High-Performance Triboelectric Nanogenerator Based on Silk Fibroin-MXene Composite Film for Diagnosing Insomnia Symptoms.

IF 8.2 1区 化学 Q1 CHEMISTRY, ANALYTICAL ACS Sensors Pub Date : 2024-11-22 Epub Date: 2024-11-04 DOI:10.1021/acssensors.4c00852
Xueqiang Tan, Zuyi Huang, Lu Chang, Hairun Pei, Zongchao Jia, Jimin Zheng
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Abstract

In this study, we developed a flexible, biocompatible, and high-output electrical performance triboelectric nanogenerator (TENG) employing a silk fibroin (SF)-MXene composite film (SF-MXene-F) and a PDMS film as the friction layer. The inclusion of MXene in the SF film increased its surface charge density, presenting a practical approach to designing high-performance SF composite film-based TENGs. At a MXene content of 40%, our SF-MXene composite film-based TENG (SF-MXene-FTENG) achieved optimal output electrical performance, featuring a maximum open-circuit voltage (Voc) of 418 V, a maximum short-circuit current (Isc) of 11.6 μA, and a maximum output power density of 9.92 W/m2. The Voc and power densities of the SF-MXene-FTENG surpassed previously reported optimal values for SF-based TENGs by 1.6 and 3.8 times, respectively. Furthermore, leveraging the exceptional biocompatibility and light shading performance of TENGs, we designed a wearable smart TENG eye mask capable of diagnosing insomnia symptoms and monitoring sleep quality in real time. The SF-MXene-FTENG holds promising application potential as a wearable electronic device for diagnosing sleep-related diseases.

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用于失眠症状诊断的基于蚕丝纤维素-二甲苯复合膜的高性能三电纳米发电机
在这项研究中,我们采用蚕丝纤维素(SF)-MXene 复合薄膜(SF-MXene-F)和 PDMS 薄膜作为摩擦层,开发了一种柔性、生物相容性和高输出电性能的三电纳米发电机(TENG)。在 SF 薄膜中加入 MXene 增加了其表面电荷密度,为设计基于 SF 复合薄膜的高性能 TENG 提供了一种实用方法。当 MXene 含量为 40% 时,我们基于 SF-MXene 复合薄膜的 TENG(SF-MXene-FTENG)实现了最佳输出电气性能,其最大开路电压(Voc)为 418 V,最大短路电流(Isc)为 11.6 μA,最大输出功率密度为 9.92 W/m2。SF-MXene-FTENG的Voc和功率密度分别比之前报道的基于SF的TENG最佳值高出1.6倍和3.8倍。此外,利用 TENG 的优异生物相容性和遮光性能,我们设计了一种可穿戴智能 TENG 眼罩,能够诊断失眠症状并实时监测睡眠质量。作为诊断睡眠相关疾病的可穿戴电子设备,SF-MXene-FTENG 具有广阔的应用前景。
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来源期刊
ACS Sensors
ACS Sensors Chemical Engineering-Bioengineering
CiteScore
14.50
自引率
3.40%
发文量
372
期刊介绍: ACS Sensors is a peer-reviewed research journal that focuses on the dissemination of new and original knowledge in the field of sensor science, particularly those that selectively sense chemical or biological species or processes. The journal covers a broad range of topics, including but not limited to biosensors, chemical sensors, gas sensors, intracellular sensors, single molecule sensors, cell chips, and microfluidic devices. It aims to publish articles that address conceptual advances in sensing technology applicable to various types of analytes or application papers that report on the use of existing sensing concepts in new ways or for new analytes.
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