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Analysis of the Influence of Clear-Sky Fluxes on the Cloud-Type Mean Cloud Radiative Effects in the Tropical Convectively Active Regions With CERES Satellite Data 利用 CERES 卫星数据分析晴空通量对热带对流活跃区云型平均云辐射效应的影响
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-20 DOI: 10.1029/2024JD041525
Kuan-Man Xu, Moguo Sun, Yaping Zhou

Cloud radiative effects (CREs) and cloud-type mean CREs depend upon how clear-sky fluxes are computed over a large area: those of the immediate environment of clouds or the regional mean clear-sky fluxes. Five convectively active regions in the Tropics, two over land (Africa and Amazon) and three over ocean (eastern and western Pacific and Atlantic), are selected to understand the influence of immediate environment of clouds on CREs. Fluxes derived from 19 years of high-resolution CERES satellite data, categorized by cloud type, are utilized. The cloud types are classified based on the joint cloud top pressure and cloud optical depth distribution. For the entire tropical region, differences in cloud-type mean CRE with regional mean and immediate environment clear skies range from −7.8 to 10.7 Wm−2 for shortwave (SW), 2.9 to 15.8 Wm−2 for longwave (LW), and 6.1 to 17.9 Wm−2 for net, respectively. The oceanic and Amazonia regions have negative (positive) SW (LW) CRE differences, typically 2–6 Wm−2 in SW but 7–10 Wm−2 in LW, whereas Africa has positive SW and LW CRE differences (typically 20–30 Wm−2, up to 40–50 Wm−2). The influence of immediate environment reduces the regionally averaged, that is, cloud-type mean CREs weighted by cloud fractions, SW cloud cooling, and LW cloud warming in four of the five regions except for Africa. For Africa, it increases the SW cloud cooling and greatly reduces the LW cloud warming, resulting in net cloud cooling as in other regions instead of warming. The implications of these findings for observational and modeling studies are discussed.

云辐射效应(CRE)和云类型平均 CRE 取决于如何计算大面积的晴空通量:云的直接环境通量或区域平均晴空通量。为了了解云的直接环境对 CREs 的影响,我们选择了热带地区对流活跃的五个区域,其中两个在陆地上(非洲和亚马逊),三个在海洋上(东、西太平洋和大西洋)。通量来自 19 年的高分辨率 CERES 卫星数据,按云类型分类。云类型是根据云顶气压和云光学深度的联合分布来划分的。在整个热带地区,云类型平均 CRE 与区域平均值和直接环境晴天的差异分别为:短波(SW)-7.8 至 10.7 Wm-2,长波(LW)2.9 至 15.8 Wm-2,净空 6.1 至 17.9 Wm-2。大洋和亚马孙地区的西南(长波)CRE 差异为负(正),通常西南为 2-6 Wm-2,长波为 7-10 Wm-2,而非洲的西南和长波 CRE 差异为正(通常为 20-30 Wm-2,最高可达 40-50 Wm-2)。受直接环境影响,除非洲外,五个地区中有四个地区的区域平均 CRE(即按云分数加权的云类型平均 CRE)、西南云降温和左岸云升温都有所降低。就非洲而言,它增加了西南云的降温,大大减少了左岸云的升温,导致与其他地区一样出现净云降温而非升温。讨论了这些发现对观测和建模研究的影响。
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引用次数: 0
A Simple Model for the Evaporation of Hydrometeors and Their Isotopes 水介质及其同位素蒸发的简单模型
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-20 DOI: 10.1029/2024JD041126
Simon P. de Szoeke, Mampi Sarkar, Estefanía Quiñones Meléndez, Peter N. Blossey, David Noone

