Pub Date : 2024-07-01DOI: 10.1016/j.combustflame.2024.113589
Shixiang Liu , Michael A. Delichatsios , Longhua Hu
Non-vertical turbulent non-premixed jet flame occur in combustion systems and by accidental release of fuels caused fires. Understanding the combustion dynamics of these asymmetric diffusion jet flames is needed to characterize the flame morphology and entrainment, which is a foundation for further detailed analysis of the physics and implications. This paper investigates experimentally and theoretically the flame morphological characteristics of non-vertical turbulent jets at both positive- and negative inclined angles in a systematic way. A total of 168 experimental cases were considered involving various initial fuel flow rates, inclined angles and nozzle diameters. Dimensional analysis was performed taking into account the controlling parameters of the physical mechanisms, namely the momentum flux, the fuel mass flow rate, the flame buoyancy, the stoichiometric ratio and the jet initial inclined angle, which together determine a characteristic length scale and a characteristic volumetric flow rate. These two characteristic parameters provide successful non-dimensional correlations for the location of the flame tip. A new integral model was also developed physically considering the momentum and continuity equations along the trajectory to predict the flame tip, as well as the lowest point for negative inclined jets. By comparing the experimental correlations with numerical prediction, the effective air entrainment coefficients were derived for different jet initial inclined angles, which showed little change with inclined angle from positive to negative, but the constant relating the average values to the integrals of the (Gaussian) radial profiles decreased as the initial angle decreased from positive to negative. This change is related to the variation of the profile properties normal to the trajectory as well as to mass detrainment laterally escaping from the jet flame especially for negative inclined angles. Finally, the local Richardson number and the flame lowest point for negative inclined angles was numerically predicted and compared well with the experimental results.
{"title":"Morphological characteristics of non-vertical turbulent jet flames: Experimental investigation and analytical model","authors":"Shixiang Liu , Michael A. Delichatsios , Longhua Hu","doi":"10.1016/j.combustflame.2024.113589","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113589","url":null,"abstract":"<div><p>Non-vertical turbulent non-premixed jet flame occur in combustion systems and by accidental release of fuels caused fires. Understanding the combustion dynamics of these asymmetric diffusion jet flames is needed to characterize the flame morphology and entrainment, which is a foundation for further detailed analysis of the physics and implications. This paper investigates experimentally and theoretically the flame morphological characteristics of non-vertical turbulent jets at both positive- and negative inclined angles in a systematic way. A total of 168 experimental cases were considered involving various initial fuel flow rates, inclined angles and nozzle diameters. Dimensional analysis was performed taking into account the controlling parameters of the physical mechanisms, namely the momentum flux, the fuel mass flow rate, the flame buoyancy, the stoichiometric ratio and the jet initial inclined angle, which together determine a characteristic length scale and a characteristic volumetric flow rate. These two characteristic parameters provide successful non-dimensional correlations for the location of the flame tip. A new integral model was also developed physically considering the momentum and continuity equations along the trajectory to predict the flame tip, as well as the lowest point for negative inclined jets. By comparing the experimental correlations with numerical prediction, the effective air entrainment coefficients were derived for different jet initial inclined angles, which showed little change with inclined angle from positive to negative, but the constant relating the average values to the integrals of the (Gaussian) radial profiles decreased as the initial angle decreased from positive to negative. This change is related to the variation of the profile properties normal to the trajectory as well as to mass detrainment laterally escaping from the jet flame especially for negative inclined angles. Finally, the local Richardson number and the flame lowest point for negative inclined angles was numerically predicted and compared well with the experimental results.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-07-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485988","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-28DOI: 10.1016/j.combustflame.2024.113592
Dohyung Park, Jaehyun Park, Kyu Tae Kim
Knowledge of the underlying physical mechanisms responsible for the triggering of high-frequency transverse combustion dynamics is of fundamental importance in the development of heavy-duty gas turbine combustors, aircraft engine afterburners, and bipropellant liquid rocket engines. Detailed information about three-dimensional thermoacoustic interactions and local flame dynamics, however, remains largely unknown and unanticipated, mainly because high-amplitude transverse mode instabilities are challenging to excite and detect in well-controlled sub-scale laboratory environments. To overcome this impasse, here we exploit a spatially tailored rectangular injector assembly consisting of ten equidistant horizontal slit nozzles to eliminate the complications of out-of-plane flame dynamics characterization. A total of 56 datasets of self-induced instabilities were acquired over a wide range of operating conditions to understand spatiotemporal phase dynamics and important mode shapes, in conjunction with 2D Rayleigh angle reconstruction and phase-resolved OH PLIF-based local flame front identification. Experimentally, we show that high-frequency transverse instabilities are excited only under high temperature and high thermal power conditions, manifested as non-evanescent pressure fluctuations at 6.50 kHz strongly coupled to the second-order tangential mode of the rectangular combustion chamber. Two vertically-oriented pressure nodal planes and the characteristic phase transition perpendicular to the horizontal slit injector direction are accurately measured and reconfirmed by Helmholtz simulations in terms of their interpositions and spatial orientation. Remarkably, the periodic formation of co-propagating coherent structures and concomitant local flame displacement/pinch-off are revealed to play an important role in driving the high-frequency hydrogen combustion dynamics.
