Hetero-Dimensional Micro-Nano Architectures Toward Electromagnetic Devices and Hybrid Energy Transport

IF 19 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Advanced Functional Materials Pub Date : 2024-11-14 DOI:10.1002/adfm.202417972
Qi Zheng, Jing-Qi Wang, Wen-Qiang Cao, Hua-Zhang Zhai, Mao-Sheng Cao
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Abstract

Human spaceflight, lunar exploration projects, and interstellar travel are the grand visions of human exploration of the universe. However, the energy sustainability of these projects is a concern. Electromagnetic functional materials and devices are expected to fulfill their potential in electronic communication and energy utilization. Herein, hetero-dimensional micro-nano architectures composed of Cu3Se2 microspheres and reduced graphene oxide (rGO) sheets are fabricated for the first time by the sacrificial template method, anion substitution engineering, electrostatic adsorption, and reduction-oxidation reaction. Based on the excellent electromagnetic response of the composites, they exhibit strong and ultra-wide microwave absorption ability with the effective absorption bandwidth (EAB) reaching 8.24 GHz at a thickness of 2.2 mm. In addition, an electromagnetic metamaterial with an EAB to ≈13.5 GHz is proposed, exhibiting significant properties. More significantly, the composites can be used to construct a range of electromagnetic devices: a spiral antenna with adjustable return loss and gain, with a maximum gain of up to 2.5 dBi; a microstrip power divider that can efficiently split the input signal into four equal parts and output it; a hybridized energy transport device can convert and store electromagnetic energy. This work provides new inspiration for electromagnetic protection, electronic communication, and energy development.

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面向电磁设备和混合能源传输的异维微纳米结构
载人航天、探月工程和星际旅行是人类探索宇宙的宏伟愿景。然而,这些项目的能源可持续性令人担忧。电磁功能材料和器件有望在电子通信和能源利用方面发挥其潜力。本文通过牺牲模板法、阴离子置换工程、静电吸附和还原氧化反应,首次制备了由 Cu3Se2 微球和还原氧化石墨烯(rGO)片组成的异维微纳米结构。基于复合材料优异的电磁响应,它们表现出了强大的超宽微波吸收能力,在厚度为 2.2 毫米时,有效吸收带宽(EAB)达到 8.24 GHz。此外,还提出了一种电磁超材料,其有效吸收带宽(EAB)达到≈13.5 GHz,表现出显著的特性。更重要的是,这种复合材料可用于构建一系列电磁设备:回波损耗和增益可调的螺旋天线,最大增益可达 2.5 dBi;可有效地将输入信号分成四等分并输出的微带功率分配器;可转换和存储电磁能的混合能量传输设备。这项工作为电磁防护、电子通信和能源开发提供了新的灵感。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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