Cloud condensation and hydrometeor evaporation fractionate stable isotopes of water, enriching liquid with heavy isotopes; whereupon updrafts, downdrafts, and rain vertically redistribute water and its isotopes in the lower troposphere. These vertical water fluxes through the marine boundary layer affect low cloud climate feedback and, combined with isotope fractionation, are hypothesized to explain the depletion of tropical precipitation at higher precipitation rates known as the “amount effect.” Here, an efficient and numerically stable quasi-analytical model simulates the evaporation of raindrops and enrichment of their isotope composition. It is applied to a drop size distribution and subcloud environment representative of Atlantic trade cumulus clouds. Idealized physics experiments artificially zero out selected processes to discern the separate effects on the isotope ratio of raindrops, of exchange with the environment, evaporation, and kinetic molecular diffusion. A parameterization of size-dependent molecular and eddy diffusion is formulated that enriches raindrops much more strongly (+5‰ for deuterated water [HDO] and +3.5‰ for H218 ${mathrm{H}}_{2}^{18}$O) than equilibrium evaporation as they become smaller than 1 mm. The effect on evaporated vapor is also assessed. Rain evaporation enriches subcloud vapor by +12‰ per mm rain (for HDO), explaining observations of enriched vapor in cold pools sourced by evaporatively cooled downdrafts. Drops smaller than 0.5 mm evaporate completely before falling 700 m in typical subtropical marine boundary layer conditions. The early and complete evaporation of these smaller drops in the rain size distribution enriches the vapor produced by rain evaporation.

云凝结和水流星蒸发会分馏出稳定的水同位素,使液体富含重同位素;随后上升气流、下降气流和降雨会在对流层低层垂直重新分配水及其同位素。这些通过海洋边界层的垂直水通量影响低云气候反馈,并与同位素分馏相结合,被假定为可以解释在较高降水率下热带降水的耗竭,即所谓的 "量效应"。在这里,一个高效且数值稳定的准分析模型模拟了雨滴的蒸发及其同位素组成的富集。该模型适用于代表大西洋贸易积云的雨滴大小分布和云下环境。理想化物理实验人为地将选定的过程归零,以辨别与环境交换、蒸发和分子动力学扩散对雨滴同位素比率的不同影响。制定了一个尺寸依赖性分子扩散和涡流扩散的参数化,当雨滴变得小于 1 毫米时,它比平衡蒸发富集得更强(氘化水 [HDO] 富集 +5‰,H 2 18 ${mathrm{H}}_{2}^{18}$ O 富集 +3.5‰)。还评估了对蒸发水汽的影响。雨水蒸发使云下水汽富集,每毫米雨水富集+12‰(HDO),这解释了在由蒸发冷却的下沉气流形成的冷池中观测到的富集水汽。在典型的亚热带海洋边界层条件下,小于 0.5 毫米的雨滴在下降 700 米之前就完全蒸发了。在雨滴大小分布中,这些较小雨滴的提前和完全蒸发,丰富了雨滴蒸发产生的水汽。
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引用次数: 0
Modeling the Effects of Vegetation and Snow on Dust Storm Over the Gobi Desert 模拟植被和积雪对戈壁滩沙尘暴的影响
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-19 DOI: 10.1029/2024JD041407
Yueting Hao, Zilin Wang, Lian Xue, Sijia Lou, Ke Ding, Yue Qin, Xin Huang

The Gobi Desert is a prominent dust source in Asia, where the dust storm is severe and features great interannual and seasonal variability. Previous studies have found land surface variation plausibly plays an important role in the occurrence and intensity of dust storms. However, the quantitative estimation and numerical description in current models are still limited. Here, a comprehensive study utilizing multiple observations and modeling methods to assess the influence of vegetation and snow on dust was conducted. We found that Gobi deserts exhibit substantial monthly and interannual variability in dust storms, which shows a close connection with vegetation and snow. To quantitatively understand the impact of vegetation and snow cover on dust emissions and also to better characterize such effects in numerical models, we introduced a high-resolution dynamic dust source function that incorporates the effects of vegetation and snow on erodibility. The new parameterization noticeably improved dust-related simulations, including aerosol optical thickness and PM10 concentrations, and provided insights into the distinct effects of vegetation and snow on dust emissions. This study sheds light on the effects of vegetation and snow on dust storms over the Gobi Desert, highlighting the importance of dynamic representation of time-varying surface properties in dust simulation.