{"title":"High-frequency hydrogen combustion dynamics driven by local flame displacement and multidimensional thermoacoustic interactions","authors":"Dohyung Park, Jaehyun Park, Kyu Tae Kim","doi":"10.1016/j.combustflame.2024.113592","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113592","url":null,"abstract":"<div><p>Knowledge of the underlying physical mechanisms responsible for the triggering of high-frequency transverse combustion dynamics is of fundamental importance in the development of heavy-duty gas turbine combustors, aircraft engine afterburners, and bipropellant liquid rocket engines. Detailed information about three-dimensional thermoacoustic interactions and local flame dynamics, however, remains largely unknown and unanticipated, mainly because high-amplitude transverse mode instabilities are challenging to excite and detect in well-controlled sub-scale laboratory environments. To overcome this impasse, here we exploit a spatially tailored rectangular injector assembly consisting of ten equidistant horizontal slit nozzles to eliminate the complications of out-of-plane flame dynamics characterization. A total of 56 datasets of self-induced instabilities were acquired over a wide range of operating conditions to understand spatiotemporal phase dynamics and important mode shapes, in conjunction with 2D Rayleigh angle reconstruction and phase-resolved OH PLIF-based local flame front identification. Experimentally, we show that high-frequency transverse instabilities are excited only under high temperature and high thermal power conditions, manifested as non-evanescent pressure fluctuations at 6.50 kHz strongly coupled to the second-order tangential mode of the rectangular combustion chamber. Two vertically-oriented pressure nodal planes and the characteristic phase transition perpendicular to the horizontal slit injector direction are accurately measured and reconfirmed by Helmholtz simulations in terms of their interpositions and spatial orientation. Remarkably, the periodic formation of co-propagating coherent structures and concomitant local flame displacement/pinch-off are revealed to play an important role in driving the high-frequency hydrogen combustion dynamics.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485991","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-28DOI: 10.1016/j.combustflame.2024.113575
Yue Wang , Yan Gong , Hantao Lu , Qinghua Guo , Guangsuo Yu
The thermal behaviors of high-temperature particle (HTP) and low-temperature particle (LTP) are investigated based on the bench-scale impinging entrained-flow coal-water slurry (CWS) gasification experimental platform with a modified visualization system. The size and velocity distribution of both particles, and the evolution of HTP are analyzed through the algorithmic and precise processing of the image sequences. In addition, in-situ temperature diagnosis of the particles during the reaction process were realized. The typical evolution process and the temperature of HTP in char oxidation stage are obtained. The results show that the concentration of HTP in the gasifier is greater than LTP, but the particle size is relatively small. Particles moving at the low speed (0–2 m/s) account for the largest proportion of both HTP and LTP. The char oxidation process lasts over 300 ms and can be divided into three reaction stages. During the reaction, the peak temperature at the center of the particle can reach more than 2000 K. The average temperature of the particles gradually increased, reaching a peak in reaction stage II (1500 K) followed by a gradual decrease. The particle temperature is affected by O/C and is prone to experience swelling and bubbling phenomena during char oxidation.
{"title":"Thermal behaviors of coal particles in an impinging entrained-flow gasifier: Char oxidation","authors":"Yue Wang , Yan Gong , Hantao Lu , Qinghua Guo , Guangsuo Yu","doi":"10.1016/j.combustflame.2024.113575","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113575","url":null,"abstract":"<div><p>The thermal behaviors of high-temperature particle (HTP) and low-temperature particle (LTP) are investigated based on the bench-scale impinging entrained-flow coal-water slurry (CWS) gasification experimental platform with a modified visualization system. The size and velocity distribution of both particles, and the evolution of HTP are analyzed through the algorithmic and precise processing of the image sequences. In addition, in-situ temperature diagnosis of the particles during the reaction process were realized. The typical evolution process and the temperature of HTP in char oxidation stage are obtained. The results show that the concentration of HTP in the gasifier is greater than LTP, but the particle size is relatively small. Particles moving at the low speed (0–2 m/s) account for the largest proportion of both HTP and LTP. The char oxidation process lasts over 300 ms and can be divided into three reaction stages. During the reaction, the peak temperature at the center of the particle can reach more than 2000 K. The average temperature of the particles gradually increased, reaching a peak in reaction stage II (1500 K) followed by a gradual decrease. The particle temperature is affected by O/C and is prone to experience swelling and bubbling phenomena during char oxidation.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485990","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-28DOI: 10.1016/j.combustflame.2024.113565
Zhihao Ding, Karine Truffin, Stéphane Jay
In this work, the phenomenon of cycle-to-cycle variability (CCV) of combustion in a spark ignition engine is investigated to give a deeper understanding of CCV generation. The main objective is to localize within the cylinder and all along the engine cycle the flow variabilites and identify some driving mechanisms originating in the flow structures and leading to combustion variabilites. In Part I , the application of empirical mode decomposition methods combined with topology-based techniques to the LES flow results allowed the extraction of the large-scale flow motion from the small-scale turbulence and the follow-up of their evolution during compression stroke [1]. A link was then established between the combustion process and the tumble formation and destabilization near BDC. In the present paper, the overall tumble motion development during compression and intake strokes is quantitatively analyzed, and links are built between different engine phases to establish the cause-and-effect chain. Other CCV factors, such as spray injection and exhaust gas recirculation, were not included in the current study. However, the developed methodology for in-cylinder flow analysis could be used in studies on other engine configurations to improve the development of engine designs.
