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Acoustically coupled MEMS transducer pairs with loss and gain 具有损耗和增益的声耦合MEMS传感器对
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-13 DOI: 10.1063/5.0311884
Samer Houri, Rachid Haouari, Bart P. Weekers, Veronique Rochus
This work investigates the dynamics and experimentally extracts the acoustic coupling between a pair of microelectromechanical ultrasound transducers (MUTs) that are immersed in water and acoustically coupled through the fluid medium. A series of these transducer pairs with varying diameters (and thus resonance frequency) and pitch separation (and thus coupling strength) are fabricated and measured. This work presented here models and quantifies the open-loop coupling between the MEMS transducer pairs and its dependence on pitch. Furthermore, a gain feedback loop is systematically applied to one of the device pair, the dynamics of the acoustically coupled gain-loss system is investigated, and the formation of an exceptional point or of an Hopf bifurcation is equally used to quantify the acoustic coupling coefficient. This work provides an exploration of the formation of exceptional points in acoustically coupled MEMS transducers as well as three experimental means to study acoustic coupling in MUT transducers: via open-loop dynamics, Hopf bifurcation, and the formation of an exceptional point.
本文研究了浸泡在水中的一对微机电超声换能器(MUTs)与流体介质之间的声学耦合,并通过实验提取了它们之间的动力学和声学耦合。制造并测量了一系列具有不同直径(从而谐振频率)和间距分离(从而耦合强度)的这些换能器对。本文对MEMS传感器对之间的开环耦合及其对螺距的依赖进行了建模和量化。此外,系统地将增益反馈环路应用于其中一个器件对,研究了声耦合增益损失系统的动力学,并同样使用异常点或Hopf分岔的形成来量化声耦合系数。这项工作提供了声学耦合MEMS换能器中异常点形成的探索,以及研究MUT换能器中声学耦合的三种实验手段:通过开环动力学,Hopf分岔和异常点的形成。
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引用次数: 0
Ultralow threshold polariton laser and vortex formation in an organic microcavity at room temperature 室温下有机微腔中超低阈值极化激子激光与涡旋的形成
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-13 DOI: 10.1063/5.0313470
Dongxue Wang, Jiaxiang Mu, Chenxi Yang, Yao Li, Xiaokun Zhai, Zuofang Feng, Qiang Ai, Chunzi Xing, Xinmiao Yang, Yilong Lei, Haitao Dai, Liefeng Feng, Tingge Gao
Exciton polaritons represent hybrid bosonic quasiparticles that emerge from the strong coupling between excitons and photons. Their distinctive properties provide a robust platform for investigating light–matter interactions. These properties facilitate spontaneous coherence and pronounced nonlinear optical phenomena, making them highly suitable for exploring thresholdless lasing, ultrafast optical switching, and quantum fluid dynamics. Organic semiconductors are especially advantageous for polaritonic applications, owing to their high exciton binding energies and superior processability. In this study, we report a microcavity incorporating DPAVBi plate-like single crystals in a distinct polymorphic phase, achieving a lasing threshold approximately 60 times lower than that of previously reported DPAVBi micro-belts. Furthermore, we demonstrate the emergence of exciton–polariton vortex modes within this organic microcavity at room temperature. Our findings establish a viable pathway for investigating low-power organic photonic lasers and demonstrate their potential utility in quantum information processing and next-generation organic optoelectronic devices.
