Banasree Sadhukhan, Anders Bergman, Patrik Thunström, Manuel Pereiro Lopez, Olle Eriksson, Anna Delin
{"title":"Topological magnon in exchange frustration driven incommensurate spin spiral of kagome-latticeYMn6Sn6","authors":"Banasree Sadhukhan, Anders Bergman, Patrik Thunström, Manuel Pereiro Lopez, Olle Eriksson, Anna Delin","doi":"10.1103/physrevb.110.174412","DOIUrl":null,"url":null,"abstract":"<mjx-container ctxtmenu_counter=\"39\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(7 (2 0 1) 6 (5 3 4))\"><mjx-mrow data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"2,5\" data-semantic-content=\"6\" data-semantic- data-semantic-owns=\"2 6 5\" data-semantic-role=\"implicit\" data-semantic-speech=\"upper Y upper M n 6 upper S n 6\" data-semantic-type=\"infixop\"><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-owns=\"0 1\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">Y</mjx-c><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">M</mjx-c><mjx-c style=\"padding-top: 0.657em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"7\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-msub data-semantic-children=\"3,4\" data-semantic- data-semantic-owns=\"3 4\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\" space=\"2\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.669em;\">S</mjx-c><mjx-c style=\"padding-top: 0.669em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-math></mjx-container> consists of two types of Mn-based kagome planes stacked along the <mjx-container ctxtmenu_counter=\"40\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"0\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-role=\"latinletter\" data-semantic-speech=\"c\" data-semantic-type=\"identifier\"><mjx-c>𝑐</mjx-c></mjx-mi></mjx-math></mjx-container>-axis having a complex magnetic interaction. We report a spin reconstruction in <mjx-container ctxtmenu_counter=\"41\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(7 (2 0 1) 6 (5 3 4))\"><mjx-mrow data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"2,5\" data-semantic-content=\"6\" data-semantic- data-semantic-owns=\"2 6 5\" data-semantic-role=\"implicit\" data-semantic-speech=\"upper Y upper M n 6 upper S n 6\" data-semantic-type=\"infixop\"><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-owns=\"0 1\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">Y</mjx-c><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">M</mjx-c><mjx-c style=\"padding-top: 0.657em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"7\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-msub data-semantic-children=\"3,4\" data-semantic- data-semantic-owns=\"3 4\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\" space=\"2\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.669em;\">S</mjx-c><mjx-c style=\"padding-top: 0.669em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-math></mjx-container> from ferromagnetic (FM) into a combination of two incommensurate spin spirals (SSs) originating from two different types of Mn kagome planes driven by frustrated magnetic exchanges along the <mjx-container ctxtmenu_counter=\"42\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"0\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-role=\"latinletter\" data-semantic-speech=\"c\" data-semantic-type=\"identifier\"><mjx-c>𝑐</mjx-c></mjx-mi></mjx-math></mjx-container>-axis with the inclusion of the Hubbard <mjx-container ctxtmenu_counter=\"43\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"0\"><mjx-mi data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"italic\" data-semantic- data-semantic-role=\"latinletter\" data-semantic-speech=\"upper U\" data-semantic-type=\"identifier\"><mjx-c>𝑈</mjx-c></mjx-mi></mjx-math></mjx-container>. The pitch angle and wave vector of the incommensurate SSs are <mjx-container ctxtmenu_counter=\"44\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(8 (7 6 0 1) 2 (5 3 4))\"><mjx-mrow data-semantic-children=\"7,2,5\" data-semantic-content=\"2\" data-semantic- data-semantic-owns=\"7 2 5\" data-semantic-role=\"sequence\" data-semantic-speech=\"tilde 89 period 3 Superscript ring\" data-semantic-type=\"punctuated\"><mjx-mrow data-semantic-added=\"true\" data-semantic-children=\"6,1\" data-semantic-content=\"0\" data-semantic- data-semantic-owns=\"6 0 1\" data-semantic-parent=\"8\" data-semantic-role=\"equality\" data-semantic-type=\"relseq\"><mjx-mrow data-semantic-added=\"true\" data-semantic- data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"empty\"></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\"relseq,∼\" data-semantic-parent=\"7\" data-semantic-role=\"equality\" data-semantic-type=\"relation\"><mjx-c>∼</mjx-c></mjx-mo><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"7\" data-semantic-role=\"integer\" data-semantic-type=\"number\" space=\"4\"><mjx-c noic=\"true\" style=\"padding-top: 0.647em;\">8</mjx-c><mjx-c style=\"padding-top: 0.647em;\">9</mjx-c></mjx-mn></mjx-mrow><mjx-mo data-semantic- data-semantic-operator=\"punctuated\" data-semantic-parent=\"8\" data-semantic-role=\"fullstop\" data-semantic-type=\"punctuation\"><mjx-c>.