Novelty and significance statement
In this work, the cycle-to-cycle variability (CCV) of combustion in a spark ignition engine is investigated to give a deeper understanding of CCV generation. The present study focuses on CCV caused by the stochastic nature of internal turbulent flow structures. LES approach is chosen due to its ability to capture CCV, and advanced flow analysis tools are developed and applied to LES results to characterize instantaneous flow structures of different scales in the three-dimensional domain and separately quantify their impacts on combustion.
A first important finding is that flow-wall interactions near BDC determine the tumble evolution.
A second novelty is the characterization of several 3D dominant flow interactions during intake yielding large-scale flow variability.
A third novelty and important finding is that links are found between the flow organization during intake, the tumble development, and destabilization during early compression and the combustion. Throughout our analyses starting from the spark timing and going back to the early intake phase, a cause-and-effect chain is finally established between the development of in-cylinder flow and the combustion variability.
在这项工作中,对火花点火发动机中燃烧的周期变异(CCV)现象进行了研究,以深入了解 CCV 的产生。主要目的是定位气缸内和发动机整个循环过程中的流动变异,并确定一些源于流动结构并导致燃烧变异的驱动机制。在第一部分中,将经验模式分解方法与基于拓扑的技术相结合应用于 LES 流动结果,可以从小规模湍流中提取大规模流动运动,并跟踪其在压缩冲程中的演变[1]。随后,在燃烧过程与 BDC 附近的翻滚形成和失稳之间建立了联系。本文定量分析了压缩冲程和进气冲程中的整体翻滚运动发展,并在发动机不同阶段之间建立联系,以建立因果关系链。本研究不包括其他 CCV 因素,如喷射和废气再循环。然而,所开发的气缸内流动分析方法可用于其他发动机配置的研究,以改进发动机设计的开发。本研究的重点是由内部湍流结构的随机性引起的 CCV。由于 LES 能够捕捉 CCV,因此选择了 LES 方法,并开发了先进的流动分析工具,将其应用于 LES 结果,以表征三维域中不同尺度的瞬时流动结构,并分别量化其对燃烧的影响。第三个新颖而重要的发现是,我们发现进气过程中的流动组织、翻滚发展以及早期压缩和燃烧过程中的不稳定之间存在联系。我们的分析从火花定时开始,一直追溯到进气早期阶段,最终在缸内流动的发展和燃烧变化之间建立了因果关系链。
{"title":"Cause-and-effect chain analysis of combustion cyclic variability in a spark-ignition engine using large-eddy simulation, Part II: Origins of flow variations from intake","authors":"Zhihao Ding, Karine Truffin, Stéphane Jay","doi":"10.1016/j.combustflame.2024.113565","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113565","url":null,"abstract":"<div><p>In this work, the phenomenon of cycle-to-cycle variability (CCV) of combustion in a spark ignition engine is investigated to give a deeper understanding of CCV generation. The main objective is to localize within the cylinder and all along the engine cycle the flow variabilites and identify some driving mechanisms originating in the flow structures and leading to combustion variabilites. In Part I , the application of empirical mode decomposition methods combined with topology-based techniques to the LES flow results allowed the extraction of the large-scale flow motion from the small-scale turbulence and the follow-up of their evolution during compression stroke <span>[1]</span>. A link was then established between the combustion process and the tumble formation and destabilization near BDC. In the present paper, the overall tumble motion development during compression and intake strokes is quantitatively analyzed, and links are built between different engine phases to establish the cause-and-effect chain. Other CCV factors, such as spray injection and exhaust gas recirculation, were not included in the current study. However, the developed methodology for in-cylinder flow analysis could be used in studies on other engine configurations to improve the development of engine designs.</p><p><strong>Novelty and significance statement</strong></p><p>In this work, the cycle-to-cycle variability (CCV) of combustion in a spark ignition engine is investigated to give a deeper understanding of CCV generation. The present study focuses on CCV caused by the stochastic nature of internal turbulent flow structures. LES approach is chosen due to its ability to capture CCV, and advanced flow analysis tools are developed and applied to LES results to characterize instantaneous flow structures of different scales in the three-dimensional domain and separately quantify their impacts on combustion.</p><p>A first important finding is that flow-wall interactions near BDC determine the tumble evolution.</p><p>A second novelty is the characterization of several 3D dominant flow interactions during intake yielding large-scale flow variability.</p><p>A third novelty and important finding is that links are found between the flow organization during intake, the tumble development, and destabilization during early compression and the combustion. Throughout our analyses starting from the spark timing and going back to the early intake phase, a cause-and-effect chain is finally established between the development of in-cylinder flow and the combustion variability.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485989","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-27DOI: 10.1016/j.combustflame.2024.113573
Amanda Matson , Leonid Kagan , Claude-Michel Brauner , Gregory Sivashinsky , Peter V. Gordon
