Assessing the impact of oil and gas activities on ambient hydrocarbon concentrations in North Texas: A retrospective analysis from 2000 to 2022

IF 4.2 2区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Atmospheric Environment Pub Date : 2024-10-31 DOI:10.1016/j.atmosenv.2024.120907
Jithin Kanayankottupoyil, Kuruvilla John
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Abstract

Over the past two decades, significant advancements in shale gas extraction technologies have led to a vast increase in oil and gas production in the Barnett Shale region of North Texas. This study provides a detailed analysis of the trends in air pollutants, such as total nonmethane hydrocarbons (NMHC), linked to oil and gas production changes in the Barnett shale region from 2000 to 2022. The analysis spans urban (Dallas - DAL), semi-urban (Fort Worth - FWNW), and non-urban (Denton - DEN) ambient air quality monitoring sites operated by the Texas Commission on Environmental Quality (TCEQ), highlighting how varying levels of urbanization and industrial activities influence air quality. DEN recorded the highest NMHC concentrations at an average of 210.27 ppb-C, significantly exceeding those at FWNW (83.14 ppb-C) and DAL (62.50 ppb-C). Alkanes were the predominant NMHCs across all sites, forming 96% at DEN, 89% at FWNW, and 67% at DAL. The i/n-pentane ratio at DEN suggests oil and gas activities as the main NMHC source, whereas DAL, and FWNW indicate substantial influences from urban traffic alongside industrial emissions. NMHC concentrations at DEN and FWNW correlated strongly with gas and condensate production, demonstrating a shift from condensate to gas over the study period.

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评估石油和天然气活动对北德克萨斯州环境碳氢化合物浓度的影响:2000 年至 2022 年的回顾性分析
在过去的二十年里,页岩气开采技术的巨大进步使得北德克萨斯州巴尼特页岩地区的石油和天然气产量大幅增加。本研究详细分析了 2000 年至 2022 年巴尼特页岩地区与石油和天然气生产变化相关的空气污染物(如非甲烷总烃 (NMHC))的变化趋势。该分析跨越了得克萨斯州环境质量委员会 (TCEQ) 管理的城市(达拉斯 - DAL)、半城市(沃斯堡 - FWNW)和非城市(丹顿 - DEN)环境空气质量监测点,突出了不同程度的城市化和工业活动对空气质量的影响。DEN 记录的 NMHC 浓度最高,平均为 210.27 ppb-C,大大超过 FWNW(83.14 ppb-C)和 DAL(62.50 ppb-C)。烷烃是所有地点的主要 NMHC,在 DEN 占 96%,在 FWNW 占 89%,在 DAL 占 67%。DEN 的 i/n-pentane 比率表明石油和天然气活动是 NMHC 的主要来源,而 DAL 和 FWNW 则表明城市交通和工业排放对 NMHC 有很大影响。DEN 和 FWNW 的 NMHC 浓度与天然气和凝析油的产量密切相关,表明在研究期间,凝析油已转向天然气。
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来源期刊
Atmospheric Environment
Atmospheric Environment 环境科学-环境科学
CiteScore
9.40
自引率
8.00%
发文量
458
审稿时长
53 days
期刊介绍: Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review. Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.
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