{"title":"Congruent Glass Composite Scintillator for Efficient High-Energy Ray Detection.","authors":"Dazhao Wang, Hongwei Li, Jingfei Chen, Dianhao Hou, Xunpiao Liu, Zhuoming Yu, Shichao Lv, Jianrong Qiu, Shifeng Zhou","doi":"10.1002/adma.202412661","DOIUrl":null,"url":null,"abstract":"<p><p>The scintillator is the most crucial component in the high-energy ray detection system. The available scintillators suffer from the insurmountable drawbacks including poor shaping ability for single crystal and ceramic and low efficiency for glass. Here, a glass composite scintillator is proposed from a congruent crystallization system which possesses both excellent processability and high scintillating yield. It can be fabricated into diverse shapes and sizes including the bulk and tiny fiber. Benefitting from the unique compositing combination with a high crystallization ratio, the glass composite exhibits a giant scintillating light yield of ≈26,000 photons per MeV. The practical application for X-ray imaging is demonstrated and a high spatial resolution of 12 l p mm<sup>-1</sup> is achieved. Furthermore, the fiber derived detector is built and the remote and micro-area detection is realized. These findings not only represent a novel design concept for the development of glass composite but also suggest a great step for expanding the scope of scintillators.</p>","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":null,"pages":null},"PeriodicalIF":27.4000,"publicationDate":"2024-11-06","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adma.202412661","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The scintillator is the most crucial component in the high-energy ray detection system. The available scintillators suffer from the insurmountable drawbacks including poor shaping ability for single crystal and ceramic and low efficiency for glass. Here, a glass composite scintillator is proposed from a congruent crystallization system which possesses both excellent processability and high scintillating yield. It can be fabricated into diverse shapes and sizes including the bulk and tiny fiber. Benefitting from the unique compositing combination with a high crystallization ratio, the glass composite exhibits a giant scintillating light yield of ≈26,000 photons per MeV. The practical application for X-ray imaging is demonstrated and a high spatial resolution of 12 l p mm-1 is achieved. Furthermore, the fiber derived detector is built and the remote and micro-area detection is realized. These findings not only represent a novel design concept for the development of glass composite but also suggest a great step for expanding the scope of scintillators.
闪烁体是高能射线探测系统中最关键的部件。现有的闪烁体存在难以克服的缺点,包括单晶和陶瓷闪烁体的成型能力差,玻璃闪烁体的效率低。本文提出了一种玻璃复合闪烁体,该闪烁体采用了同向结晶体系,具有出色的可加工性和高闪烁率。它可以制成各种形状和尺寸,包括块状和微小纤维状。得益于与高结晶比的独特复合组合,这种玻璃复合材料的闪烁光产率高达 ≈26,000 光子/兆电子伏。在 X 射线成像方面的实际应用得到了验证,并实现了 12 l p mm-1 的高空间分辨率。此外,还建立了光纤衍生探测器,实现了远程和微区探测。这些发现不仅代表了开发玻璃复合材料的新颖设计理念,而且为扩大闪烁体的应用范围迈出了一大步。
期刊介绍:
Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.