding: 0.828em 0px 0.221em; width: 3px;\" variant=\"-explicitFont\"> </mjx-utext></mjx-mtext><mjx-mtext data-semantic-annotation=\"clearspeak:unit\" data-semantic- data-semantic-parent=\"10\" data-semantic-role=\"space\" data-semantic-type=\"text\" style='font-family: MJX-STX-ZERO, \"Helvetica Neue\", Helvetica, Roboto, Arial, sans-serif;'><mjx-utext style=\"font-size: 90.6%; padding: 0.828em 0px 0.221em; width: 3px;\" variant=\"-explicitFont\"> </mjx-utext></mjx-mtext><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"10\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\" space=\"2\"><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">e</mjx-c><mjx-c style=\"padding-top: 0.657em;\">V</mjx-c></mjx-mi></mjx-mrow></mjx-math></mjx-container>), while it is well-known for metals even at energies of only a few eV. Recent theoretical investigations concerning dielectrics such as silica predict values for <mjx-container ctxtmenu_counter=\"28\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"0\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-role=\"latinletter\" data-semantic-speech=\"s\" data-semantic-type=\"identifier\"><mjx-c>𝑠</mjx-c></mjx-mi></mjx-math></mjx-container> significantly below 1. With precision charge measurements on microparticles in the sheath of a low-pressure plasma, a difference in charge between silica and gold-coated particles is found, challenging the long-standing assumption in dusty plasma physics that dielectric and metallic particles charge in the same way for the first time. Based on the measured charging difference, the low-energy sticking coefficient of silica is obtained, validating the theoretical predictions and offering a new diagnostic for the otherwise quasi-inaccessible low-energy electron sticking of dielectric materials.","PeriodicalId":20069,"journal":{"name":"Physical review letters","volume":"240 1","pages":""},"PeriodicalIF":8.1000,"publicationDate":"2024-10-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical review letters","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physrevlett.133.185301","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
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Abstract

In any physical system where a surface is hit by electrons, the sticking probability 𝑠 of the electrons is a central parameter governing, for example, the charging of the surface. For dielectrics, it could previously only be measured for high energies (>100eV), while it is well-known for metals even at energies of only a few eV. Recent theoretical investigations concerning dielectrics such as silica predict values for 𝑠 significantly below 1. With precision charge measurements on microparticles in the sheath of a low-pressure plasma, a difference in charge between silica and gold-coated particles is found, challenging the long-standing assumption in dusty plasma physics that dielectric and metallic particles charge in the same way for the first time. Based on the measured charging difference, the low-energy sticking coefficient of silica is obtained, validating the theoretical predictions and offering a new diagnostic for the otherwise quasi-inaccessible low-energy electron sticking of dielectric materials.
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低温等离子体中导电材料和介电材料不同充电行为的证据以及低能电子吸收的新诊断方法
在任何表面受到电子撞击的物理系统中,电子的粘滞概率𝑠都是控制表面充电等的核心参数。对于电介质来说,以前只能测量高能量(100 eV),而对于金属来说,即使只有几 eV 的能量,𝑠 也是众所周知的。通过对低压等离子体鞘中的微粒子进行精确的电荷测量,发现二氧化硅和镀金粒子之间存在电荷差异,首次挑战了尘埃等离子体物理学中长期存在的电介质粒子和金属粒子以相同方式充电的假设。根据测量到的电荷差异,得到了二氧化硅的低能粘滞系数,从而验证了理论预测,并为电介质材料的低能电子粘滞提供了一种新的诊断方法。
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来源期刊
Physical review letters
Physical review letters 物理-物理:综合
CiteScore
16.50
自引率
7.00%
发文量
2673
审稿时长
2.2 months
期刊介绍: Physical review letters(PRL)covers the full range of applied, fundamental, and interdisciplinary physics research topics: General physics, including statistical and quantum mechanics and quantum information Gravitation, astrophysics, and cosmology Elementary particles and fields Nuclear physics Atomic, molecular, and optical physics Nonlinear dynamics, fluid dynamics, and classical optics Plasma and beam physics Condensed matter and materials physics Polymers, soft matter, biological, climate and interdisciplinary physics, including networks
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