{"title":"Materials of Value-Added Electrolysis for Green Hydrogen Production","authors":"Endalkachew Asefa Moges, Keseven Lakshmanan, Chia-Yu Chang, Wei-Sheng Liao, Fikiru Temesgen Angerasa, Woldesenbet Bafe Dilebo, Habib Gemechu Edao, Kirubel Teshome Tadele, Dessalew Dagnew Alemayehu, Baru Debtera Bejena, Chemeda Barasa Guta, Chun-Chi Chang, Meng-Che Tsai, Wei-Nien Su* and Bing Joe Hwang*, ","doi":"10.1021/acsmaterialslett.4c01173","DOIUrl":null,"url":null,"abstract":"<p >The increasing energy consumption and resulting environmental pollution present a major challenge for society. This has led to a global demand for ultrapure energy and valuable chemical products. Therefore, a sustainable and ecofriendly approach to green energy production is essential. Recently, combining anodic oxidation reactions with hydrogen evolution reactions has shown potential in transforming low-grade molecules such as alcohols (such as ethanol, methanol, ethylene glycol, and glycerol), iodide, and biomass-derived compounds. This method could replace the sluggish oxygen evolution reaction in sustainable electrochemical energy systems. This review summarizes electro-oxidation reactions that produce green hydrogen with low electricity consumption and valuable chemicals from inexpensive small-molecule oxidants. It also explores rational design approaches for catalysts, including late transition metals on carbon-based supports, metal oxides, surface engineering, and interface engineering. Finally, the current challenges and future perspectives for developing material catalysts for value-added electrolysis technologies (power-to-green hydrogen production).</p>","PeriodicalId":19,"journal":{"name":"ACS Materials Letters","volume":"6 11","pages":"4932–4954 4932–4954"},"PeriodicalIF":8.7000,"publicationDate":"2024-10-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acsmaterialslett.4c01173","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Materials Letters","FirstCategoryId":"92","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsmaterialslett.4c01173","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The increasing energy consumption and resulting environmental pollution present a major challenge for society. This has led to a global demand for ultrapure energy and valuable chemical products. Therefore, a sustainable and ecofriendly approach to green energy production is essential. Recently, combining anodic oxidation reactions with hydrogen evolution reactions has shown potential in transforming low-grade molecules such as alcohols (such as ethanol, methanol, ethylene glycol, and glycerol), iodide, and biomass-derived compounds. This method could replace the sluggish oxygen evolution reaction in sustainable electrochemical energy systems. This review summarizes electro-oxidation reactions that produce green hydrogen with low electricity consumption and valuable chemicals from inexpensive small-molecule oxidants. It also explores rational design approaches for catalysts, including late transition metals on carbon-based supports, metal oxides, surface engineering, and interface engineering. Finally, the current challenges and future perspectives for developing material catalysts for value-added electrolysis technologies (power-to-green hydrogen production).
期刊介绍：
ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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