Optimisation of CuO/AC, Fe2O3/AC synergistic multi-electrode DBD reactor for degradation of ATZ in water

IF 1.9 4区 工程技术 Q3 ENGINEERING, ELECTRICAL & ELECTRONIC Journal of Electrostatics Pub Date : 2024-11-28 DOI:10.1016/j.elstat.2024.104003
Xinjun Shen , Fan He , Jing Zhang , Cong Wang
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Abstract

Atrazine (ATZ) is a synthetic triazine herbicide and has become a new pollutant in environment water. In this study, a multi-high-voltage, double-grounded- pole dielectric barrier discharge (DBD) reactor was designed to degrade ATZ in water. The effects of different factors, such as input voltage, air flow rate, and pH, on the degradation of ATZ in the DBD reactor were compared using response surface methodology. The optimal reaction conditions for the degradation of ATZ by DBD were determined by fitting the model to the experiment: air flow rate of 100 L/h, input voltage of 32 kV and pH of 10. The degradation efficiency obtained was 97.89 %, which closely matched the simulation, indicating that the model had good correlation and consistency with the measured data. In this experiment, catalysts such as activated carbon loaded with CuO and Fe2O3 were added to DBD reactor to improve the utilization of active substances and enhance the degradation of ATZ. The catalysts were characterized by FT-IR, XRD, XPS and SEM, proving that they promoted the degradation of ATZ.
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优化用于降解水中 ATZ 的 CuO/AC、Fe2O3/AC 协同多电极 DBD 反应器
阿特拉津(ATZ)是一种人工合成的三嗪类除草剂,已成为一种新的水环境污染物。本研究设计了一个多高压、双接地极介质阻挡放电(DBD)反应器来降解水中的阿特拉津。采用响应面方法比较了输入电压、空气流速和 pH 值等不同因素对 DBD 反应器中 ATZ 降解的影响。通过将模型与实验进行拟合,确定了 DBD 降解 ATZ 的最佳反应条件:空气流量为 100 L/h,输入电压为 32 kV,pH 值为 10。得到的降解效率为 97.89%,与模拟结果非常吻合,表明该模型与测量数据具有良好的相关性和一致性。本实验在 DBD 反应器中添加了负载 CuO 和 Fe2O3 的活性炭等催化剂,以提高活性物质的利用率并增强 ATZ 的降解能力。通过傅立叶变换红外光谱、X射线衍射、XPS和扫描电镜对催化剂进行表征,证明催化剂促进了ATZ的降解。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Journal of Electrostatics
Journal of Electrostatics 工程技术-工程:电子与电气
CiteScore
4.00
自引率
11.10%
发文量
81
审稿时长
49 days
期刊介绍: The Journal of Electrostatics is the leading forum for publishing research findings that advance knowledge in the field of electrostatics. We invite submissions in the following areas: Electrostatic charge separation processes. Electrostatic manipulation of particles, droplets, and biological cells. Electrostatically driven or controlled fluid flow. Electrostatics in the gas phase.
期刊最新文献
Editorial Board Optimisation of CuO/AC, Fe2O3/AC synergistic multi-electrode DBD reactor for degradation of ATZ in water Triboelectric charging of polydisperse particles in a developed pipe flow Effect of field emission on contact spark in the spark test apparatus A theoretical approach towards developing space charge formation in lossy dielectrics
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