Electrical Dissipation Factor Measurements of Droplet Impact-Derived Microgels with Different Topological Structures

IF 26.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Advanced Materials Pub Date : 2024-12-01 DOI:10.1002/adma.202413457
Lei Wang, Xuerong Ding, Yiheng Hu, Qiurui Li, Yibing Bian, Yefan Duan, Shujie Lu, Hongbin Han, Ning Gu, Jianfei Sun
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Abstract

Topology, the study of properties that are invariant under continuous transformations, in which the number of pores (genus) is a profound concept that determines a number of properties that have been verified in many microscopic systems, but have not been studied in macroscopic materials. Microgels are widely used materials, and based on microfluidics, regular, stable, and reproducible microgels can be prepared, but studies from the perspective of topological principles have not been reported. In this paper, a system based on a boric acid ester rapid cross-linking strategy that can rapidly capture topological changes during the transient process of droplet-to-ring transition is proposed. The electrical dissipation properties associated with different transient topologies during the process are also investigated, demonstrating that the change of topological structures in macroscopic materials also affected their electrical properties, laying the foundation for the design of modulated macroscopic micro structured materials based on topology theory.

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具有不同拓扑结构的液滴冲击微凝胶的电耗散系数测量
拓扑学,研究连续变换下不变的性质,其中孔隙(属)的数量是一个深刻的概念,它决定了许多性质,这些性质在许多微观系统中得到了验证,但在宏观材料中尚未得到研究。微凝胶是一种应用广泛的材料,基于微流体可以制备出规则、稳定、可重复的微凝胶,但从拓扑学原理角度进行的研究尚未见报道。本文提出了一种基于硼酸酯快速交联策略的系统,该系统可以快速捕获液滴到环过渡过程中的拓扑变化。研究了不同暂态拓扑在此过程中的电耗散特性,表明宏观材料中拓扑结构的变化也会影响其电性能,为基于拓扑理论的调制宏观微结构材料的设计奠定了基础。
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阿拉丁
Polyvinyl alcohol
阿拉丁
Boric acid
阿拉丁
Sodium metasilicate
阿拉丁
Sodium hydroxide
阿拉丁
Ethanol
阿拉丁
Rhodamine B labeled bovine serum albumin
阿拉丁
FeCl2·4H2O
阿拉丁
Na2S·9H2O
阿拉丁
Bovine serum albumin
阿拉丁
Polyvinyl alcohol
阿拉丁
boric acid
阿拉丁
sodium metasilicate
阿拉丁
sodium hydroxide
阿拉丁
ethanol
阿拉丁
rhodamine B labeled bovine serum albumin
阿拉丁
FeCl2·4H2O
阿拉丁
Na2S·9H2O
阿拉丁
bovine serum albumin
阿拉丁
Polyvinyl alcohol
阿拉丁
boric acid
阿拉丁
sodium metasilicate
阿拉丁
sodium hydroxide
阿拉丁
ethanol
阿拉丁
rhodamine B labeled bovine serum albumin
阿拉丁
FeCl2·4H2O
阿拉丁
Na2S·9H2O
阿拉丁
bovine serum albumin
来源期刊
Advanced Materials
Advanced Materials 工程技术-材料科学:综合
CiteScore
43.00
自引率
4.10%
发文量
2182
审稿时长
2 months
期刊介绍: Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.
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