In this paper we consider a classical model of gasless combustion in a one dimensional formulation under the assumption of ignition temperature kinetics. We study the propagation of flame fronts in this model when the initial distribution of the solid fuel is a spatially periodic function that varies on a large scale. It is shown that in certain parametric regimes the model supports periodic traveling fronts. An accurate asymptotic formula for the velocity of the flame front is derived and studied. The stability of periodic fronts is also explored, and a critical condition in terms of parameters of the problem is derived. It is also shown that the instability of periodic fronts, in certain parametric regimes, results in a propagation-extinction-conduction-reignition pattern which is studied numerically.
Novelty and significance statement: This work provides a closed form asymptotic description of periodic traveling fronts in a gasless combustion model with step-wise ignition temperature kinetics with a slowly varying concentration field. The stability analysis is performed, and the range of applicability of asymptotic formulas is given. A new propagation-extinction-conduction-reignition regime is identified. This regime emerges exclusively due to periodicity of the concentration field.
{"title":"On dynamics of gasless combustion in slowly varying periodic media","authors":"Amanda Matson , Leonid Kagan , Claude-Michel Brauner , Gregory Sivashinsky , Peter V. Gordon","doi":"10.1016/j.combustflame.2024.113573","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113573","url":null,"abstract":"<div><p>In this paper we consider a classical model of gasless combustion in a one dimensional formulation under the assumption of ignition temperature kinetics. We study the propagation of flame fronts in this model when the initial distribution of the solid fuel is a spatially periodic function that varies on a large scale. It is shown that in certain parametric regimes the model supports periodic traveling fronts. An accurate asymptotic formula for the velocity of the flame front is derived and studied. The stability of periodic fronts is also explored, and a critical condition in terms of parameters of the problem is derived. It is also shown that the instability of periodic fronts, in certain parametric regimes, results in a propagation-extinction-conduction-reignition pattern which is studied numerically.</p><p>Novelty and significance statement: This work provides a closed form asymptotic description of periodic traveling fronts in a gasless combustion model with step-wise ignition temperature kinetics with a slowly varying concentration field. The stability analysis is performed, and the range of applicability of asymptotic formulas is given. A new propagation-extinction-conduction-reignition regime is identified. This regime emerges exclusively due to periodicity of the concentration field.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-27","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0010218024002827/pdfft?md5=7a20bd668ecfd7d4839b9a3431289541&pid=1-s2.0-S0010218024002827-main.pdf","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485987","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"OA","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-26DOI: 10.1016/j.combustflame.2024.113591
Hao Liu , Shu Zheng , Xinyi Chen , Tipeng Wang , Ran Sui , Qiang Lu
Due to the characteristics of heat absorption and decomposition, endothermic hydrocarbon fuels (EHFs) have been widely used in scramjets for thermal protection and heat recirculation. The understanding of ignition characteristics of EHFs is of great importance for their safe and efficient utilization. In this paper, the ignition processes of EHFs were numerically simulated at atmospheric pressure and with an initial temperature of 500 K. Three different ignition stages were identified based on the chemical heat release and flame kernel propagation. A 3-component kerosene surrogate model composed of n-dodecane, methyl cyclohexane and m-xylene was adopted, as well as the corresponding chemical kinetic model with 369 species and 2691 reactions. Results showed that the discrepant decomposition characteristics of n-alkanes and cycloalkanes affected the chemical heat release and propagation during the ignition process. Two-stage exothermic characteristic was observed in the time evolutions of chemical heat release rate and fuel decomposition. The mass production of molecules and accumulation of radicals dominated the first and second exothermic peaks, respectively. Furthermore, the minimum ignition energies (MIEs) of EHFs with various methyl cyclohexane were determined to quantify the effect of fuel composition on ignition performance. Characteristically, the MIE dramatically decreased from 10.2 to 2.15 mJ when 20% n-dodecane was replaced by methyl cyclohexane. However, it was slightly increased as methyl cyclohexane continued to increase. Analyses from both physical and chemical aspects were conducted to elaborate the dependence of MIE on fuel composition. The dominant effects of flame-dynamic and chemical effects on different ignition stages were analysed. The faster propagation speed and stronger endothermic ability of methyl cyclohexane led to the nonlinear variation of MIEs. The results in this study provide useful guidance for composition optimization and safety evaluation of EHFs.
