Optimize neutron minimum detectable dose of OSL composite neutron detectors based on Al2O3:C and 6LiF

IF 2.8 3区 物理与天体物理 Q3 CHEMISTRY, PHYSICAL Radiation Physics and Chemistry Pub Date : 2025-04-01 Epub Date: 2024-11-28 DOI:10.1016/j.radphyschem.2024.112432
Kaiyong Tang , Hui Cui , Li Fu , Siyuan Zhang , Haijun Fan , Yan Zeng , Mo Zhou
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Abstract

The n/γ ratio and minimum detectable dose (MDD) are two crucial parameters in the measurement of neutrons in a mixed field comprising both neutrons and gamma rays. In this study, four OSL neutron detectors based on 6LiF and very sensitive α-Al2O3:C powder with grain sizes of less than 100 and 38 μm, respectively, were developed. The first use of the detector pair comprised single-crystal α-Al2O3:C detectors and neutron-sensitive OSL composite detectors represents a pioneering advancement in the field. The n/γ ratio and MDD at various integration times were first investigated. For the four neutron detectors, the neutron response of the neutron detectors with a mixture of 1:1 mass ratio of the α-Al2O3:C powder with grain sizes of less than 100 μm and 6LiF exposed to the D2O moderated 252Cf source was the highest. When the integration time was 0.5 s, the MDD of the neutron detectors with a mixture of 1:1 mass ratio of the α-Al2O3:C powder with grain sizes of less than 100 μm and 6LiF was 6.1, 41.0, and 56.1 μSv, respectively, when irradiated by a calibrated D2O moderated 252Cf source, a bare 252Cf source and a bare 241Am–Be source. A comparison of the results indicates that the composite OSL neutron detectors based on Al2O3:C and 6LiF of this study have demonstrated a notable improvement in MDD.
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基于Al2O3:C和6LiF的OSL复合中子探测器中子最小可探测剂量优化
n/γ比和最小可探测剂量(MDD)是测量中子和伽马射线混合场中中子的两个关键参数。在本研究中,分别研制了4种基于6LiF和高灵敏度α-Al2O3:C粉末(晶粒尺寸小于100 μm和38 μm)的OSL中子探测器。首次使用由单晶α-Al2O3:C探测器和中子敏感OSL复合探测器组成的探测器对代表了该领域的开创性进步。首先研究了不同积分时间的n/γ比和MDD。在D2O慢化的252Cf源中,α-Al2O3:C粉末(粒径小于100 μm)与6LiF质量比为1:1时,中子探测器的中子响应最高。当积分时间为0.5 s时,经标定D2O慢化252Cf源、裸252Cf源和裸241Am-Be源辐照后,α-Al2O3:C(粒径小于100 μm)粉末质量比为1:1和6LiF混合的中子探测器的MDD分别为6.1、41.0和56.1 μSv。结果表明,本研究的Al2O3:C和6LiF复合OSL中子探测器在MDD方面有明显改善。
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来源期刊
Radiation Physics and Chemistry
Radiation Physics and Chemistry 化学-核科学技术
CiteScore
5.60
自引率
17.20%
发文量
574
审稿时长
12 weeks
期刊介绍: Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing. The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.
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