</mjx-c></mjx-mo><mjx-msup data-semantic-children=\"3,4\" data-semantic- data-semantic-owns=\"3 4\" data-semantic-parent=\"8\" data-semantic-role=\"integer\" data-semantic-type=\"superscript\" space=\"2\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\"><mjx-c>3</mjx-c></mjx-mn><mjx-script style=\"vertical-align: 0.363em;\"><mjx-mo data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\" size=\"s\"><mjx-c>∘</mjx-c></mjx-mo></mjx-script></mjx-msup></mjx-mrow></mjx-math></mjx-container> and <mjx-container ctxtmenu_counter=\"45\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"0\"><mjx-mo data-semantic- data-semantic-role=\"equality\" data-semantic-speech=\"tilde\" data-semantic-type=\"relation\"><mjx-c>∼</mjx-c></mjx-mo></mjx-math></mjx-container> (0 0 0.248), respectively, which are in excellent agreement with the experiment. We employ an effective model Hamiltonian constructed out of exchange interactions to capture the experimentally observed nonequivalent nature of the two incommensurate SSs which also explain the FM-SS crossover due to antiferromagntic spin exchange with correlation. We further report the existence of a topological magnon with spin-orbit coupling in the incommensurate SS phase of <mjx-container ctxtmenu_counter=\"46\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(7 (2 0 1) 6 (5 3 4))\"><mjx-mrow data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"2,5\" data-semantic-content=\"6\" data-semantic- data-semantic-owns=\"2 6 5\" data-semantic-role=\"implicit\" data-semantic-speech=\"upper Y upper M n 6 upper S n 6\" data-semantic-type=\"infixop\"><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-owns=\"0 1\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">Y</mjx-c><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">M</mjx-c><mjx-c style=\"padding-top: 0.657em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"7\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-msub data-semantic-children=\"3,4\" data-semantic- data-semantic-owns=\"3 4\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\" space=\"2\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.669em;\">S</mjx-c><mjx-c style=\"padding-top: 0.669em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-math></mjx-container> by calculating the topological invariants and Berry curvature profile. The location of the Dirac magnon in the energy landscape at 73 meV matches with another experimental report. We demonstrate the accuracy of our results by highlighting the experimental features in <mjx-container ctxtmenu_counter=\"47\" ctxtmenu_oldtabindex=\"1\" jax=\"CHTML\" overflow=\"linebreak\" role=\"tree\" sre-explorer- style=\"font-size: 100.7%;\" tabindex=\"0\"><mjx-math data-semantic-structure=\"(7 (2 0 1) 6 (5 3 4))\"><mjx-mrow data-semantic-annotation=\"clearspeak:unit\" data-semantic-children=\"2,5\" data-semantic-content=\"6\" data-semantic- data-semantic-owns=\"2 6 5\" data-semantic-role=\"implicit\" data-semantic-speech=\"upper Y upper M n 6 upper S n 6\" data-semantic-type=\"infixop\"><mjx-msub data-semantic-children=\"0,1\" data-semantic- data-semantic-owns=\"0 1\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">Y</mjx-c><mjx-c noic=\"true\" style=\"padding-top: 0.657em;\">M</mjx-c><mjx-c style=\"padding-top: 0.657em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"2\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub><mjx-mo data-semantic-added=\"true\" data-semantic- data-semantic-operator=\"infixop,\" data-semantic-parent=\"7\" data-semantic-role=\"multiplication\" data-semantic-type=\"operator\"><mjx-c></mjx-c></mjx-mo><mjx-msub data-semantic-children=\"3,4\" data-semantic- data-semantic-owns=\"3 4\" data-semantic-parent=\"7\" data-semantic-role=\"unknown\" data-semantic-type=\"subscript\" space=\"2\"><mjx-mi data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"unknown\" data-semantic-type=\"identifier\"><mjx-c noic=\"true\" style=\"padding-top: 0.669em;\">S</mjx-c><mjx-c style=\"padding-top: 0.669em;\">n</mjx-c></mjx-mi><mjx-script style=\"vertical-align: -0.15em;\"><mjx-mn data-semantic-annotation=\"clearspeak:simple\" data-semantic-font=\"normal\" data-semantic- data-semantic-parent=\"5\" data-semantic-role=\"integer\" data-semantic-type=\"number\" size=\"s\"><mjx-c>6</mjx-c></mjx-mn></mjx-script></mjx-msub></mjx-mrow></mjx-math></mjx-container>.","PeriodicalId":20082,"journal":{"name":"Physical Review B","volume":"18 1","pages":""},"PeriodicalIF":3.7000,"publicationDate":"2024-11-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review B","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physrevb.110.174412","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"Physics and Astronomy","Score":null,"Total":0}
引用次数: 0
Abstract
YMn6Sn6 consists of two types of Mn-based kagome planes stacked along the 𝑐-axis having a complex magnetic interaction. We report a spin reconstruction in YMn6Sn6 from ferromagnetic (FM) into a combination of two incommensurate spin spirals (SSs) originating from two different types of Mn kagome planes driven by frustrated magnetic exchanges along the 𝑐-axis with the inclusion of the Hubbard 𝑈. The pitch angle and wave vector of the incommensurate SSs are ∼89.3∘ and ∼ (0 0 0.248), respectively, which are in excellent agreement with the experiment. We employ an effective model Hamiltonian constructed out of exchange interactions to capture the experimentally observed nonequivalent nature of the two incommensurate SSs which also explain the FM-SS crossover due to antiferromagntic spin exchange with correlation. We further report the existence of a topological magnon with spin-orbit coupling in the incommensurate SS phase of YMn6Sn6 by calculating the topological invariants and Berry curvature profile. The location of the Dirac magnon in the energy landscape at 73 meV matches with another experimental report. We demonstrate the accuracy of our results by highlighting the experimental features in YMn6Sn6.
期刊介绍:
Physical Review B (PRB) is the world’s largest dedicated physics journal, publishing approximately 100 new, high-quality papers each week. The most highly cited journal in condensed matter physics, PRB provides outstanding depth and breadth of coverage, combined with unrivaled context and background for ongoing research by scientists worldwide.
PRB covers the full range of condensed matter, materials physics, and related subfields, including:
-Structure and phase transitions
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-Magnetism
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-Surfaces, nanoscience, and two-dimensional materials
-Topological states of matter