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Wearable Biodevices Based on Two-Dimensional Materials: From Flexible Sensors to Smart Integrated Systems
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-15 DOI: 10.1007/s40820-024-01597-w
Yingzhi Sun, Weiyi He, Can Jiang, Jing Li, Jianli Liu, Mingjie Liu

Highlights

  • Two-dimensional (2D) materials are highlighted for their exceptional mechanical, electrical, optical, and chemical properties, making them ideal for fabricating high-performance wearable biodevices.

  • The review categorizes cutting-edge wearable biodevices by their interactions with physical, electrophysiological, and biochemical signals, showcasing how 2D materials enhance these devices' functionality, mainly including self-powering and human-machine interaction.

  • 2D materials enable multifunctional, high-performance biodevices, integrating self-powered systems, treatment platforms, and human-machine interactions, though challenges remain in practical applications.

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引用次数: 0
Correction: Self-Assembly of Binderless MXene Aerogel for Multiple-Scenario and Responsive Phase Change Composites with Ultrahigh Thermal Energy Storage Density and Exceptional Electromagnetic Interference Shielding
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-15 DOI: 10.1007/s40820-024-01582-3
Chuanbiao Zhu, Yurong Hao, Hao Wu, Mengni Chen, Bingqing Quan, Shuang Liu, Xinpeng Hu, Shilong Liu, Qinghong Ji, Xiang Lu, Jinping Qu
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引用次数: 0
Correction: A Broad Range Triboelectric Stiffness Sensor for Variable Inclusions Recognition
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-14 DOI: 10.1007/s40820-024-01614-y
Ziyi Zhao, Zhentan Quan, Huaze Tang, Qinghao Xu, Hongfa Zhao, Zihan Wang, Ziwu Song, Shoujie Li, Ishara Dharmasena, Changsheng Wu, Wenbo Ding
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引用次数: 0
Tuning Isomerism Effect in Organic Bulk Additives Enables Efficient and Stable Perovskite Solar Cells
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-10 DOI: 10.1007/s40820-024-01613-z
Qi Zhang, Qiangqiang Zhao, Han Wang, Yiguo Yao, Lei Li, Yulin Wei, Ruida Xu, Chenyang Zhang, Erik O. Shalenov, Yongguang Tu, Kai Wang, Mingjia Xiao

Highlights

  • By anchoring the perovskite sites with the functional groups of CzBP (P = O···Pb, N–H···I and P = O···N–H), the bulk nonradiative recombination is suppressed and ion migration is inhibited. Doping perovskite films with CzBP led to enhanced intercrystallite interactions in the bulk and improved photoluminescence quantum yield.

  • Using a typical electron-rich moiety as the π-linker to replace the classic alkyl spacer in CzBP facilitated the charge-carrier transport processes and the passivation effect of carbazole further contributed to high VOC. The optimized 2,7-CzBP-treated device achieves the highest power conversion efficiency (PCE) of 25.88%, with VOC of 1.189 V for 0.090 cm2 and the perovskite solar cell module with a PCE of 21.04% for 14 cm2.

  • For 2,7-CzBP, the more extended conjugation and the more linear molecular geometry result in a more effective improvement in the performance.

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引用次数: 0
Advancements in Passive Wireless Sensing Systems in Monitoring Harsh Environment and Healthcare Applications
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-09 DOI: 10.1007/s40820-024-01599-8
Wei Yue, Yunjian Guo, Jong‐Chul Lee, Enkhzaya Ganbold, Jia-Kang Wu, Yang Li, Cong Wang, Hyun Soo Kim, Young-Kee Shin, Jun-Ge Liang, Eun-Seong Kim, Nam-Young Kim

Recent advancements in passive wireless sensor technology have significantly extended the application scope of sensing, particularly in challenging environments for monitoring industry and healthcare applications. These systems are equipped with battery-free operation, wireless connectivity, and are designed to be both miniaturized and lightweight. Such features enable the safe, real-time monitoring of industrial environments and support high-precision physiological measurements in confined internal body spaces and on wearable epidermal devices. Despite the exploration into diverse application environments, the development of a systematic and comprehensive research framework for system architecture remains elusive, which hampers further optimization of these systems. This review, therefore, begins with an examination of application scenarios, progresses to evaluate current system architectures, and discusses the function of each component—specifically, the passive sensor module, the wireless communication model, and the readout module—within the context of key implementations in target sensing systems. Furthermore, we present case studies that demonstrate the feasibility of proposed classified components for sensing scenarios, derived from this systematic approach. By outlining a research trajectory for the application of passive wireless systems in sensing technologies, this paper aims to establish a foundation for more advanced, user-friendly applications.

