Kaiyong Tang , Hui Cui , Li Fu , Siyuan Zhang , Haijun Fan , Yan Zeng , Mo Zhou
{"title":"Optimize neutron minimum detectable dose of OSL composite neutron detectors based on Al2O3:C and 6LiF","authors":"Kaiyong Tang , Hui Cui , Li Fu , Siyuan Zhang , Haijun Fan , Yan Zeng , Mo Zhou","doi":"10.1016/j.radphyschem.2024.112432","DOIUrl":null,"url":null,"abstract":"<div><div>The n/γ ratio and minimum detectable dose (MDD) are two crucial parameters in the measurement of neutrons in a mixed field comprising both neutrons and gamma rays. In this study, four OSL neutron detectors based on <sup>6</sup>LiF and very sensitive α-Al<sub>2</sub>O<sub>3</sub>:C powder with grain sizes of less than 100 and 38 μm, respectively, were developed. The first use of the detector pair comprised single-crystal α-Al<sub>2</sub>O<sub>3</sub>:C detectors and neutron-sensitive OSL composite detectors represents a pioneering advancement in the field. The n/γ ratio and MDD at various integration times were first investigated. For the four neutron detectors, the neutron response of the neutron detectors with a mixture of 1:1 mass ratio of the α-Al<sub>2</sub>O<sub>3</sub>:C powder with grain sizes of less than 100 μm and <sup>6</sup>LiF exposed to the D<sub>2</sub>O moderated <sup>252</sup>Cf source was the highest. When the integration time was 0.5 s, the MDD of the neutron detectors with a mixture of 1:1 mass ratio of the α-Al<sub>2</sub>O<sub>3</sub>:C powder with grain sizes of less than 100 μm and <sup>6</sup>LiF was 6.1, 41.0, and 56.1 μSv, respectively, when irradiated by a calibrated D<sub>2</sub>O moderated <sup>252</sup>Cf source, a bare <sup>252</sup>Cf source and a bare <sup>241</sup>Am–Be source. A comparison of the results indicates that the composite OSL neutron detectors based on Al<sub>2</sub>O<sub>3</sub>:C and <sup>6</sup>LiF of this study have demonstrated a notable improvement in MDD.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"229 ","pages":"Article 112432"},"PeriodicalIF":2.8000,"publicationDate":"2024-11-28","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969806X24009241","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
The n/γ ratio and minimum detectable dose (MDD) are two crucial parameters in the measurement of neutrons in a mixed field comprising both neutrons and gamma rays. In this study, four OSL neutron detectors based on 6LiF and very sensitive α-Al2O3:C powder with grain sizes of less than 100 and 38 μm, respectively, were developed. The first use of the detector pair comprised single-crystal α-Al2O3:C detectors and neutron-sensitive OSL composite detectors represents a pioneering advancement in the field. The n/γ ratio and MDD at various integration times were first investigated. For the four neutron detectors, the neutron response of the neutron detectors with a mixture of 1:1 mass ratio of the α-Al2O3:C powder with grain sizes of less than 100 μm and 6LiF exposed to the D2O moderated 252Cf source was the highest. When the integration time was 0.5 s, the MDD of the neutron detectors with a mixture of 1:1 mass ratio of the α-Al2O3:C powder with grain sizes of less than 100 μm and 6LiF was 6.1, 41.0, and 56.1 μSv, respectively, when irradiated by a calibrated D2O moderated 252Cf source, a bare 252Cf source and a bare 241Am–Be source. A comparison of the results indicates that the composite OSL neutron detectors based on Al2O3:C and 6LiF of this study have demonstrated a notable improvement in MDD.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.