Low-Velocity Impact Resistance and Compression After Impact Strength of Thermoplastic Nanofiber Toughened Carbon/Epoxy Composites with Different Layups.

IF 4.7 3区 工程技术 Q1 POLYMER SCIENCE Polymers Pub Date : 2024-10-30 DOI:10.3390/polym16213060
Timo Meireman, Erik Verboven, Mathias Kersemans, Wim Van Paepegem, Karen De Clerck, Lode Daelemans
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Abstract

This study investigates the effectiveness of polyether block amide (PEBA) thermoplastic elastomeric nanofibers in reducing low-velocity impact damage across three carbon fiber composite lay-up configurations: a cross-ply [0°/90°]2s (CP) and a quasi-isotropic [0°/45°/90°/-45°]s (QI) lay-up utilizing unidirectional plies, and a stacked woven [(0°,90°)]4s (W) lay-up using twill woven fabric plies. The flexural strength and interlaminar shear strength of the composites remained unaffected by the addition of nanofibers: around 750 MPa and 63 MPa for CP, 550 MPa and 58 MPa for QI, and 650 MPa and 50 MPa for W, respectively. The incorporation of nanofibers in the interlaminar regions resulted in a substantial reduction in projected damage area, ranging from 30% to 50% reduction over an impact energy range of 5-20 J. Microscopic analysis showed that especially the delamination damage decreased in toughened composites, while intralaminar damage remained similar for the cross-ply and quasi-isotropic lay-ups and decreased only in the woven lay-up. This agrees with the broad body of research that shows that interleaved nanofibers result in a higher delamination resistance due to toughening mechanisms related to nanofiber bridging of cracks. Despite their ability to mitigate delamination during impact, nanofibers showed limited positive effects on Compression After Impact (CAI) strength in quasi-isotropic and cross-ply composites. Interestingly, only the woven fabric composites demonstrated improved CAI strength, with a 12% improvement on average over the impact energy range, attributed to a reduction in both interlaminar and intralaminar damage. This study indicates the critical role of fiber integrity over delamination size in determining CAI performance, suggesting that the delaminations are not sufficiently large to induce buckling of sub-layers, thereby minimizing the effect of nanofiber toughening on the CAI strength.

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不同层叠结构的热塑性纳米纤维增韧碳/环氧树脂复合材料的低速抗冲击性和压缩后冲击强度
本研究调查了聚醚嵌段酰胺(PEBA)热塑性弹性体纳米纤维在三种碳纤维复合材料铺层结构中减少低速冲击损伤的效果:利用单向层的交叉层 [0°/90°]2s (CP) 和准各向同性 [0°/45°/90°/-45°]s (QI) 铺层,以及利用斜纹编织层的叠层编织 [(0°,90°)]4s (W)铺层。复合材料的抗弯强度和层间剪切强度不受纳米纤维添加量的影响:CP 分别为 750 MPa 和 63 MPa,QI 分别为 550 MPa 和 58 MPa,W 分别为 650 MPa 和 50 MPa。显微分析表明,增韧复合材料中的分层损伤尤其减少,而层内损伤在交叉层叠和准各向同性层叠中保持相似,仅在编织层叠中有所减少。这与大量研究结果一致,这些研究结果表明,由于纳米纤维桥接裂缝的增韧机制,交错纳米纤维具有更高的抗分层能力。尽管纳米纤维能够减轻冲击过程中的分层,但对准各向同性和交叉层复合材料的冲击后压缩(CAI)强度的积极影响有限。有趣的是,只有编织物复合材料的 CAI 强度有所提高,在冲击能量范围内平均提高了 12%,这归因于层间和层内损伤的减少。这项研究表明,在决定 CAI 性能方面,纤维的完整性比分层大小起着关键作用,这表明分层的大小不足以引起子层的屈曲,从而最大限度地降低了纳米纤维增韧对 CAI 强度的影响。
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来源期刊
Polymers
Polymers POLYMER SCIENCE-
CiteScore
8.00
自引率
16.00%
发文量
4697
审稿时长
1.3 months
期刊介绍: Polymers (ISSN 2073-4360) is an international, open access journal of polymer science. It publishes research papers, short communications and review papers. Our aim is to encourage scientists to publish their experimental and theoretical results in as much detail as possible. Therefore, there is no restriction on the length of the papers. The full experimental details must be provided so that the results can be reproduced. Polymers provides an interdisciplinary forum for publishing papers which advance the fields of (i) polymerization methods, (ii) theory, simulation, and modeling, (iii) understanding of new physical phenomena, (iv) advances in characterization techniques, and (v) harnessing of self-assembly and biological strategies for producing complex multifunctional structures.
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