Updated uranium reference material 231Pa/235U consensus model ages for nuclear forensics

IF 1.5 3区 化学 Q3 CHEMISTRY, ANALYTICAL Journal of Radioanalytical and Nuclear Chemistry Pub Date : 2024-10-19 DOI:10.1007/s10967-024-09818-7
Mark A. Edwards, Zsolt Varga, Amy M. Gaffney, Joanna S. Denton, John R. Engel, Matthew S. Gonzales, Theresa M. Kayzar-Boggs, Klaus Mayer, Adrian Nicholl, Matthew E. Sanborn, Robert E. Steiner, Cheng Tarng, Kerri C. Treinen, Maria Wallenius, Allison M. Wende
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Abstract

Radiochronometry provides the model age of nuclear materials, which is useful for understanding the production history of materials found outside of regulatory control. Certified reference materials (CRMs) are important for radiochronometry to increase confidence in measurement quality; however, the absence of 231Pa/235U CRMs necessitates that nuclear forensic laboratories measure the 231Pa/235U model ages of preexisting uranium reference materials. Here, new consensus 231Pa/235U model ages are reported from three nuclear forensic laboratories for three reference materials using current analytical methods. These updated consensus values can be used for quality control of 231Pa/235U model age measurements.

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更新铀参考材料231Pa/235U共识模型年龄核法医
放射性计时法提供了核材料的模型年龄,这对于了解在监管控制之外发现的材料的生产历史是有用的。经认证的标准物质(CRMs)对于提高测量质量的信心至关重要;然而,由于缺乏231Pa/235U标准物质,核法医实验室必须测量先前存在的铀参考物质的231Pa/235U模型年龄。本文报道了三个核法医实验室使用现有分析方法对三种标准物质的231Pa/235U模型年龄的新共识。这些更新的共识值可用于231Pa/235U模型年龄测量的质量控制。
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来源期刊
CiteScore
2.80
自引率
18.80%
发文量
504
审稿时长
2.2 months
期刊介绍: An international periodical publishing original papers, letters, review papers and short communications on nuclear chemistry. The subjects covered include: Nuclear chemistry, Radiochemistry, Radiation chemistry, Radiobiological chemistry, Environmental radiochemistry, Production and control of radioisotopes and labelled compounds, Nuclear power plant chemistry, Nuclear fuel chemistry, Radioanalytical chemistry, Radiation detection and measurement, Nuclear instrumentation and automation, etc.
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