{"title":"Roles of fuel composition on the ignition process of endothermic hydrocarbons","authors":"Hao Liu , Shu Zheng , Xinyi Chen , Tipeng Wang , Ran Sui , Qiang Lu","doi":"10.1016/j.combustflame.2024.113591","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113591","url":null,"abstract":"<div><p>Due to the characteristics of heat absorption and decomposition, endothermic hydrocarbon fuels (EHFs) have been widely used in scramjets for thermal protection and heat recirculation. The understanding of ignition characteristics of EHFs is of great importance for their safe and efficient utilization. In this paper, the ignition processes of EHFs were numerically simulated at atmospheric pressure and with an initial temperature of 500 K. Three different ignition stages were identified based on the chemical heat release and flame kernel propagation. A 3-component kerosene surrogate model composed of <em>n</em>-dodecane, methyl cyclohexane and <em>m</em>-xylene was adopted, as well as the corresponding chemical kinetic model with 369 species and 2691 reactions. Results showed that the discrepant decomposition characteristics of <em>n</em>-alkanes and cycloalkanes affected the chemical heat release and propagation during the ignition process. Two-stage exothermic characteristic was observed in the time evolutions of chemical heat release rate and fuel decomposition. The mass production of molecules and accumulation of radicals dominated the first and second exothermic peaks, respectively. Furthermore, the minimum ignition energies (MIEs) of EHFs with various methyl cyclohexane were determined to quantify the effect of fuel composition on ignition performance. Characteristically, the MIE dramatically decreased from 10.2 to 2.15 mJ when 20% <em>n</em>-dodecane was replaced by methyl cyclohexane. However, it was slightly increased as methyl cyclohexane continued to increase. Analyses from both physical and chemical aspects were conducted to elaborate the dependence of MIE on fuel composition. The dominant effects of flame-dynamic and chemical effects on different ignition stages were analysed. The faster propagation speed and stronger endothermic ability of methyl cyclohexane led to the nonlinear variation of MIEs. The results in this study provide useful guidance for composition optimization and safety evaluation of EHFs.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485993","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
An improved consistent soot model is proposed and applied to evaluate the effect of 2-butanone addition (10 % to 50 % on a volume basis represented as case 1 to case 5) to ethylene fuel on soot formation using a counterflow burner configuration. The predictive capability of the suggested soot model is verified by assessing its performance against existing experimental data on soot formation (SF) configuration-type ethylene counterflow flames at diverse strain rates and various fuel additives. The proposed soot model comprises 55 inception reactions with temperature-dependent collision efficiency and 10 condensation reactions from 10 PAH species (from naphthalene to larger PAHs up to coronene), including modified HACA surface growth and oxidation reactions. 2-butanone is produced as a byproduct during the pyrolysis of biomass and the microbiological fermentation of agricultural waste. It holds various benefits as a prospective biofuel for spark ignition (SI) engines. Limited information exists regarding its sooting characteristics due to a lack of available soot measurements. The simulations are conducted for the soot formation (SF) type counterflow flames with a fixed fuel and oxidizer jet velocity. The proposed soot model can effectively replicate both the qualitative and quantitative aspects of the experimental trends and shows a better agreement than the existing models available in the literature. The soot volume fraction (SVF) and the particle number density (PND) decrease with increasing the 2-butanone concentration in the binary fuel mixture. The PAH concentration decreases with increasing 2-butanone addition in the fuel mixture. The peak SVF and the maximum temperature are reduced by ∼22.7 % and ∼3.6 %, with a 40 % increase in the 2-butanone portion in the fuel mixture from case 1 to case 5. Increasing the 2-butanone content in the fuel mixture decreases the inception rate, HACA rate, and condensation rate while it increases the oxidation rate.