激子极化子是由激子和光子之间的强耦合产生的杂化玻色子准粒子。它们独特的性质为研究光-物质相互作用提供了一个强大的平台。这些特性促进了自发相干性和明显的非线性光学现象,使它们非常适合用于探索无阈值激光,超快光开关和量子流体动力学。有机半导体由于其高激子结合能和优越的可加工性,在极化应用中尤其有利。在这项研究中,我们报道了一个包含具有明显多晶相的DPAVBi片状单晶的微腔,实现了比先前报道的DPAVBi微带低约60倍的激光阈值。此外,我们证明了在室温下该有机微腔内出现激子-极化子涡旋模式。我们的发现为研究低功率有机光子激光器建立了一条可行的途径,并展示了它们在量子信息处理和下一代有机光电器件中的潜在应用。
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引用次数: 0
Surface nanoprocessing with unfocused beams of high-energy femtosecond lasers: A tool to produce surface characteristics libraries 用未聚焦的高能飞秒激光进行表面纳米加工:一种产生表面特性库的工具
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-13 DOI: 10.1063/5.0306168
J. Bohus, Á. Mohácsi, A. P. Farkas, L. Égerházi, T. Szörényi
We demonstrate a single-shot method for probing ultrafast laser–matter interactions using unfocused multi-terawatt femtosecond beams. The intrinsic fluence inhomogeneity of the beams is exploited to accomplish parallel, spatially encoded experiments performed under strictly identical conditions across a wide energy range in a single step, enabling systematic mapping of energy-dependent surface responses without beam scanning. As proof of the technique, the large set of simultaneously collected data points below, at, and above the threshold inherently allows for a threshold evaluation approach, different from both the diameter/depth regression analysis and the statistical method. Using copper as a test system, we quantify the fluence dependence of reflectance and morphology and identify a multi-pulse optical threshold of 0.020 J/cm2, coinciding with the onset of ablation confirmed by SEM imaging. The minimum specular reflectance observed, around 0.10%, favorably compares to the respective figures reported. Applying this parallelized surface mapping technique with high-energy laser systems featuring suitably large beam diameters thereby provides a versatile platform for exploring ultrafast laser-induced surface responses, with potential applications in material design, surface engineering, and optical damage studies.
我们演示了使用无聚焦多太瓦飞秒光束探测超快激光-物质相互作用的单射方法。利用光束的内在影响不均匀性,在一个步骤中在严格相同的条件下在宽能量范围内完成平行的空间编码实验,从而在没有光束扫描的情况下系统地绘制能量依赖的表面响应。作为该技术的证明,同时收集的大量数据点低于、等于和高于阈值,本质上允许阈值评估方法,不同于直径/深度回归分析和统计方法。使用铜作为测试系统,我们量化了反射率和形貌的影响关系,并确定了0.020 J/cm2的多脉冲光阈值,与SEM成像证实的烧蚀开始一致。观测到的最小镜面反射率约为0.10%,与各自报告的数据相比有利。将这种并行表面映射技术应用于具有适当大光束直径的高能激光系统,从而为探索超快激光诱导的表面响应提供了一个多功能平台,在材料设计、表面工程和光学损伤研究中具有潜在的应用前景。
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引用次数: 0
Magnetic aftereffect and Barkhausen jumps in thin altermagnetic Mn5Si3 films Mn5Si3薄膜的磁后效应和巴克豪森跳变
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-12 DOI: 10.1063/5.0314005
Gregor Skobjin, Javier Rial, Sebastian Beckert, Helena Reichlova, Vincent Baltz, Lisa Michez, Richard Schlitz, Michaela Lammel, Sebastian T. B. Goennenwein
In ferromagnets, the anomalous Hall effect (AHE) can exhibit time-dependent relaxation, including magnetic aftereffect and Barkhausen jumps, and thus provide insights into magnetic susceptibility and domain dynamics. Recently, a finite AHE has also been reported in compensated collinear magnets—termed altermagnets—which, due to their spin and crystal symmetries, combine properties usually attributed to either ferromagnets or antiferromagnets. To date, a possible time-dependent relaxation of the AHE in altermagnets has not been explored. Here, we study the Hall effect response of micrometer-scale Hall bars patterned into thin films of Mn5Si3, an altermagnet featuring a finite spontaneous AHE. Recording transport data as a function of time, at a fixed magnetic field magnitude, we observe a relaxation of the Hall voltage qualitatively and quantitatively similar to the magnetic aftereffect in ferromagnetic films. In addition, the Hall voltage time traces feature clear unidirectional jumps, which we interpret as Barkhausen jumps, i.e., as experimental evidence for abrupt reorientations of Hall vector domains in Mn5Si3. A quantitative analysis yields a Barkhausen length of around 18 nm in the Hall bar devices with the smallest width of 100 nm.