戈壁滩是亚洲的一个主要沙尘源,那里的沙尘暴十分严重,而且年际和季节变化很大。以往的研究发现,地表变化可能在沙尘暴的发生和强度中扮演了重要角色。然而,目前模型中的定量估计和数值描述仍然有限。在此,我们利用多种观测和建模方法进行了一项综合研究,以评估植被和积雪对沙尘的影响。我们发现,戈壁沙漠的沙尘暴呈现出很大的月变率和年际变率,这表明沙尘暴与植被和积雪密切相关。为了定量了解植被和积雪对沙尘排放的影响,同时也为了在数值模式中更好地描述这种影响,我们引入了一个高分辨率动态沙尘源函数,其中包含了植被和积雪对可侵蚀性的影响。新的参数化明显改善了与沙尘有关的模拟,包括气溶胶光学厚度和 PM10 浓度,并为植被和积雪对沙尘排放的不同影响提供了见解。这项研究揭示了植被和积雪对戈壁滩沙尘暴的影响,强调了在沙尘模拟中动态表示时变表面特性的重要性。
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引用次数: 0
Environmental Controls on Deep and Overshooting Convection Over the Contiguous U.S. 美国毗连地区深对流和过对流的环境控制因素
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-18 DOI: 10.1029/2024JD041841
Kenneth P. Bowman, Anita D. Rapp

During the summer season, deep convection over the central United States has a significant impact on the dynamics and composition of the upper troposphere and lower stratosphere (UTLS). These storms transport tropospheric air containing trace gases, ice particles, and aerosols into the UTLS, which can affect chemical and radiative processes over a large region. Because overshooting storms necessarily have strong updrafts, there is a marked correlation between overshooting and the occurrence of severe weather at the surface. Heat released by these storms also helps to drive the North American Monsoon Anticyclone (NAMA) in the UTLS, which partially confines air injected into the stratosphere by overshooting storms. In support of the Dynamics and Chemistry of the Summer Stratosphere (DCOTSS) project, this study is a climatological analysis of the environmental factors that affect the occurrence of deep and overshooting storms. Using hourly analyses of overshooting storms based on GridRad radar data and ERA5 reanalyzes, we focus on the roles of convective available potential energy (CAPE), convective inhibition (CIN), jet location, and other relevant dynamical and thermodynamic variables. The results show that northward intrusion of airmasses containing moist high CAPE air from the Gulf of Mexico into the central plains plays a major role in producing the conditions necessary for overshooting storms with other factors playing secondary roles.

在夏季,美国中部上空的深层对流对对流层上部和平流层下部(UTLS)的动力学和组成有重大影响。这些风暴将对流层中含有痕量气体、冰颗粒和气溶胶的空气输送到 UTLS,从而影响到大片区域的化学和辐射过程。由于凌空风暴必然具有强大的上升气流,因此凌空风暴与地表恶劣天气的发生有明显的相关性。这些风暴释放的热量还有助于推动UTLS中的北美季风反气旋(NAMA),该反气旋部分限制了过冲风暴注入平流层的空气。为支持夏季平流层动力学和化学(DCOTSS)项目,本研究对影响深层和超调风暴发生的环境因素进行了气候学分析。利用基于 GridRad 雷达数据和ERA5 再分析的过冲风暴小时分析,我们重点研究了对流可用势能(CAPE)、对流抑制(CIN)、喷流位置以及其他相关动力学和热力学变量的作用。结果表明,含有高对流势能的湿润空气团从墨西哥湾向北侵入中部平原,在产生超调风暴所需的条件方面发挥了主要作用,而其他因素则起次要作用。
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引用次数: 0
Origins of Extreme CAPE Around the World 世界各地极端 CAPE 的起源
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-18 DOI: 10.1029/2024JD041833
P. J. Tuckman, Kerry Emanuel