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引用次数: 0
Plant Cell Wall-Like Soft Materials: Micro- and Nanoengineering, Properties, and Applications
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-08 DOI: 10.1007/s40820-024-01569-0
Roya Koshani, Mica L. Pitcher, Jingyi Yu, Christine L. Mahajan, Seong H. Kim, Amir Sheikhi

Highlights

  • This review provides a detailed account of engineered plant cell wall (CW)-mimetic soft materials, which are designed to replicate the intricate composition, structure, and mechanical properties of natural plant CWs.

  • Experimental methods to create CW-like materials are reviewed, and relevant characterization techniques, including mechanical, chemical, structural, and morphological analyses, are discussed.

  •  The applications of CW-like materials in several fields, including food packaging, edible films, drug delivery, construction materials, and biocatalysis are highlighted.

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引用次数: 0
Photolithographic Microfabrication of Microbatteries for On-Chip Energy Storage
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-08 DOI: 10.1007/s40820-024-01625-9
Yuan Ma, Sen Wang, Zhong-Shuai Wu

Microbatteries (MBs) are crucial to power miniaturized devices for the Internet of Things. In the evolutionary journey of MBs, fabrication technology emerges as the cornerstone, guiding the intricacies of their configuration designs, ensuring precision, and facilitating scalability for mass production. Photolithography stands out as an ideal technology, leveraging its unparalleled resolution, exceptional design flexibility, and entrenched position within the mature semiconductor industry. However, comprehensive reviews on its application in MB development remain scarce. This review aims to bridge that gap by thoroughly assessing the recent status and promising prospects of photolithographic microfabrication for MBs. Firstly, we delve into the fundamental principles and step-by-step procedures of photolithography, offering a nuanced understanding of its operational mechanisms and the criteria for photoresist selection. Subsequently, we highlighted the specific roles of photolithography in the fabrication of MBs, including its utilization as a template for creating miniaturized micropatterns, a protective layer during the etching process, a mold for soft lithography, a constituent of MB active component, and a sacrificial layer in the construction of micro-Swiss-roll structure. Finally, the review concludes with a summary of the key challenges and future perspectives of MBs fabricated by photolithography, providing comprehensive insights and sparking research inspiration in this field.

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引用次数: 0
Local Strain Engineering of Two-Dimensional Transition Metal Dichalcogenides Towards Quantum Emitters
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-08 DOI: 10.1007/s40820-024-01611-1
Ruoqi Ai, Ximin Cui, Yang Li, Xiaolu Zhuo

Highlights

  • Methods for creating the local deformation in two-dimensional transition metal dichalcogenides (2D TMDCs) are introduced.

  • Modulations of local strain on their optical properties and excitonic behaviors are discussed.

  • Quantum emitters based on strained 2D TMDCs and other applications are presented.

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引用次数: 0
Biomimetic Micro-Nanostructured Evaporator with Dual-Transition-Metal MXene for Efficient Solar Steam Generation and Multifunctional Salt Harvesting
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2025-01-06 DOI: 10.1007/s40820-024-01612-0
Ruiqi Xu, Hongzhi Cui, Na Wei, Yang Yu, Lin Dai, Xiaohua Chen

Highlights

  • The design of composite membrane with biomimetic micro-nanostructured superhydrophobic surface and (V1/2Mo1/2)2C MXene photothermal nanomaterials.

  • The double‐transition‐metal (V1/2Mo1/2)2CTx MXene exhibits enhanced photothermal conversion performance via the elevated joint densities of states.

  • The (V1/2Mo1/2)2CTx MXene-200 composite membrane achieves an evaporation rate of 2.23 kg m−2 h−1 under one sun, directed salt harvesting, and excellent multifunctionality of anti-/de-icing, anti-fouling, and antibacterial.

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引用次数: 0
Ti3C2Tx Composite Aerogels Enable Pressure Sensors for Dialect Speech Recognition Assisted by Deep Learning
IF 26.6 1区 材料科学 Q1 Engineering Pub Date : 2024-12-30 DOI: 10.1007/s40820-024-01605-z
Yanan Xiao, He Li, Tianyi Gu, Xiaoteng Jia, Shixiang Sun, Yong Liu, Bin Wang, He Tian, Peng Sun, Fangmeng Liu, Geyu Lu

Highlights

  • Emphasized the innovation in both the material design and methodology between the sensing performance and mechanical properties.

  • The composite aerogel pressure sensors exhibited low hysteresis (13.69%), wide detection range (6.25 Pa-1200 kPa), and cyclic stability to acquire stable and accurate pronunciation signals.

  • Over 6888 and 4158 pronunciation signals were collected by the pressure sensor and utilized for training the convolutional neural network model, allowing for accurate recognition of six dialects (96.2% accuracy) and seven words (96.6% accuracy).

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引用次数: 0
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Nano-Micro Letters
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