在铁磁体中,反常霍尔效应(AHE)可以表现出随时间的弛豫,包括磁后效应和巴克豪森跳变,从而提供了对磁化率和畴动力学的见解。最近,在补偿共线磁体(称为交替磁体)中也报道了有限AHE,这种磁体由于其自旋和晶体对称性,结合了通常属于铁磁体或反铁磁体的性质。迄今为止,交替磁体中AHE的可能的随时间的弛豫尚未被探索。在这里,我们研究了微米尺度霍尔棒的霍尔效应响应,霍尔棒是一种具有有限自发AHE的交替磁体Mn5Si3薄膜。将输运数据作为时间的函数记录下来,在固定的磁场量级下,我们观察到霍尔电压的弛豫在定性和定量上类似于铁磁薄膜中的磁后效应。此外,霍尔电压时间轨迹具有明显的单向跳变,我们将其解释为巴克豪森跳变,即作为Mn5Si3中霍尔矢量畴突然重定向的实验证据。定量分析表明,霍尔棒器件的巴克豪森长度约为18 nm,最小宽度为100 nm。
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引用次数: 0
Dynamic terahertz focal planar scanning via cascaded metasurfaces 通过级联超表面的动态太赫兹焦平面扫描
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-12 DOI: 10.1063/5.0315215
Wenhui Xu, Guibin Li, Hui Li, Qi Tan, Yufei Liu, Jie Li, Hang Xu, Yan Zhang, Jianquan Yao
Terahertz (THz) planar focal spot scanning is critical for imaging, sensing, and optical routing, but traditional approaches suffer from bulkiness or limited tunability. Herein, we propose a cascaded metasurface device with two mechanically rotatable dielectric layers (M1 and M2) to achieve dynamic focal scanning. The core mechanism relies on rotation-induced phase superposition: tuning angles α1 and α2 modulates the combined phase distribution, enabling continuous in-plane focal displacement. Simulations demonstrate controllable scanning under M2 rotation (α1 = 0°, α2: −75° to 75°) and opposite co-rotation (α1 = −α2: −60° to 60°), with stable focal length and efficiency. Experimental characterization via a THz near-field system confirms close agreement between simulated and measured scanning trajectories, verifying the device's predictability and reliability. This passive scheme offers simplicity, large tuning range, and broadband compatibility, avoiding external energy supplies. The proposed cascaded platform enriches THz optical manipulation tools and facilitates integration into dynamic imaging, sensing, and beam steering systems.
太赫兹(THz)平面焦点点扫描对于成像、传感和光路由至关重要,但传统方法存在体积大或可调性有限的问题。在此,我们提出了一个级联的超表面器件,具有两个机械可旋转的介电层(M1和M2),以实现动态焦扫描。核心机制依赖于旋转诱导的相位叠加:α1和α2调谐角调节组合相位分布,实现连续的面内焦位移。仿真结果表明,在M2旋转(α1 = 0°,α2:−75°~ 75°)和反向共旋转(α1 =−α2:−60°~ 60°)条件下扫描可控,焦距稳定,扫描效率高。通过太赫兹近场系统进行的实验表征证实了模拟和测量的扫描轨迹之间的密切一致,验证了设备的可预测性和可靠性。这种无源方案提供简单、大调谐范围和宽带兼容性,避免了外部能源供应。所提出的级联平台丰富了太赫兹光学操作工具,便于集成到动态成像、传感和光束转向系统中。
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引用次数: 0
Electrical control of polarization-resolved photodetection in GeSe/MoTe2 heterostructures for optoelectronic encryption 用于光电加密的GeSe/MoTe2异质结构偏振分辨光探测的电气控制
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-12 DOI: 10.1063/5.0320086
Xiaoqi Zi, Shaoguang Zhao, Hang Deng, Qiman Zhang, Ziheng Zhao, Li Tao
Polarimetric optical encryption enables parallel information channels and enhanced eavesdropping prevention capabilities, improving data transmission capacity and information security. However, conventional systems rely heavily on bulky and discrete components such as polarizers and wave plates, which complicate device integration and miniaturization. To address these limitations, we demonstrate a polarization-resolved photodetector based on the heterostructure of GeSe/2H-MoTe2. Leveraging the type-II energy band arrangement and strong interface coupling between anisotropic GeSe and ambipolar 2H-MoTe2 layers, the device enables efficient carrier separation and broadband light response from visible to near-infrared regions. Under 638 nm irradiation, the device achieves self-powered operation with a responsivity of 1.98 A/W, a specific detectivity of 1.15 × 1011 Jones, and an external quantum efficiency of 387%. Moreover, the polarization ratio of the device is electrically tunable (1.47–3.17), enabling the realization of an XNOR-based optical encryption system in which polarization angles and gate voltages serve as optical data bits and electrical keys, respectively. This work not only presents an efficient strategy for enhancing polarization sensitivity and broadband self-powered detection but also establishes a route toward secure and reconfigurable optoelectronic information processing based on 2D van der Waals (vdW) heterostructures.