{"title":"Effect of 2-butanone addition to ethylene fuel on soot formation in counterflow diffusion flames using newly proposed soot model","authors":"Subrat Garnayak, Hrishikesh Gadgil, Sudarshan Kumar","doi":"10.1016/j.combustflame.2024.113572","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113572","url":null,"abstract":"<div><p>An improved consistent soot model is proposed and applied to evaluate the effect of 2-butanone addition (10 % to 50 % on a volume basis represented as case 1 to case 5) to ethylene fuel on soot formation using a counterflow burner configuration. The predictive capability of the suggested soot model is verified by assessing its performance against existing experimental data on soot formation (SF) configuration-type ethylene counterflow flames at diverse strain rates and various fuel additives. The proposed soot model comprises 55 inception reactions with temperature-dependent collision efficiency and 10 condensation reactions from 10 PAH species (from naphthalene to larger PAHs up to coronene), including modified HACA surface growth and oxidation reactions. 2-butanone is produced as a byproduct during the pyrolysis of biomass and the microbiological fermentation of agricultural waste. It holds various benefits as a prospective biofuel for spark ignition (SI) engines. Limited information exists regarding its sooting characteristics due to a lack of available soot measurements. The simulations are conducted for the soot formation (SF) type counterflow flames with a fixed fuel and oxidizer jet velocity. The proposed soot model can effectively replicate both the qualitative and quantitative aspects of the experimental trends and shows a better agreement than the existing models available in the literature. The soot volume fraction (SVF) and the particle number density (PND) decrease with increasing the 2-butanone concentration in the binary fuel mixture. The PAH concentration decreases with increasing 2-butanone addition in the fuel mixture. The peak SVF and the maximum temperature are reduced by ∼22.7 % and ∼3.6 %, with a 40 % increase in the 2-butanone portion in the fuel mixture from case 1 to case 5. Increasing the 2-butanone content in the fuel mixture decreases the inception rate, HACA rate, and condensation rate while it increases the oxidation rate.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485977","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-24DOI: 10.1016/j.combustflame.2024.113566
Zhihao Ding , Karine Truffin, Stéphane Jay
Understanding, modeling, and reducing the cycle-to-cycle variability (CCV) of combustion in internal combustion engines (ICE) is a critical challenge to design engines of high efficiency and low emissions. A high level of CCV may contribute to partial burn, misfire, and knock in extreme engine cycles, which affects engine performance and eventually damages the engine. The origins of CCV have been studied both experimentally and numerically, and the variability of in-cylinder aerodynamics is recognized as one of the most important sources of CCV. However, a detailed and quantitative explanation of how in-cylinder flow CCV is generated is not yet clear. The objective of the present study is to develop a methodology to localize inside the chamber of a spark-ignition engine (SIE) the origins of flow variabilities and to identify some driving mechanisms leading to combustion variabilities. Multi-cycle wall-modeled large-eddy simulations (LES) for the TU Darmstadt optical engine under fired conditions are performed using the CFD solver Converge 3.0. The evolution of organized large-scale structures and the small-scale turbulence of the in-cylinder flow are analyzed using a developed methodology that includes the empirical mode decomposition (EMD) method adapted for 2D and 3D flow fields, and a vortex identification tool . The contributions of different parts of the flow to CCV are quantified. In Part I of this work, the LES framework is validated against experimental data, and CCV of large-scale structures is characterized at spark timing. In Part II, the overall flow development during compression and intake strokes are quantitatively analyzed, and links are built between different engine phases to establish the cause-and-effect chain. Other CCV factors, such as spray injection and exhaust gas recirculation, are not included in the current study. However, the developed methodology for in-cylinder flow analysis could be used in studies on other engine configurations to improve the development of engine designs.
Novelty and significance statement
In this work, the cycle-to-cycle variability (CCV) of combustion in a spark ignition engine is investigated to give a deeper understanding of CCV generation. The present study focuses on CCV caused by the stochastic nature of internal turbulent flow structures. LES approach is chosen due to its ability to capture CCV. The LES methodology was validated in a motored case in Ding et al. (2023). In the present study, it is validated in a reactive case against experimental in-cylinder pressures and velocity fields.
A first novelty is the application of EMD methods combined with topology-based techniques to reactive LES results to characterize flow structures of different scales in the three-dimensional domain and to quantify separately their impacts on combustion.
