Tunable ultrabroadband hybrid terahertz emitter combining a spintronic and a GaSe source

IF 3.5 2区 物理与天体物理 Q2 PHYSICS, APPLIED Applied Physics Letters Pub Date : 2024-11-19 DOI:10.1063/5.0226564
Afnan Alostaz, Oliver Gueckstock, Junwei Tong, Jana Kredl, Chihun In, Markus Münzenberg, Claus M. Schneider, Tobias Kampfrath, Tom S. Seifert
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Abstract

Terahertz (THz) time-domain spectroscopy (TDS) is a sensitive approach to material characterization. It critically relies on a sufficiently large bandwidth, which is not straightforwardly available in typical THz-TDS systems that are often limited to below 3 THz. Here, we introduce a hybrid THz-source concept based on a spintronic THz emitter (STE) deposited onto a thin, free-standing GaSe nonlinear crystal. By tuning the magnetic state and the phase-matching parameters of the hybrid emitter, we generate an ultrabroadband spectrum covering the full range from 1 to 40 THz. We achieve significantly enhanced spectral amplitudes above 10 THz compared to the bare STE, resulting in ultrashort THz-pulse durations down to 32 fs. Finally, we demonstrate the straightforward tunability of the shape of the few-cycle pulse from symmetric to antisymmetric.
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结合自旋电子和 GaSe 源的可调超宽带混合太赫兹发射器
太赫兹(THz)时域光谱(TDS)是一种灵敏的材料表征方法。它主要依赖于足够大的带宽,而典型的太赫兹-TDS 系统通常将带宽限制在 3 太赫兹以下,无法直接获得足够大的带宽。在这里,我们介绍了一种混合太赫兹源概念,它基于沉积在独立的薄 GaSe 非线性晶体上的自旋电子太赫兹发射器 (STE)。通过调整混合发射器的磁性状态和相位匹配参数,我们产生了覆盖 1 至 40 太赫兹全范围的超宽带频谱。与裸 STE 相比,我们在 10 THz 以上实现了明显增强的光谱振幅,从而产生了低至 32 fs 的超短 THz 脉冲持续时间。最后,我们展示了从对称到非对称的几周期脉冲形状的直接可调性。
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来源期刊
Applied Physics Letters
Applied Physics Letters 物理-物理:应用
CiteScore
6.40
自引率
10.00%
发文量
1821
审稿时长
1.6 months
期刊介绍: Applied Physics Letters (APL) features concise, up-to-date reports on significant new findings in applied physics. Emphasizing rapid dissemination of key data and new physical insights, APL offers prompt publication of new experimental and theoretical papers reporting applications of physics phenomena to all branches of science, engineering, and modern technology. In addition to regular articles, the journal also publishes invited Fast Track, Perspectives, and in-depth Editorials which report on cutting-edge areas in applied physics. APL Perspectives are forward-looking invited letters which highlight recent developments or discoveries. Emphasis is placed on very recent developments, potentially disruptive technologies, open questions and possible solutions. They also include a mini-roadmap detailing where the community should direct efforts in order for the phenomena to be viable for application and the challenges associated with meeting that performance threshold. Perspectives are characterized by personal viewpoints and opinions of recognized experts in the field. Fast Track articles are invited original research articles that report results that are particularly novel and important or provide a significant advancement in an emerging field. Because of the urgency and scientific importance of the work, the peer review process is accelerated. If, during the review process, it becomes apparent that the paper does not meet the Fast Track criterion, it is returned to a normal track.
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