Theory of magnetotrion-polaritons in transition metal dichalcogenide monolayers

IF 9.1 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY npj 2D Materials and Applications Pub Date : 2024-11-27 DOI:10.1038/s41699-024-00517-1
Andrejs Kudlis, Ivan Aleksandrov, Zaur Alisultanov, Kalman Varga, Ivan Shelykh, Vanik Shahnazaryan
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Abstract

Magnetic field is a powerful tool for the manipulation of material’s electronic and optical properties. In the domain of transition metal dichalcogenide monolayers, it allows one to unveil the spin, valley, and orbital properties of many-body excitonic complexes. Here we study theoretically the impact of normal-to-plane magnetic field on trions and trion-polaritons. We demonstrate that spin and orbital effects of a magnetic field give comparable contributions to the trion energies. Moreover, as magnetic field redistributes the free electron gas between two valleys in the conductance band, the trion-photon coupling becomes polarization and valley dependent. This results in an effective giant Zeeman splitting of trion-polaritons, in-line with the recent experimental observations.

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过渡金属二卤化物单层中的磁三离子极化子理论
磁场是操纵材料电子和光学特性的有力工具。在过渡金属二卤化物单层领域,磁场可以揭示多体激子复合物的自旋、谷和轨道特性。在这里,我们从理论上研究了法向平面磁场对三离子和三离子极化子的影响。我们证明,磁场的自旋和轨道效应对三离子能量的贡献不相上下。此外,由于磁场重新分配了电导带中两个波谷之间的自由电子气体,三离子-光子耦合变得与极化和波谷有关。这导致了三离子-极化子的有效巨型泽曼分裂,与最近的实验观测结果一致。
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来源期刊
npj 2D Materials and Applications
npj 2D Materials and Applications Engineering-Mechanics of Materials
CiteScore
14.50
自引率
2.10%
发文量
80
审稿时长
15 weeks
期刊介绍: npj 2D Materials and Applications publishes papers on the fundamental behavior, synthesis, properties and applications of existing and emerging 2D materials. By selecting papers with the potential for impact, the journal aims to facilitate the transfer of the research of 2D materials into wide-ranging applications.
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