偏振光加密实现了信息通道并行,增强了防窃听能力,提高了数据传输能力和信息安全性。然而,传统的系统严重依赖于体积庞大且离散的组件,如偏振器和波片,这使得设备集成和小型化变得复杂。为了解决这些限制,我们展示了一种基于GeSe/2H-MoTe2异质结构的偏振分辨光电探测器。利用各向异性GeSe和双极性2H-MoTe2层之间的ii型能带排列和强界面耦合,该器件实现了从可见光到近红外区域的高效载流子分离和宽带光响应。在638 nm辐照下,器件实现自供电运行,响应度为1.98 a /W,比探测率为1.15 × 1011 Jones,外量子效率为387%。此外,器件的偏振比是电可调的(1.47-3.17),可以实现基于xnor的光加密系统,其中偏振角和栅极电压分别作为光数据位和电密钥。这项工作不仅提出了提高偏振灵敏度和宽带自供电检测的有效策略,而且为基于二维范德华(vdW)异质结构的安全和可重构光电信息处理建立了一条途径。
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引用次数: 0
Diverse nanostructures of bc8 silicon mediated by controllable transition kinetics of beta-Sn silicon β - sn硅的可控转变动力学介导bc8硅的不同纳米结构
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-12 DOI: 10.1063/5.0322983
Yingxue Han, Shang Peng, Mei Li, Jun Yuan, Tingting Zhao, Bohao Zhao, Yanlong Chen, Qi Feng, Jiao An, Chuanlong Lin
Metastable polymorphs of silicon exhibit direct and narrow band gaps, offering broad application potential. The transition kinetics in the formation of metastable Si have been extensively studied, but the relationship between transition conditions and nanostructures of product phases remains unclear. Here, we report diverse nanostructures of body-centered cubic (bc8) Si formed by rapid decompression of beta-Sn Si at different rates. High-resolution transmission electron microscopy images show slow decompression results in the formation of bc8 nanocrystals with long-range order and abundant interfacial defects, including dislocation, twin, stacking fault, and internal lattice strain. In contrast, rapid decompression generates bc8 nanoclusters with a macroscopic amorphous characteristic, as evidenced by the broad diffuse halo in fast Fourier transform pattern. Statistical analysis of the size distribution shows that the grain size decreases with the increasing decompression rate, indicating a clear rate-dependent behavior. These findings provide structural evidence and mechanistic insights into the kinetically controlled formation of the metastable nanostructures for promising applications.
硅的亚稳态多晶具有直接和狭窄的带隙,具有广泛的应用潜力。亚稳硅形成过程中的转变动力学已被广泛研究,但转变条件与产物相纳米结构之间的关系尚不清楚。在这里,我们报道了不同的体心立方(bc8) Si纳米结构形成的快速减压-锡硅以不同的速率。高分辨率透射电镜图像显示,缓慢的减压导致bc8纳米晶体的形成,具有长程有序和丰富的界面缺陷,包括位错、孪晶、层错和内部晶格应变。相比之下,快速减压产生的bc8纳米团簇具有宏观无定形特征,这可以从快速傅里叶变换图中广泛的弥散晕中得到证明。尺寸分布的统计分析表明,随着减压速率的增加,晶粒尺寸减小,具有明显的速率依赖行为。这些发现为亚稳纳米结构的动力学控制形成提供了结构证据和机理见解,具有广阔的应用前景。
{"title":"Diverse nanostructures of bc8 silicon mediated by controllable transition kinetics of beta-Sn silicon","authors":"Yingxue Han, Shang Peng, Mei Li, Jun Yuan, Tingting Zhao, Bohao Zhao, Yanlong Chen, Qi Feng, Jiao An, Chuanlong Lin","doi":"10.1063/5.0322983","DOIUrl":"https://doi.org/10.1063/5.0322983","url":null,"abstract":"Metastable polymorphs of silicon exhibit direct and narrow band gaps, offering broad application potential. The transition kinetics in the formation of metastable Si have been extensively studied, but the relationship between transition conditions and nanostructures of product phases remains unclear. Here, we report diverse nanostructures of body-centered cubic (bc8) Si formed by rapid decompression of beta-Sn Si at different rates. High-resolution transmission electron microscopy images show slow decompression results in the formation of bc8 nanocrystals with long-range order and abundant interfacial defects, including dislocation, twin, stacking fault, and internal lattice strain. In contrast, rapid decompression generates bc8 nanoclusters with a macroscopic amorphous characteristic, as evidenced by the broad diffuse halo in fast Fourier transform pattern. Statistical analysis of the size distribution shows that the grain size decreases with the increasing decompression rate, indicating a clear rate-dependent behavior. These findings provide structural evidence and mechanistic insights into the kinetically controlled formation of the metastable nanostructures for promising applications.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"31 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2026-03-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147454402","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