{"title":"Cause-and-effect chain analysis of combustion cyclic variability in a spark-ignition engine using large-eddy simulation, Part I: From tumble compression to flame initiation","authors":"Zhihao Ding , Karine Truffin, Stéphane Jay","doi":"10.1016/j.combustflame.2024.113566","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113566","url":null,"abstract":"<div><p>Understanding, modeling, and reducing the cycle-to-cycle variability (CCV) of combustion in internal combustion engines (ICE) is a critical challenge to design engines of high efficiency and low emissions. A high level of CCV may contribute to partial burn, misfire, and knock in extreme engine cycles, which affects engine performance and eventually damages the engine. The origins of CCV have been studied both experimentally and numerically, and the variability of in-cylinder aerodynamics is recognized as one of the most important sources of CCV. However, a detailed and quantitative explanation of how in-cylinder flow CCV is generated is not yet clear. The objective of the present study is to develop a methodology to localize inside the chamber of a spark-ignition engine (SIE) the origins of flow variabilities and to identify some driving mechanisms leading to combustion variabilities. Multi-cycle wall-modeled large-eddy simulations (LES) for the TU Darmstadt optical engine under fired conditions are performed using the CFD solver Converge 3.0. The evolution of organized large-scale structures and the small-scale turbulence of the in-cylinder flow are analyzed using a developed methodology that includes the empirical mode decomposition (EMD) method adapted for 2D and 3D flow fields, and a vortex identification tool <span><math><msub><mrow><mi>Γ</mi></mrow><mrow><mn>3</mn><mi>p</mi></mrow></msub></math></span>. The contributions of different parts of the flow to CCV are quantified. In Part I of this work, the LES framework is validated against experimental data, and CCV of large-scale structures is characterized at spark timing. In Part II, the overall flow development during compression and intake strokes are quantitatively analyzed, and links are built between different engine phases to establish the cause-and-effect chain. Other CCV factors, such as spray injection and exhaust gas recirculation, are not included in the current study. However, the developed methodology for in-cylinder flow analysis could be used in studies on other engine configurations to improve the development of engine designs.</p><p><strong>Novelty and significance statement</strong></p><p>In this work, the cycle-to-cycle variability (CCV) of combustion in a spark ignition engine is investigated to give a deeper understanding of CCV generation. The present study focuses on CCV caused by the stochastic nature of internal turbulent flow structures. LES approach is chosen due to its ability to capture CCV. The LES methodology was validated in a motored case in Ding et al. (2023). In the present study, it is validated in a reactive case against experimental in-cylinder pressures and velocity fields.</p><p>A first novelty is the application of EMD methods combined with topology-based techniques to reactive LES results to characterize flow structures of different scales in the three-dimensional domain and to quantify separately their impacts on combustion.</p><p>A second n","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485979","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
Pub Date : 2024-06-24DOI: 10.1016/j.combustflame.2024.113556
Hao Tang , Zeinab Al Hadi , Thibault F. Guiberti , Wenting Sun , Gaetano Magnotti
This study reports an experimental investigation of quantitative Nitric Oxide (NO) distribution in both premixed and non-premixed NH3/H2-air flames using a counterflow burner at atmospheric pressure. One-dimensional (1D) NO laser-induced fluorescence (LIF) spectroscopy and Raman/Rayleigh spectroscopy were conducted to accurately resolve the quantitative 1D NO profile in terms of mixture fraction, temperature, and physical space. We calibrated a saturated NO-LIF model in 5 premixed lean H2/N2/NO-air flames with different seeded NO levels in a McKenna burner and validated its accuracy in three H2N2NO-air counterflow diffusion flames. The overall uncertainty of NO quantification was less than90 ppm. Our measurements were compared with simulations using different ammonia chemical kinetic models, revealing that current models have over 30% uncertainty in predicting peak NO concentrations (mole fraction) in 1D non-premixed and premixed flames and over 100% uncertainty in lower temperature regions. In premixed flames, measured NO concentrations fell within the intermediate range of current chemical kinetic models at lean and stoichiometric conditions, but were lower than the models at rich conditions. In non-premixed flames, all models overestimated the peak NO concentrations by more than 1000 ppm. It is noted that the measured peak NO concentrations increased with higher NH3/H2 ratios (from 4/6 to 8/2), strain rates (from 80 to 140 1/s), and N2 dilution ratios in a 1:1 NH3/H2 mixture (from 0 to 30%). Although most models could qualitatively predict the trends, they were inaccurate in quantifying NO. Additionally, the measured width of the NO profile in mixture fraction space expanded with increasing NH3/H2 ratio, N2 dilution ratio, and strain rate. While models could qualitatively predict this behavior, they consistently underestimated NO in the fuel-rich, lower-temperature region, resulting in a narrower NO profile width. The Manna model showed a better prediction of NO distribution in the fuel rich portion of non-premixed flames, accounting for NH3NO interactions at lower temperatures. These findings highlight the critical need to improve models to accurately predict NO concentrations in ammonia-containing flames and their behavior in fuel rich regions.
