Electrode/Electrolyte Optimization-Induced Double-Layered Architecture for High-Performance Aqueous Zinc-(Dual) Halogen Batteries

IF 26.6 1区 材料科学 Q1 Engineering Nano-Micro Letters Pub Date : 2024-11-07 DOI:10.1007/s40820-024-01551-w
Chengwang Zhou, Zhezheng Ding, Shengzhe Ying, Hao Jiang, Yan Wang, Timing Fang, You Zhang, Bing Sun, Xiao Tang, Xiaomin Liu
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Abstract

Highlights

  • A double-layered protective film based on zinc-based coordination compound and ZnF2-rich solid electrolyte interphase layer has been successfully fabricated on the zinc metal anode via electrode/electrolyte synergistic optimization.

  • The double-layered architecture can effectively modulate Zn2+ flux and suppress the zinc dendrite growth, thus facilitating the uniform zinc deposition.

  • The as-developed zinc-(dual) halogen batteries based on double-layered protective film can present high areal capacity and satisfactory cycling stability.

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电极/电解质优化--高性能水性锌-(双)卤素电池的双层结构
通过电极/电解质协同优化,在锌金属阳极上成功制备了基于锌基配位化合物和富含 ZnF2 的固体电解质相间层的双层保护膜。双层结构可有效调节 Zn2+ 通量并抑制锌枝晶的生长,从而促进锌的均匀沉积。
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来源期刊
Nano-Micro Letters
Nano-Micro Letters NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
32.60
自引率
4.90%
发文量
981
审稿时长
1.1 months
期刊介绍: Nano-Micro Letters is a peer-reviewed, international, interdisciplinary, and open-access journal published under the SpringerOpen brand. Nano-Micro Letters focuses on the science, experiments, engineering, technologies, and applications of nano- or microscale structures and systems in various fields such as physics, chemistry, biology, material science, and pharmacy.It also explores the expanding interfaces between these fields. Nano-Micro Letters particularly emphasizes the bottom-up approach in the length scale from nano to micro. This approach is crucial for achieving industrial applications in nanotechnology, as it involves the assembly, modification, and control of nanostructures on a microscale.
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