Severe convection, responsible for hazards such as tornadoes, flash floods, and hail, is usually preceded by abundant convective available potential energy (CAPE). In this work, we use a Lagrangian approach to study the buildup of anomalously large values of CAPE from 2012 to 2013 in various regions. Nearly all extreme values of CAPE arise from surface fluxes underneath a layer of convective inhibition (the CIN layer) over several diurnal cycles, but the origin of the CIN layer and the diurnal cycle of surface fluxes differ around the world. In some regions, such as North America and Europe, the air above the boundary layer must be much warmer than usual to form this CIN layer, whereas in other regions, especially the Middle East and central Africa, a CIN layer is common. Additionally, high CAPE occurrences that are over land (those in the Americas, Europe, Africa, and Southeast Asia) tend to lose their CIN layers before the time of maximum CAPE due to large diurnal cycles of sensible heating, whereas those that occur over coastal waters (in the Middle East, Northern Australia, South Asia, and the Mediterranean) usually retain substantial convective inhibition. Uniquely, CAPE in Southeast Australia often builds up due to cooling aloft rather than to boundary layer warming. These results show that one hoping to understand or predict CAPE patterns must understand a variety of mechanisms acting in different regions.

造成龙卷风、山洪暴发和冰雹等灾害的强对流,通常是由丰富的对流可用势能(CAPE)引起的。在这项工作中,我们使用拉格朗日方法研究了 2012 年至 2013 年期间不同地区异常大的 CAPE 值的积累情况。几乎所有的 CAPE 极端值都来自对流抑制层(CIN 层)下几个日周期的地表通量,但 CIN 层的起源和地表通量的日周期在世界各地有所不同。在某些地区,如北美和欧洲,边界层上方的空气必须比平时暖得多,才能形成 CIN 层,而在其他地区,特别是中东和非洲中部,CIN 层很常见。此外,在陆地上空出现的高 CAPE(美洲、欧洲、非洲和东南亚的高 CAPE),往往在 CAPE 最大值出现之前,就会由于较大的昼夜显热周期而失去 CIN 层,而在沿岸水域上空出现的高 CAPE(中东、澳大利亚北部、南亚和地中海的高 CAPE),通常会保留大量的对流抑制。与众不同的是,澳大利亚东南部的 CAPE 通常是由于高空冷却而不是边界层增温造成的。这些结果表明,希望了解或预测 CAPE 模式的人必须了解作用于不同地区的各种机制。
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引用次数: 0
A More Transparent Infrared Window 更透明的红外窗口
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-18 DOI: 10.1029/2024JD041366
Eli J. Mlawer, Jeana Mascio, David D. Turner, Vivienne H. Payne, Connor J. Flynn, Robert Pincus

The infrared window region (780–1,250 cm−1, 12.8 to 8.0 μm) is of great importance to Earth's climate due to its high transparency and thermal energy. We present here a new investigation of the transparency of this spectral region based on observations by interferometers of downwelling surface radiance at two DOE Atmospheric Radiation Measurement program sites. We focus on the dominant source of absorption in this region, the water vapor continuum, and derive updated values of spectral absorption coefficients for both the self and foreign continua. Our results show that the self continuum is too strong in the previous version of Mlawer-Tobin_Clough-Kneizys-Davies (MT_CKD) water vapor continuum model, a result that is consistent with other recent analyses, while the foreign continuum is too weak in MT_CKD. In general, the weaker self continuum derived in this study results in an overall increase in atmospheric transparency in the window, although in atmospheres with low amounts of water vapor the transparency may slightly decrease due to the increase in foreign continuum absorption. These continuum changes lead to a significant decrease in downwelling longwave flux at the surface for moist atmospheres and a modest increase in outgoing longwave radiation. The increased fraction of surface-leaving radiation that escapes to space leads to a notable increase (∼5–10%) in climate feedback, implying that climate simulations that use the new infrared window continuum will show somewhat less warming than before. This study also points out the possibly important role that aerosol absorption may play in the longwave radiative budget.

