Goki Iwai, Andrea Fiorani, Chiaki Terashima and Yasuaki Einaga
{"title":"Solar light-assisted electrochemical CO2 reduction on a boron-doped diamond cathode†","authors":"Goki Iwai, Andrea Fiorani, Chiaki Terashima and Yasuaki Einaga","doi":"10.1039/D4SE00947A","DOIUrl":null,"url":null,"abstract":"<p >In this study, photoelectrochemical water oxidation with a hematite (α-Fe<small><sub>2</sub></small>O<small><sub>3</sub></small>) photoanode and electrochemical CO<small><sub>2</sub></small> reduction with a boron-doped diamond (BDD) cathode were combined to convert CO<small><sub>2</sub></small> into formic acid under 1 sun AM 1.5 simulated solar light irradiation. The faradaic efficiency of formic acid production by solar light-assisted CO<small><sub>2</sub></small> reduction reached 62% and the electrical-to-chemical energy conversion efficiency was 46%. The photo-assisted electrolysis efficiency reached 0.37%.</p>","PeriodicalId":104,"journal":{"name":"Sustainable Energy & Fuels","volume":" 22","pages":" 5271-5275"},"PeriodicalIF":5.0000,"publicationDate":"2024-10-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Sustainable Energy & Fuels","FirstCategoryId":"88","ListUrlMain":"https://pubs.rsc.org/en/content/articlelanding/2024/se/d4se00947a","RegionNum":3,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
In this study, photoelectrochemical water oxidation with a hematite (α-Fe2O3) photoanode and electrochemical CO2 reduction with a boron-doped diamond (BDD) cathode were combined to convert CO2 into formic acid under 1 sun AM 1.5 simulated solar light irradiation. The faradaic efficiency of formic acid production by solar light-assisted CO2 reduction reached 62% and the electrical-to-chemical energy conversion efficiency was 46%. The photo-assisted electrolysis efficiency reached 0.37%.
期刊介绍：
Sustainable Energy & Fuels will publish research that contributes to the development of sustainable energy technologies with a particular emphasis on new and next-generation technologies.
京公网安备 11010802042870号
京ICP备2023020795号-1
分享
求助内容：
应助结果提醒方式：
扫码关注我们
