Enhancement of Water Productivity and Energy Efficiency in Sorption-based Atmospheric Water Harvesting Systems: From Material, Component to System Level.

IF 2.9 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY ACS Earth and Space Chemistry Pub Date : 2024-11-19 Epub Date: 2024-11-04 DOI:10.1021/acsnano.4c09582
Shengxi Bai, Xiaoxue Yao, Man Yi Wong, Qili Xu, Hao Li, Kaixin Lin, Yiying Zhou, Tsz Chung Ho, Aiqiang Pan, Jianheng Chen, Yihao Zhu, Steven Wang, Chi Yan Tso
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Abstract

To address the increasingly serious water scarcity across the world, sorption-based atmospheric water harvesting (SAWH) continues to attract attention among various water production methods, due to it being less dependent on climatic and geographical conditions. Water productivity and energy efficiency are the two most important evaluation indicators. Therefore, this review aims to comprehensively and systematically summarize and discuss the water productivity and energy efficiency enhancement methods for SAWH systems based on three levels, from material to component to system. First, the material level covers the characteristics, categories, and mechanisms of different sorbents. Second, the component level focuses on the sorbent bed, regeneration energy, and condenser. Third, the system level encompasses the system design, operation, and synergetic effect generation with other mechanisms. Specifically, the key and promising improvement methods are: synthesizing composite sorbents with high water uptake, fast sorption kinetics, and low regeneration energy (material level); improving thermal insulation between the sorbent bed and condenser, utilizing renewable energy or electrical heating for desorption and multistage design (component level); achieving continuous system operation with a desired number of sorbent beds or rotational structure, and integrating with Peltier cooling or passive radiative cooling technologies (system level). In addition, applications and challenges of SAWH systems are explored, followed by potential outlooks and future perspectives. Overall, it is expected that this review article can provide promising directions and guidelines for the design and operation of SAWH systems with the aim of achieving high water productivity and energy efficiency.

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提高基于吸附的大气集水系统的水生产力和能源效率:从材料、组件到系统层面。
为解决全球日益严重的缺水问题,基于吸附技术的大气集水(SAWH)因其对气候和地理条件的依赖性较小,在各种制水方法中持续受到关注。水生产率和能源效率是两个最重要的评价指标。因此,本综述旨在从材料、组件和系统三个层面,全面系统地总结和讨论提高 SAWH 系统水生产率和能效的方法。首先,材料层面涵盖了不同吸附剂的特点、类别和机理。其次,组件层面侧重于吸附剂床、再生能源和冷凝器。第三,系统层面包括系统设计、运行以及与其他机制产生的协同效应。具体来说,关键且有前景的改进方法包括:合成具有高吸水率、快速吸附动力学和低再生能的复合吸附剂(材料层面);改善吸附剂床和冷凝器之间的隔热性能,利用可再生能源或电加热进行解吸和多级设计(组件层面);以所需数量的吸附剂床或旋转结构实现系统的连续运行,以及与珀尔帖冷却或被动辐射冷却技术相结合(系统层面)。此外,还探讨了 SAWH 系统的应用和挑战,以及潜在前景和未来展望。总之,希望这篇综述文章能为 SAWH 系统的设计和运行提供有前景的方向和指导,以实现高水生产率和能源效率。
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来源期刊
ACS Earth and Space Chemistry
ACS Earth and Space Chemistry Earth and Planetary Sciences-Geochemistry and Petrology
CiteScore
5.30
自引率
11.80%
发文量
249
期刊介绍: The scope of ACS Earth and Space Chemistry includes the application of analytical, experimental and theoretical chemistry to investigate research questions relevant to the Earth and Space. The journal encompasses the highly interdisciplinary nature of research in this area, while emphasizing chemistry and chemical research tools as the unifying theme. The journal publishes broadly in the domains of high- and low-temperature geochemistry, atmospheric chemistry, marine chemistry, planetary chemistry, astrochemistry, and analytical geochemistry. ACS Earth and Space Chemistry publishes Articles, Letters, Reviews, and Features to provide flexible formats to readily communicate all aspects of research in these fields.
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