红外窗口区域(780-1250 cm-1,12.8-8.0 μm)因其高透明度和高热能而对地球气候非常重要。我们在此介绍根据干涉仪在两个能源部大气辐射测量计划站点对下沉表面辐射率的观测结果,对该光谱区域的透明度进行的一项新研究。我们重点研究了这一区域的主要吸收源--水汽连续波,并得出了自连续波和外来连续波的光谱吸收系数的最新值。我们的结果表明,在先前版本的 Mlawer-Tobin_Clough-Kneizys-Davies (MT_CKD)水汽连续面模型中,自连续面太强,这一结果与最近的其他分析一致,而在 MT_CKD 中,外来连续面太弱。一般来说,本研究得出的较弱的自连续相会导致窗口中大气透明度的整体增加,不过在水汽含量较低的大气中,由于外来连续相吸收的增加,透明度可能会略有下降。这些连续波变化导致潮湿大气表面的下沉长波通量显著减少,而外向长波辐射则略有增加。由于离开地表的辐射逃逸到太空的部分增加,导致气候反馈显著增加(∼5-10%),这意味着使用新的红外窗口连续体的气候模拟将比以前显示出更少的变暖。这项研究还指出了气溶胶吸收可能在长波辐射预算中扮演的重要角色。
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引用次数: 0
On the Multiscale Processes Leading to an Extreme Gust Wind Event in East China: Insights From Radar Wind Profiler Mesonet Observations 中国东部极端阵风事件的多尺度过程:雷达风廓线中间网观测的启示
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-16 DOI: 10.1029/2024JD041484
Tianmeng Chen, Jianping Guo, Xiaoran Guo, Yang Zhang, Hui Xu, Da-Lin Zhang

In this study, a record-breaking surface gust wind event of over 45 m s−1, which occurred in the coastal region of East China during the early evening hours of 30 April 2021, is examined. The dynamical characteristics of this event is explored by using a high-resolution mesonet comprised of eight radar wind profilers (RWPs), surface observations, radar and satellite data. Observational analyses show the development of several cloud clusters ahead of the axis of a midlevel trough with pronounced baroclinicity, and the subsequent organization into a comma-shaped squall system with a leading convective line over land and a trailing stratiform region moved offshore. The latter is embedded by a mesovortex with intense northerly rear inflows descending to the surface, accounting for the generation of the gusty winds. Results indicate the different roles of multi-scale processes in accelerating the surface winds to extreme intensity. Specifically, the large-scale baroclinic trough provides intense background rear inflows that are enhanced by the formation of the mesovortex, while moist downdrafts in the rear inflows account for the downward transport of horizontal momentum, leading to the generation of intense cold outflows and gusty winds close to the leading convective line. Despite the lack of sufficient observations for quantitative analysis, this study provides a qualitative analysis that offers valuable insights into the dynamics of extreme gusty winds. Moreover, the above results underscore the value of RWP mesonet observations in enhancing our understanding of extreme wind events and in improving the nowcasting and prediction efforts in the future.

本研究考察了 2021 年 4 月 30 日傍晚发生在华东沿海地区的一次超过 45 m s-1 的破纪录地面阵风事件。通过使用由八个雷达风廓线仪(RWPs)组成的高分辨率中间网、地面观测、雷达和卫星数据,探讨了该事件的动力学特征。观测分析表明,在具有明显条带倾向的中层槽轴线前方出现了几个云团,随后组织成一个逗号状的斜风系统,其前方的对流线位于陆地上空,后方的层状区域移至近海。后者由一个中涡嵌入,中涡后部有强烈的偏北气流下沉到地表,这就是阵风产生的原因。结果表明,多尺度过程在加速地表风达到极端强度方面发挥了不同的作用。具体来说,大尺度的巴氏槽提供了强烈的背景后部流入气流,中涡的形成增强了后部流入气流的强度,而后部流入气流中的潮湿下沉气流造成了水平动量的向下输送,导致在对流前线附近产生强烈的冷外流和阵风。尽管缺乏足够的观测数据进行定量分析,但本研究提供的定性分析为了解极端阵风的动态提供了宝贵的见解。此外,上述结果还强调了 RWP 介电观测在加强我们对极端大风事件的了解和改进未来的预报和预测工作方面的价值。
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引用次数: 0
Vapor Pressure Deficit Controls the Extent of Burned Area Over the Himalayas 水汽压力不足控制着喜马拉雅山上空的燃烧区域范围
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-16 DOI: 10.1029/2024JD041155
Leena Khadke, Subimal Ghosh

