Self-assembled porous salt crystals for solar-powered crystallization

IF 32.4 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Energy & Environmental Science Pub Date : 2024-11-12 DOI:10.1039/d4ee04741a
Jie Yu, Lenan Zhang, Jintong Gao, Wenyu Han, Ruzhu Wang, Zhenyuan Xu
{"title":"Self-assembled porous salt crystals for solar-powered crystallization","authors":"Jie Yu, Lenan Zhang, Jintong Gao, Wenyu Han, Ruzhu Wang, Zhenyuan Xu","doi":"10.1039/d4ee04741a","DOIUrl":null,"url":null,"abstract":"Thermally localized solar evaporation has been recognized as an efficient and suitable pathway for desalination and brine treatment. However, the annoying salt crystallization inside the porous evaporator brings challenges for hypersaline brine evaporation. Here we argue that salt crystals can serve as an ideal structure for evaporation with proper manipulations. Taking advantage of the self-amplifying salt creeping and efflorescence effects, the salt crystals self-assemble to form a hierarchical porous salt evaporator (HPSE), enabling passive liquid supply and efficient evaporation. With a low-cost, solar-powered device based on HPSE, we achieve stable evaporation and crystallization when treating the hypersaline brine with 27.3 wt% salinity under one-sun illumination, resulting in a high evaporation rate of 18.78 kg m-2 h-1. This work bridges the important knowledge gap between fundamental salt crystallization and brine treatment, paving a path toward sustainable water economy.","PeriodicalId":72,"journal":{"name":"Energy & Environmental Science","volume":null,"pages":null},"PeriodicalIF":32.4000,"publicationDate":"2024-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Energy & Environmental Science","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1039/d4ee04741a","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Thermally localized solar evaporation has been recognized as an efficient and suitable pathway for desalination and brine treatment. However, the annoying salt crystallization inside the porous evaporator brings challenges for hypersaline brine evaporation. Here we argue that salt crystals can serve as an ideal structure for evaporation with proper manipulations. Taking advantage of the self-amplifying salt creeping and efflorescence effects, the salt crystals self-assemble to form a hierarchical porous salt evaporator (HPSE), enabling passive liquid supply and efficient evaporation. With a low-cost, solar-powered device based on HPSE, we achieve stable evaporation and crystallization when treating the hypersaline brine with 27.3 wt% salinity under one-sun illumination, resulting in a high evaporation rate of 18.78 kg m-2 h-1. This work bridges the important knowledge gap between fundamental salt crystallization and brine treatment, paving a path toward sustainable water economy.
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
用于太阳能结晶的自组装多孔盐晶体
热局部太阳能蒸发已被公认为是海水淡化和盐水处理的一种高效、合适的途径。然而,多孔蒸发器内部恼人的盐结晶给高盐度盐水蒸发带来了挑战。在此,我们认为盐结晶可以作为一种理想的蒸发结构,只要操作得当。利用盐的自放大蠕变和风化效应,盐晶体可自组装形成分层多孔盐蒸发器(HPSE),从而实现无源液体供应和高效蒸发。利用基于 HPSE 的低成本太阳能供电装置,我们在单太阳光照下处理含盐量为 27.3 wt% 的高盐度盐水时,实现了稳定的蒸发和结晶,蒸发率高达 18.78 kg m-2 h-1。这项研究填补了基础盐结晶和盐水处理之间的重要知识空白,为实现可持续水经济铺平了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
Energy & Environmental Science
Energy & Environmental Science 化学-工程:化工
CiteScore
50.50
自引率
2.20%
发文量
349
审稿时长
2.2 months
期刊介绍: Energy & Environmental Science, a peer-reviewed scientific journal, publishes original research and review articles covering interdisciplinary topics in the (bio)chemical and (bio)physical sciences, as well as chemical engineering disciplines. Published monthly by the Royal Society of Chemistry (RSC), a not-for-profit publisher, Energy & Environmental Science is recognized as a leading journal. It boasts an impressive impact factor of 8.500 as of 2009, ranking 8th among 140 journals in the category "Chemistry, Multidisciplinary," second among 71 journals in "Energy & Fuels," second among 128 journals in "Engineering, Chemical," and first among 181 scientific journals in "Environmental Sciences." Energy & Environmental Science publishes various types of articles, including Research Papers (original scientific work), Review Articles, Perspectives, and Minireviews (feature review-type articles of broad interest), Communications (original scientific work of an urgent nature), Opinions (personal, often speculative viewpoints or hypotheses on current topics), and Analysis Articles (in-depth examination of energy-related issues).
期刊最新文献
Multifunctional zeolite film enables stable high-voltage operation of LiCoO2 cathode Efficient Fully Textured Perovskite Silicon Tandems with Thermally Evaporated Hole Transporting Materials Scalable electrified cementitious materials production and recycling High triboelectrification and charge collection efficiency of direct current triboelectric nanogenerator achieved by tri-synergistic enhancement strategy A self-adsorption molecule passivated interface enables efficient and stable lithium metal batteries
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1