Memcapacitors and Memristor Characteristics of ISGE-SOT and SHE-SOT Gain-Driven MoS2:Er Ferromagnets.

IF 8.3 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2024-11-02 DOI:10.1021/acsami.4c09201
Haoqun Zeng, Xi Chen, Jianyu Ling, Hongpeng Zhang, Yu Tong, Kewei Zhang, Mingzhe Zhang
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Abstract

The enhancement of the spin-orbit torque (SOT) effect through the integration of intrinsic inverse spin galvanic effect spin-orbit torque and spin Hall effect spin-orbit torque is fundamentally dependent on the structural and material properties of the ferromagnets. Consequently, the synthesis of ferromagnets with superior structural integrity and material characteristics is of paramount importance. In this study, a gas-liquid chemical reaction, in conjunction with ultrasonic crushing, was employed to synthesize few-layer MoS2:Er nanosheets. X-ray diffraction, X-ray photoelectron spectroscopy, and energy-dispersive spectroscopy analyses confirm the successful substitution of Mo4+ by Er3+ through doping within the MoS2 lattice. Vibrating sample magnetometry and MT measurements indicate that MoS2:Er exhibits room-temperature ferromagnetism (RTFM), with the underlying mechanism elucidated through first-principles calculations. Furthermore, the unique electron density of states at the Fermi level suggests the presence of ferromagnetism in MoS2:Er. A wedge-shaped Pt/MoS2:Er/Au structure was fabricated and subsequently evaluated for current-induced SOT switching, as well as for its memcapacitor and memristor characteristics. The precession of a magnetic moment in three-dimensional space was successfully simulated by solving the Landau-Lifshitz-Gilbert-Slonczewski equation using the Mumax.

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ISGE-SOT和SHE-SOT增益驱动MoS2:Er铁磁体的薄膜电容器和薄膜晶体管特性。
通过整合固有反向自旋电偶效应自旋轨道力矩和自旋霍尔效应自旋轨道力矩来增强自旋轨道力矩(SOT)效应,从根本上说取决于铁磁体的结构和材料特性。因此,合成具有优异结构完整性和材料特性的铁磁体至关重要。本研究采用气液化学反应结合超声波粉碎的方法合成了几层 MoS2:Er 纳米片。X 射线衍射、X 射线光电子能谱和能量色散光谱分析证实,通过在 MoS2 晶格内掺杂 Er3+ 成功地取代了 Mo4+。振动样品磁力计和 MT 测量表明,MoS2:Er 具有室温铁磁性(RTFM),并通过第一原理计算阐明了其基本机制。此外,费米级独特的电子态密度也表明 MoS2:Er 中存在铁磁性。我们制作了一种楔形的 Pt/MoS2:Er/Au 结构,随后对其电流诱导的 SOT 开关及其记忆电容器和记忆晶体管特性进行了评估。通过使用 Mumax 解决 Landau-Lifshitz-Gilbert-Slonczewski 方程,成功模拟了磁矩在三维空间中的前驱现象。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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