Globally, increasing occurrences of forest fires are major threats to the ecosystem. The rich forests in the Himalayas also suffer from high incidents of forest fires in the pre-monsoon summer months, March to June. Research studies are limited in identifying the meteorological factors governing the spatiotemporal distribution of forest fires. Using three satellite-based data sets of monthly burned area (BA) for March to June, we found higher BA in the Eastern Himalayas (EH) compared to the Central (CH) and Western Himalayas (WH). Using statistical methods, we found Vapor Pressure Deficit (VPD) to be the most dominating variable controlling BA in the Himalayas. Precipitation, soil moisture and temperature, with their relative variability, control VPD that governs the interannual and intraseasonal variations of BA. Our results imply that a good forecast of VPD will facilitate alert generation for the Himalayan forest fires.

在全球范围内,森林火灾的日益频繁是对生态系统的主要威胁。喜马拉雅山脉丰富的森林在夏季季风前的 3 月至 6 月也是森林火灾的高发期。在确定影响森林火灾时空分布的气象因素方面,研究十分有限。利用三组基于卫星的 3 月至 6 月月度烧毁面积(BA)数据,我们发现东喜马拉雅山(EH)的烧毁面积高于中喜马拉雅山(CH)和西喜马拉雅山(WH)。通过统计方法,我们发现水汽压差(VPD)是控制喜马拉雅山 BA 的最主要变量。降水、土壤水分和温度及其相对变化控制着 VPD,而 VPD 则控制着 BA 的年际和季节内变化。我们的研究结果表明,对 VPD 的良好预测将有助于喜马拉雅山森林火灾警报的生成。
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引用次数: 0
Satellite-Based Identification of Large Anthropogenic NMVOC Emission Sources 基于卫星的大型人为 NMVOC 排放源识别
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-16 DOI: 10.1029/2024JD042047
B. Franco, L. Clarisse, M. Van Damme, J. Hadji-Lazaro, C. Clerbaux, P. Coheur
<p>Nonmethane volatile organic compounds (NMVOCs) emitted in excess from anthropogenic sources significantly contribute to the formation of harmful pollutants, thereby degrading air quality. While satellite measurements have become valuable tools for tracking anthropogenic emitters, they have primarily targeted inorganic species and methane (<span></span><math> <semantics> <mrow> <msub> <mtext>CH</mtext> <mn>4</mn> </msub> </mrow> <annotation> ${text{CH}}_{4}$</annotation> </semantics></math>). This study demonstrates the potential of infrared atmospheric sounding interferometers (IASI) to detect anthropogenic NMVOC point sources on a global scale. Using an advanced oversampling technique, we enhance the spatial resolution of IASI measurements to identify emitters of three major NMVOCs: methanol (<span></span><math> <semantics> <mrow> <msub> <mtext>CH</mtext> <mn>3</mn> </msub> </mrow> <annotation> ${text{CH}}_{3}$</annotation> </semantics></math>OH), acetylene (<span></span><math> <semantics> <mrow> <msub> <mi>C</mi> <mn>2</mn> </msub> <msub> <mi>H</mi> <mn>2</mn> </msub> </mrow> <annotation> ${mathrm{C}}_{2}{mathrm{H}}_{2}$</annotation> </semantics></math>), and propylene (<span></span><math> <semantics> <mrow> <msub> <mi>C</mi> <mn>3</mn> </msub> <msub> <mi>H</mi> <mn>6</mn> </msub> </mrow> <annotation> ${mathrm{C}}_{3}{mathrm{H}}_{6}$</annotation> </semantics></math>). These point sources are primarily associated with chemical and petrochemical facilities, coal-burning activities, metallurgy, pharmaceutical manufacturing sites, and megacities. We also highlight the value of combining IASI measurements of NMVOCs with those of the inorganic species, such as sulfur dioxide (<span></span><math> <semantics> <mrow> <msub> <mtext>SO</mtext> <mn>2</mn> </msub> </mrow> <annotation> ${text{SO}}_{2}$</annotation> </semantics></math>) and ammonia (<span></span><math> <semantics> <mrow>
人为排放源过量排放的非甲烷挥发性有机化合物(NMVOCs)极大地促成了有害污染物的形成,从而降低了空气质量。虽然卫星测量已成为追踪人为排放物的重要工具,但它们主要针对的是无机物和甲烷(CH 4 ${text{CH}}_{4}$ )。这项研究证明了红外大气探测干涉仪(IASI)在全球范围内探测人为非甲烷挥发性有机化合物点源的潜力。利用先进的超采样技术,我们提高了 IASI 测量的空间分辨率,从而确定了三种主要非甲烷挥发性有机化合物的排放源:甲醇(CH 3 ${text{CH}}_{3}$ OH)、乙炔(C 2 H 2 ${mathrm{C}}_{2}mathrm{H}}_{2}$ )和丙烯(C 3 H 6 ${mathrm{C}}_{3}mathrm{H}}_{6}$ )。这些点源主要与化工和石化设施、燃煤活动、冶金、制药厂和特大城市有关。我们还强调了将非甲烷总挥发性有机化合物的 IASI 测量值与二氧化硫 ( SO 2 ${text{SO}}_{2}$ ) 和氨 ( NH 3 ${text{NH}}_{3}$ ) 等无机物的 IASI 测量值相结合,以帮助识别人为点源的价值。
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引用次数: 0
The Impact of Temperature on the Adiabaticity and Coverage of a Single Shallow Cumulus Cloud 温度对单层浅积云绝热性和覆盖范围的影响
IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES Pub Date : 2024-11-16 DOI: 10.1029/2024JD041585
Kang-En Huang, Minghuai Wang, Daniel Rosenfeld, Yannian Zhu, Xiaoran Ouyang

