Flame structure of single aluminum droplets burning in hot steam-dominated flows

IF 5.8 2区 工程技术 Q2 ENERGY & FUELS Combustion and Flame Pub Date : 2024-11-11 DOI:10.1016/j.combustflame.2024.113838
Zhiyong Wu , Can Ruan , Yue Qiu , Mehdi Stiti , Shijie Xu , Niklas Jüngst , Edouard Berrocal , Marcus Aldén , Xue-Song Bai , Zhongshan Li
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Abstract

In this work, a specially designed experimental setup is employed to study the ignition and combustion of single aluminum droplets in hot steam-dominated flows. The transient burning behaviors of Al droplets of different sizes are characterized by simultaneously visualizing the flame incandescence and droplet shadowgraphs with two high-speed cameras at high magnification. The combustion process can be described in three stages: Al ignition and droplet generation, droplet evaporation and flame development, and steady combustion. During the steady combustion stage, a bright flame sheet, characterized by a narrow layer of dense nano-micron-sized alumina droplets, encapsulates the Al droplet core. The flame sheet composed of alumina droplets is located on a stagnation plane where the radial velocities relative to the droplet core are close to zero. The standoff ratio is around two, and it slightly decreases with the droplet size and increases with the oxygen content in the ambient gas. The thickness of the flame sheet (the alumina particle layer) is analyzed using Abel inversion of the projected profile of the flame incandescence and optical depth, revealing a thickness of about 50 μm for a burning droplet of a 550 μm diameter. Based on the shadowgraph images, the evaporation rate of the Al droplets is determined from the shrinking rate of the droplet projected area. Size-dependent evaporation rates are found to be related to different slip velocities, and the addition of oxygen to the oxidizer can significantly increase the evaporation rate. Finally, a conceptual model of a burning Al droplet in the steady combustion stage is proposed based on the experimental findings. The presented results provide novel datasets that contribute to model development and deepen the understanding of the physical and chemical processes involved in aluminum droplet combustion.
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在热蒸汽主导流中燃烧的单个铝液滴的火焰结构
在这项工作中,我们采用了专门设计的实验装置来研究单个铝液滴在以热蒸汽为主的气流中的点火和燃烧。通过使用两台高倍率高速摄像机同时观察火焰炽焰和液滴阴影图,对不同尺寸铝液滴的瞬态燃烧行为进行了表征。燃烧过程可分为三个阶段:Al 点火和液滴生成、液滴蒸发和火焰发展以及稳定燃烧。在稳定燃烧阶段,以纳米级氧化铝液滴窄层为特征的明亮火焰片包裹着氧化铝液滴核心。由氧化铝液滴组成的火焰片位于一个相对于液滴核心的径向速度接近于零的停滞面上。对峙比约为 2,随着液滴大小的增大而略有减小,并随着环境气体中氧气含量的增加而增大。利用阿贝尔反演火焰炽热度和光学深度的投影轮廓,分析了火焰薄片(氧化铝颗粒层)的厚度,结果显示直径为 550 μm 的燃烧液滴的厚度约为 50 μm。根据阴影图图像,可通过液滴投影面积的收缩率确定铝液滴的蒸发率。研究发现,与尺寸相关的蒸发率与不同的滑移速度有关,在氧化剂中加入氧气可显著提高蒸发率。最后,根据实验结果提出了一个处于稳定燃烧阶段的燃烧铝液滴的概念模型。所展示的结果提供了新的数据集,有助于模型的开发,并加深了对铝液滴燃烧所涉及的物理和化学过程的理解。
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来源期刊
Combustion and Flame
Combustion and Flame 工程技术-工程:化工
CiteScore
9.50
自引率
20.50%
发文量
631
审稿时长
3.8 months
期刊介绍: The mission of the journal is to publish high quality work from experimental, theoretical, and computational investigations on the fundamentals of combustion phenomena and closely allied matters. While submissions in all pertinent areas are welcomed, past and recent focus of the journal has been on: Development and validation of reaction kinetics, reduction of reaction mechanisms and modeling of combustion systems, including: Conventional, alternative and surrogate fuels; Pollutants; Particulate and aerosol formation and abatement; Heterogeneous processes. Experimental, theoretical, and computational studies of laminar and turbulent combustion phenomena, including: Premixed and non-premixed flames; Ignition and extinction phenomena; Flame propagation; Flame structure; Instabilities and swirl; Flame spread; Multi-phase reactants. Advances in diagnostic and computational methods in combustion, including: Measurement and simulation of scalar and vector properties; Novel techniques; State-of-the art applications. Fundamental investigations of combustion technologies and systems, including: Internal combustion engines; Gas turbines; Small- and large-scale stationary combustion and power generation; Catalytic combustion; Combustion synthesis; Combustion under extreme conditions; New concepts.
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