Origami folding enables ultrahigh and reversible mechanical energy storage in pillared graphene 折纸折叠可以在柱状石墨烯中实现超高可逆的机械能存储
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-12 DOI: 10.1063/5.0316430
Pan Shi, Yao Chen, Tianyu Xie, Tong Guo, Jian Feng, Pooya Sareh
The ability to accommodate large deformation while maintaining full structural recoverability remains a challenge in the design of lightweight mechanical energy storage materials. Here, we demonstrate through molecular dynamics simulations that pillared graphene, a three-dimensional nanostructure made of parallel graphene sheets interconnected by vertically aligned carbon nanotubes, can achieve an unprecedented combination of ultrahigh mechanical energy storage and complete structural recovery up to 38% compressive strain. This exceptional performance stems from a unique deformation mechanism wherein the graphene layers undergo reversible Miura origami-like folding, generating an extended stress plateau together with pronounced auxetic behavior. Parametric analyses further reveal distinct roles of geometric parameters: inter-pillar distance governs the transition between global and localized folding modes, while pillar height independently modulates the elastic modulus without compromising deformation reversibility. Our findings establish a design paradigm for high-capacity energy storage and mechanical buffering systems, and highlight architecturally guided deformation as an effective strategy for exploiting the elastic potential of carbon-based nanomaterials.
在适应大变形的同时保持结构完全可恢复性的能力仍然是轻质机械储能材料设计中的一个挑战。在这里,我们通过分子动力学模拟证明了柱状石墨烯,一种由垂直排列的碳纳米管相互连接的平行石墨烯片组成的三维纳米结构,可以实现超高机械能量存储和高达38%压缩应变的完全结构恢复的前所未有的组合。这种优异的性能源于一种独特的变形机制,其中石墨烯层经历了可逆的三浦折纸式折叠,产生了延长的应力平台,并具有明显的形变行为。参数分析进一步揭示了几何参数的不同作用:柱间距离控制着整体和局部折叠模式之间的转换,而柱高度独立地调节弹性模量,而不影响变形可变性。我们的研究结果为高容量储能和机械缓冲系统建立了一个设计范例,并强调了建筑引导变形是开发碳基纳米材料弹性潜力的有效策略。
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引用次数: 0
Stabilization of Rydberg dissipative time crystals using a scanning Fabry–Pérot interferometer transfer lock 利用扫描法布里-普氏干涉仪传输锁稳定Rydberg耗散时间晶体
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-11 DOI: 10.1063/5.0305148
D. Arumugam, B. Feyissa
Stabilization of laser frequencies is critical for sensitive Rydberg measurements, including in applications such as dissipative time-crystal (DTC) dynamics, yet conventional approaches often require complex or costly hardware. We demonstrate a compact, low-cost stabilization method using a scanning Fabry–Pérot interferometer (SFPI) to transfer lock a 960 nm coupler laser to an 852 nm Cs reference laser. The lock suppresses coupler multi-MHz free-running drift and improves the Allan deviation by up to an order of magnitude, reaching <75 kHz at τ ∼ 66 s. Applied to DTC oscillations using a Rb 2-photon D2 transition, the second harmonic generated at 480 nm (from 960 nm lock) reduces DTC frequency drift from >20 kHz to a few kHz and lowers instability by more than an order of magnitude with a minimum Allan deviation of 0.2 kHz at τ < 10 s. These results establish SFPI-based transfer locking as a practical and accurate approach for scalable multi-laser Rydberg experiments that require long-term stability in a compact and low-cost system.
