Bright Electrically Contacted Circular Bragg Grating Resonators with Deterministically Integrated Quantum Dots.

IF 15.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY ACS Nano Pub Date : 2024-11-19 Epub Date: 2024-11-05 DOI:10.1021/acsnano.4c07820
Setthanat Wijitpatima, Normen Auler, Priyabrata Mudi, Timon Funk, Avijit Barua, Binamra Shrestha, Johannes Schall, Imad Limame, Sven Rodt, Dirk Reuter, Stephan Reitzenstein
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Abstract

Cavity-enhanced emission of electrically controlled semiconductor quantum dots (QDs) is essential in the development of bright quantum devices for real-world quantum photonic applications. Combining the circular Bragg grating (CBG) approach with a PIN-diode structure, we propose and implement designs for ridge-based electrically contacted QD-CBG resonators. Through fine-tuning of device parameters in numerical simulations and deterministic nanoprocessing, we produced electrically controlled single QD-CBG resonators with excellent electro-optical emission properties. These include multiple wavelength-tunable emission lines and a photon extraction efficiency (PEE) of up to 30.4(3.4)%, where refined numerical optimization based on experimental findings suggests a substantial improvement, promising PEE > 50%. Additionally, the developed quantum light sources yield single-photon purity reaching 99.2(2)% and photon indistinguishability of 75(5)% under quasi-resonant p-shell excitation. Our results present high-performance quantum devices with combined cavity enhancement and deterministic charge-environment controls, which are relevant for the development of photonic quantum information systems such as complex quantum repeater networks.

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带有确定性集成量子点的明亮电接触环形布拉格光栅谐振器。
电控半导体量子点(QDs)的空穴增强发射对于为现实世界的量子光子应用开发明亮的量子器件至关重要。我们将圆布拉格光栅(CBG)方法与 PIN 二极管结构相结合,提出并实现了基于脊的电接触 QD-CBG 谐振器的设计。通过数值模拟和确定性纳米加工对器件参数进行微调,我们制造出了具有优异电光发射特性的电控单QD-CBG谐振器。其中包括多条波长可调的发射线和高达 30.4(3.4)% 的光子萃取效率 (PEE),根据实验结果进行的精细数值优化表明,PEE 有望大幅提高,达到 50%。此外,所开发的量子光源在准共振 p 壳激发下的单光子纯度达到 99.2(2)%,光子不可分辨度达到 75(5)%。我们的研究成果展示了结合腔体增强和确定性电荷环境控制的高性能量子器件,这与复杂量子中继网络等光子量子信息系统的开发息息相关。
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来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
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