{"title":"Cross-sections for formation of 73Ga through natGe(n, x)73Ga reaction induced by d-T neutrons","authors":"Junhua Luo , Long He , Liang Zhou , Li Jiang","doi":"10.1016/j.radphyschem.2024.112384","DOIUrl":null,"url":null,"abstract":"<div><div>The formation of <sup>73</sup>Ga through <sup>nat</sup>Ge(n,<em>x</em>)<sup>73</sup>Ga reaction induced by d-T neutrons was investigated using cross-sections measured by four characteristic gamma-rays employing the weighted average method. The neutron energy and uncertainty were determined by the Q equation of reaction <sup>3</sup>H(d,n)<sup>4</sup>He combined with the solid angle of the sample. The gamma spectrum of the activated sample was obtained by an off-line technique using a high-resolution, high-purity germanium detector (HPGe). The contribution of nuclear reactions <sup>76</sup>Ge(n,α)<sup>73</sup>Zn, <sup>73</sup>Ge(n,p)<sup>73</sup>Ga, and <sup>74</sup>Ge(n,d∗)<sup>73</sup>Ga to residual nuclei <sup>73</sup>Ga was analyzed and the cross-sections of reaction <sup>73</sup>Ge(n,p)<sup>73</sup>Ga were determined with a small uncertainty. The TALYS-1.96 package was utilized for performing the theoretical calculation of the cross section of <sup>76</sup>Ge(n,α)<sup>73</sup>Zn, <sup>73</sup>Ge(n,p)<sup>73</sup>Ga, and <sup>74</sup>Ge(n,d∗)<sup>73</sup>Ga reactions. The results of the theoretical calculation of nuclear reaction <sup>73</sup>Ge(n,p)<sup>73</sup>Ga were compared with the experimental measurements and the evaluation results provided by the database.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"227 ","pages":"Article 112384"},"PeriodicalIF":2.8000,"publicationDate":"2024-11-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969806X24008764","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
The formation of 73Ga through natGe(n,x)73Ga reaction induced by d-T neutrons was investigated using cross-sections measured by four characteristic gamma-rays employing the weighted average method. The neutron energy and uncertainty were determined by the Q equation of reaction 3H(d,n)4He combined with the solid angle of the sample. The gamma spectrum of the activated sample was obtained by an off-line technique using a high-resolution, high-purity germanium detector (HPGe). The contribution of nuclear reactions 76Ge(n,α)73Zn, 73Ge(n,p)73Ga, and 74Ge(n,d∗)73Ga to residual nuclei 73Ga was analyzed and the cross-sections of reaction 73Ge(n,p)73Ga were determined with a small uncertainty. The TALYS-1.96 package was utilized for performing the theoretical calculation of the cross section of 76Ge(n,α)73Zn, 73Ge(n,p)73Ga, and 74Ge(n,d∗)73Ga reactions. The results of the theoretical calculation of nuclear reaction 73Ge(n,p)73Ga were compared with the experimental measurements and the evaluation results provided by the database.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.