Mechanism and Application of Optical Modulation of Terahertz Waves in a Perovskite Heterojunction

IF 4.3 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC ACS Applied Electronic Materials Pub Date : 2024-11-13 DOI:10.1021/acsaelm.4c0157810.1021/acsaelm.4c01578
Wen Li, Hengzhen Cheng, Caiyu Feng, Weiyi Zhou and Bo Zhang*, 
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Abstract

We investigated the mechanism and application of the modulation of terahertz waves using perovskite heterostructures. At the interface between PEDOT:PSS and the perovskite layers under excitation by an external light source, photogenerated carriers transferred from the perovskite layer to the PEDOT:PSS layer, which was accompanied by charge accumulation. A large number of photogenerated carriers scattered terahertz waves, thereby modulating the terahertz signal in the sample. The process of modulation and recovery of the terahertz signal by a perovskite material under external light is analogous to the principle of biological synapses, which are involved in memory and learning in animal brains. This enabled us to develop perovskite-based synaptic devices. The memory properties of perovskite heterojunction materials open up applications of terahertz technology.

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过氧化物异质结中太赫兹波的光学调制机理与应用
我们研究了利用包晶异质结构调制太赫兹波的机制和应用。在外部光源的激发下,PEDOT:PSS 层和包晶层之间的界面上,光生载流子从包晶层转移到 PEDOT:PSS 层,并伴随着电荷积累。大量光生载流子散射太赫兹波,从而调制了样品中的太赫兹信号。包晶材料在外部光照下调制和恢复太赫兹信号的过程类似于生物突触的原理,而生物突触参与了动物大脑的记忆和学习。这使我们得以开发基于包晶的突触设备。包晶异质结材料的记忆特性为太赫兹技术的应用开辟了道路。
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来源期刊
CiteScore
7.20
自引率
4.30%
发文量
567
期刊介绍: ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric. Indexed/​Abstracted: Web of Science SCIE Scopus CAS INSPEC Portico
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