Digitally-assisted structure design of a large-size proton exchange membrane fuel cell

IF 32.4 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Energy & Environmental Science Pub Date : 2024-11-22 DOI:10.1039/d4ee04713c
Wenming Huo, Linhao Fan, Yunfei Xu, Mohamed Benbouzid, Wenzhen Xu, Fei Gao, Weizhuo Li, Nian Shan, Biao Xie, Haipeng Huang, Bohao Liu, Yassine Amirat, Chuan Fang, Xiaohui Li, Quanquan Gan, Feiqiang Li, Kui Jiao
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Abstract

The flow field plays a significant role in the performance of proton exchange membrane (PEM) fuel cells. However, its complex structure leads to unacceptable development costs and time commonly using the trial-and-error method based on many experiments. Herein, we propose a digitally-assisted method to accelerate the development process and reduce costs. Comprehensive experiments and tests are conducted using the commercial-size PEM fuel cell with an active area of 332 cm2, including the investigation of polarization curves, five sensitivity parameters under seven different current densities, and spatial distributions. A high-resolution printed circuit board with 408 segments of 0.8 cm2 is employed to explore the current density distribution. The commercial-size PEM fuel cell is further digitalized with a self-developed fuel cell numerical model, which is strictly verified in terms of all experimental data. The digital multi-physics information inside PEM fuel cells is obtained and evaluated via this efficient numerical model in order to search for the structure defects quickly and accurately. Afterwards, targeted structure optimization is effectively carried out to achieve a better performance, with the maximum deviation of oxygen concentration in the channels decreasing from 26.33% to 3.78%. This digital method is very valuable for the forward design of flow field structures to considerably reduce the development cost and time.

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大尺寸质子交换膜燃料电池的数字辅助结构设计
流场对质子交换膜(PEM)燃料电池的性能起着重要作用。然而,由于其结构复杂,通常采用基于多次实验的试错法,开发成本和时间都难以接受。在此,我们提出了一种数字辅助方法,以加快开发过程并降低成本。我们使用活性面积为 332 平方厘米的商用尺寸 PEM 燃料电池进行了全面的实验和测试,包括极化曲线、七种不同电流密度下的五个灵敏度参数以及空间分布的研究。为了探索电流密度分布,采用了一块有 408 个 0.8 平方厘米段的高分辨率印刷电路板。通过自主开发的燃料电池数值模型,对商用尺寸的 PEM 燃料电池进行了进一步的数字化,并对所有实验数据进行了严格验证。通过这个高效的数值模型,可以获得并评估 PEM 燃料电池内部的数字化多物理场信息,从而快速准确地寻找结构缺陷。随后,有针对性地进行结构优化,有效地提高了性能,使通道中氧气浓度的最大偏差从 26.33% 降至 3.78%。这种数字化方法对于流场结构的正向设计非常有价值,可大大减少开发成本和时间。
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来源期刊
Energy & Environmental Science
Energy & Environmental Science 化学-工程:化工
CiteScore
50.50
自引率
2.20%
发文量
349
审稿时长
2.2 months
期刊介绍: Energy & Environmental Science, a peer-reviewed scientific journal, publishes original research and review articles covering interdisciplinary topics in the (bio)chemical and (bio)physical sciences, as well as chemical engineering disciplines. Published monthly by the Royal Society of Chemistry (RSC), a not-for-profit publisher, Energy & Environmental Science is recognized as a leading journal. It boasts an impressive impact factor of 8.500 as of 2009, ranking 8th among 140 journals in the category "Chemistry, Multidisciplinary," second among 71 journals in "Energy & Fuels," second among 128 journals in "Engineering, Chemical," and first among 181 scientific journals in "Environmental Sciences." Energy & Environmental Science publishes various types of articles, including Research Papers (original scientific work), Review Articles, Perspectives, and Minireviews (feature review-type articles of broad interest), Communications (original scientific work of an urgent nature), Opinions (personal, often speculative viewpoints or hypotheses on current topics), and Analysis Articles (in-depth examination of energy-related issues).
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