激光频率的稳定对于敏感的里德伯测量至关重要,包括在耗散时间晶体(DTC)动力学等应用中,然而传统的方法通常需要复杂或昂贵的硬件。我们展示了一种紧凑,低成本的稳定方法,使用扫描法布里- p干涉仪(SFPI)将锁定960 nm的耦合器激光器转移到852 nm的Cs参考激光器。锁抑制了耦合器多mhz自由运行漂移,并将艾伦偏差提高了一个数量级,达到&;lt;75 kHz, τ ~ 66 s。利用Rb 2光子D2跃迁应用于DTC振荡,在480 nm处产生的二次谐波(从960 nm锁定)减少了DTC的频率漂移。20khz至几kHz,降低了一个数量级以上的不稳定性,在τ &;lt下的最小艾伦偏差为0.2 kHz;十年代。这些结果建立了基于sfpi的转移锁定作为可扩展的多激光里德堡实验的实用和准确的方法,需要在紧凑和低成本的系统中实现长期稳定。
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引用次数: 0
Charge-density wave-mediated soft phonon modes suppress the temperature dependence of lattice thermal conductivity in 2H-NbSe2 电荷密度波介导的软声子模式抑制了2H-NbSe2晶格热导率的温度依赖性
IF 4 2区 物理与天体物理 Q2 PHYSICS, APPLIED Pub Date : 2026-03-11 DOI: 10.1063/5.0309984
Jinfeng Yang, Zhunyun Tang, Yongze Xu, Xiaonan Wang, Tao Ouyang, Huarui Sun
Layered NbSe2 has attracted extensive interest as a prototypical system where multiband superconductivity coexists with a charge-density wave (CDW) order. Here, using self-consistent phonon theory to incorporate anharmonic renormalization, CDW critical temperatures in the bulk and monolayer 2H-NbSe2 are calculated to be 66 and 116 K, respectively, in good agreement with reported experiments. First-principles anharmonic lattice dynamics combined with Peierls–Boltzmann transport theory reveals that strong phonon anharmonicity, arising from low-energy special soft phonon modes mediated by the CDW behavior, results in a low lattice thermal conductivity (κL) with weak temperature dependence. Strikingly, four-phonon (4ph) interactions contribute to a dramatic suppression of κL, particularly in the in-plane direction, reinforcing the critical role of strong phonon anharmonicity. These results provide a detailed microscopic understanding of CDW transition and thermal transport in CDW materials.
层状NbSe2作为一种多带超导性与电荷密度波(CDW)有序共存的原型系统引起了广泛的兴趣。本研究利用自洽声子理论结合非谐波重整化,计算出本体和单层2H-NbSe2的CDW临界温度分别为66 K和116 K,与已有的实验结果吻合良好。第一原理非调和晶格动力学结合peerls - boltzmann输运理论揭示了由CDW行为介导的低能特殊软声子模式引起的强声子非调和性导致晶格热导率(κL)低且温度依赖性弱。引人注目的是,四声子(4ph)相互作用有助于显著抑制κL,特别是在平面方向上,强化了强声子非谐波的关键作用。这些结果为CDW材料中的CDW转变和热输运提供了详细的微观理解。
{"title":"Charge-density wave-mediated soft phonon modes suppress the temperature dependence of lattice thermal conductivity in 2H-NbSe2","authors":"Jinfeng Yang, Zhunyun Tang, Yongze Xu, Xiaonan Wang, Tao Ouyang, Huarui Sun","doi":"10.1063/5.0309984","DOIUrl":"https://doi.org/10.1063/5.0309984","url":null,"abstract":"Layered NbSe2 has attracted extensive interest as a prototypical system where multiband superconductivity coexists with a charge-density wave (CDW) order. Here, using self-consistent phonon theory to incorporate anharmonic renormalization, CDW critical temperatures in the bulk and monolayer 2H-NbSe2 are calculated to be 66 and 116 K, respectively, in good agreement with reported experiments. First-principles anharmonic lattice dynamics combined with Peierls–Boltzmann transport theory reveals that strong phonon anharmonicity, arising from low-energy special soft phonon modes mediated by the CDW behavior, results in a low lattice thermal conductivity (κL) with weak temperature dependence. Strikingly, four-phonon (4ph) interactions contribute to a dramatic suppression of κL, particularly in the in-plane direction, reinforcing the critical role of strong phonon anharmonicity. These results provide a detailed microscopic understanding of CDW transition and thermal transport in CDW materials.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"11 1","pages":""},"PeriodicalIF":4.0,"publicationDate":"2026-03-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":null,"resultStr":null,"platform":"Semanticscholar","paperid":"147393239","PeriodicalName":null,"FirstCategoryId":null,"ListUrlMain":null,"RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":"","EPubDate":null,"PubModel":null,"JCR":null,"JCRName":null,"Score":null,"Total":0}
引用次数: 0
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Applied Physics Letters
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