The uncertainty of climate projection is significantly related to warm cloud feedback, which involves a complex interplay of various mechanisms. However, it is hard to unentangle temperature's impact on a single cloud with experiments, since the cloud dynamics always covary with environmental thermodynamical conditions. In this study, we investigate a simulated single shallow cumulus cloud's response to temperature using two perturbation methods, namely “uniform” and “buoyancy-fixed”, the latter of which keeps the buoyancy profile unchanged in temperature perturbation. High-resolution large eddy simulations show that uniform warming significantly increases cloud buoyancy, reducing cloud adiabaticity. If buoyancy is fixed, warming only reduces cloud area, leaving adiabatic fraction almost unchanged. Such a response can be explained by the Clausius-Clapeyron effect with an idealized 1D diffusion model, showing that warming increases the cloud-environment absolute humidity difference more than the increase in cloud liquid water content, resulting in a faster loss in both cloud coverage and total liquid water solely by lateral mixing. The responses of cloud coverage and total liquid water counteract, making adiabatic fraction insensitive to temperature change. Our work shows that the cloud adiabatic fraction's response to temperature is sensitive to the perturbed structure of the boundary layer, and the cloud coverage reduction by diffusion acts as a positive cloud feedback mechanism in addition to the adjustment processes of the boundary layer.

气候预测的不确定性与暖云反馈有很大关系,其中涉及各种机制的复杂相互作用。然而,由于云的动力学总是与环境热力学条件共同作用,因此很难通过实验来厘清温度对单一云的影响。在本研究中,我们使用两种扰动方法(即 "均匀 "和 "浮力固定",后者在温度扰动中保持浮力剖面不变)研究了模拟单个浅积云对温度的响应。高分辨率大涡模拟显示,均匀升温会显著增加云的浮力,降低云的绝热性。如果浮力固定不变,变暖只会减少云的面积,使绝热部分几乎保持不变。这种响应可以用理想化的一维扩散模型中的克劳修斯-克拉皮隆效应来解释,表明气候变暖增加的云-环境绝对湿度差比增加的云液态水含量更大,从而导致云覆盖率和总液态水仅通过横向混合而更快地减少。云覆盖率和总液态水的反应相互抵消,使得绝热分数对温度变化不敏感。我们的研究表明,云的绝热分数对温度的响应对边界层的扰动结构很敏感,除了边界层的调整过程外,扩散导致的云覆盖率降低也是一种正的云反馈机制。
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引用次数: 0
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Journal of Geophysical Research: Atmospheres
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