本研究报告了在大气压力下使用逆流燃烧器对预混合和非预混合 NH3/H2- 空气火焰中一氧化氮(NO)定量分布的实验研究。我们采用了一维(1D)NO 激光诱导荧光(LIF)光谱和拉曼/雷利光谱,以准确解析一维 NO 在混合物组分、温度和物理空间方面的定量分布。我们在麦肯纳燃烧器中的 5 个具有不同 NO 种子水平的预混合贫 H2/N2/NO-air 火焰中校准了饱和 NO-LIF 模型,并在 3 个 H2N2NO-air 逆流扩散火焰中验证了其准确性。氮氧化物定量的总体不确定性小于 90 ppm。我们将测量结果与使用不同氨化学动力学模型的模拟结果进行了比较,结果表明,目前的模型在预测一维非预混合和预混合火焰中的 NO 浓度峰值(摩尔分数)时,不确定性超过 30%,而在较低温度区域,不确定性超过 100%。在预混火焰中,在贫气和化学计量条件下,测得的氮氧化物浓度在当前化学动力学模型的中间范围内,但在富气条件下低于模型。在非预混合火焰中,所有模型都高估了 NO 的峰值浓度,高出 1000 ppm 以上。值得注意的是,随着 NH3/H2 比率(从 4/6 到 8/2)、应变速率(从 80 到 140 1/s)和 1:1 NH3/H2 混合气中 N2 稀释比(从 0 到 30%)的提高,测得的 NO 峰值浓度也在增加。虽然大多数模型可以定性地预测趋势,但它们在量化 NO 方面并不准确。此外,随着 NH3/H2 比率、N2 稀释比率和应变速率的增加,在混合分数空间中测得的 NO 曲线宽度也在扩大。虽然模型可以定性地预测这种行为,但它们始终低估了富燃料、低温区域的 NO,导致 NO 剖面宽度变窄。Manna 模型能更好地预测非预混火焰中富含燃料部分的 NO 分布,并考虑到 NH3NO 在较低温度下的相互作用。这些发现突出表明,亟需改进模型,以准确预测含氨火焰中的 NO 浓度及其在富燃料区的行为。
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Pub Date : 2024-06-24DOI: 10.1016/j.combustflame.2024.113587
Gang Xiong, Dong Zeng, Yi Wang
To develop and validate numerical models for sooty fires, we have established a dataset of the thermal radiation and soot in 15 kW buoyant turbulent ethylene flames. The flames are stabilized on a water-cooled round burner with a 15.2 cm outer diameter (D) and 13.7 cm inner diameter at three oxygen concentrations (OC) of 15.2 %, 16.8 %, and 20.9 %. A two-color optical probe is used to measure the spectral radiative intensities at two wavelengths, from which soot volume fraction and temperature are determined. The overall mean soot volume fractions are consistent with results from laser induced incandescence and laser extinction measurements. For a given OC, the mean soot temperature and volume fraction conditioned on the radiative intensity greater than a threshold value (instrumental detection limit) are relatively independent of spatial location. When OC decreases from 20.9 % to 15.2 %, the conditional mean soot volume fraction decreases by a factor of two. However, the conditional mean soot temperature at different locations and OCs are within a narrow range (with a standard deviation of only 22 K). The effect of detection limit is discussed, and the results show that the correlation between soot volume fraction and temperature is weak with a sufficiently low detection limit. Based on the experimental findings, a simplified model for the turbulence-radiation interaction (TRI) is proposed for application in the numerical modeling of soot radiation. The model approximates the turbulent closure term for radiation by taking advantage of the fact that the soot temperature has a relatively unchanged mean value and a narrow quasi-normal distribution within the buoyant turbulent flame, regardless of the spatial location and oxygen concentration. Therefore, the soot emission power can be directly calculated from the mean soot volume fraction and conditional mean soot temperature in a decoupled manner.
{"title":"Thermal radiation and soot in buoyant turbulent diffusion flames under different oxygen concentrations: Measurements and implications to radiation modeling","authors":"Gang Xiong, Dong Zeng, Yi Wang","doi":"10.1016/j.combustflame.2024.113587","DOIUrl":"https://doi.org/10.1016/j.combustflame.2024.113587","url":null,"abstract":"<div><p>To develop and validate numerical models for sooty fires, we have established a dataset of the thermal radiation and soot in 15 kW buoyant turbulent ethylene flames. The flames are stabilized on a water-cooled round burner with a 15.2 cm outer diameter (D) and 13.7 cm inner diameter at three oxygen concentrations (OC) of 15.2 %, 16.8 %, and 20.9 %. A two-color optical probe is used to measure the spectral radiative intensities at two wavelengths, from which soot volume fraction and temperature are determined. The overall mean soot volume fractions are consistent with results from laser induced incandescence and laser extinction measurements. For a given OC, the mean soot temperature and volume fraction conditioned on the radiative intensity greater than a threshold value (instrumental detection limit) are relatively independent of spatial location. When OC decreases from 20.9 % to 15.2 %, the conditional mean soot volume fraction decreases by a factor of two. However, the conditional mean soot temperature at different locations and OCs are within a narrow range (with a standard deviation of only 22 K). The effect of detection limit is discussed, and the results show that the correlation between soot volume fraction and temperature is weak with a sufficiently low detection limit. Based on the experimental findings, a simplified model for the turbulence-radiation interaction (TRI) is proposed for application in the numerical modeling of soot radiation. The model approximates the turbulent closure term for radiation by taking advantage of the fact that the soot temperature has a relatively unchanged mean value and a narrow quasi-normal distribution within the buoyant turbulent flame, regardless of the spatial location and oxygen concentration. Therefore, the soot emission power can be directly calculated from the mean soot volume fraction and conditional mean soot temperature in a decoupled manner.</p></div>","PeriodicalId":280,"journal":{"name":"Combustion and Flame","volume":null,"pages":null},"PeriodicalIF":5.8,"publicationDate":"2024-06-24","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"141485992","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}