Satellite-Based Identification of Large Anthropogenic NMVOC Emission Sources

IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Journal of Geophysical Research: Atmospheres Pub Date : 2024-11-16 DOI:10.1029/2024JD042047
B. Franco, L. Clarisse, M. Van Damme, J. Hadji-Lazaro, C. Clerbaux, P. Coheur
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Abstract

Nonmethane volatile organic compounds (NMVOCs) emitted in excess from anthropogenic sources significantly contribute to the formation of harmful pollutants, thereby degrading air quality. While satellite measurements have become valuable tools for tracking anthropogenic emitters, they have primarily targeted inorganic species and methane ( CH 4 ${\text{CH}}_{4}$ ). This study demonstrates the potential of infrared atmospheric sounding interferometers (IASI) to detect anthropogenic NMVOC point sources on a global scale. Using an advanced oversampling technique, we enhance the spatial resolution of IASI measurements to identify emitters of three major NMVOCs: methanol ( CH 3 ${\text{CH}}_{3}$ OH), acetylene ( C 2 H 2 ${\mathrm{C}}_{2}{\mathrm{H}}_{2}$ ), and propylene ( C 3 H 6 ${\mathrm{C}}_{3}{\mathrm{H}}_{6}$ ). These point sources are primarily associated with chemical and petrochemical facilities, coal-burning activities, metallurgy, pharmaceutical manufacturing sites, and megacities. We also highlight the value of combining IASI measurements of NMVOCs with those of the inorganic species, such as sulfur dioxide ( SO 2 ${\text{SO}}_{2}$ ) and ammonia ( NH 3 ${\text{NH}}_{3}$ ), to aid in the identification of anthropogenic point sources.

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基于卫星的大型人为 NMVOC 排放源识别
人为排放源过量排放的非甲烷挥发性有机化合物(NMVOCs)极大地促成了有害污染物的形成,从而降低了空气质量。虽然卫星测量已成为追踪人为排放物的重要工具,但它们主要针对的是无机物和甲烷(CH 4 ${text\{CH}}_{4}$ )。这项研究证明了红外大气探测干涉仪(IASI)在全球范围内探测人为非甲烷挥发性有机化合物点源的潜力。利用先进的超采样技术,我们提高了 IASI 测量的空间分辨率,从而确定了三种主要非甲烷挥发性有机化合物的排放源:甲醇(CH 3 ${\text{CH}}_{3}$ OH)、乙炔(C 2 H 2 ${\mathrm{C}}_{2}\mathrm{H}}_{2}$ )和丙烯(C 3 H 6 ${\mathrm{C}}_{3}\mathrm{H}}_{6}$ )。这些点源主要与化工和石化设施、燃煤活动、冶金、制药厂和特大城市有关。我们还强调了将非甲烷总挥发性有机化合物的 IASI 测量值与二氧化硫 ( SO 2 ${\text{SO}}_{2}$ ) 和氨 ( NH 3 ${\text{NH}}_{3}$ ) 等无机物的 IASI 测量值相结合,以帮助识别人为点源的价值。
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来源期刊
Journal of Geophysical Research: Atmospheres
Journal of Geophysical Research: Atmospheres Earth and Planetary Sciences-Geophysics
CiteScore
7.30
自引率
11.40%
发文量
684
期刊介绍: JGR: Atmospheres publishes articles that advance and improve understanding of atmospheric properties and processes, including the interaction of the atmosphere with other components of the Earth system.
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