{"title":"All-Day, All-Weather Desalination Using a Contactless Evaporator with Antisalt Fouling Property.","authors":"Higgins M Wilson, Tawseef A Wani, Sang J Lee","doi":"10.1021/acsami.4c17002","DOIUrl":null,"url":null,"abstract":"<p><p>Interfacial solar steam generation (ISSG) technology provides a promising solution to the global issue of freshwater scarcity. However, its practical application is hindered by salt fouling and inconsistent solar illumination. In this work, a novel interfacial solar steam generator is proposed that integrates contactless design with low-voltage joule heating to provide all-day, all-weather freshwater generation. The contactless design utilizes a solar-reduced graphene oxide coated carbon fabric (SRGO-CF) as a heat generator and super hydrophilic paper walls as water transport channels. The contactless device can generate steam at the maximum rate of 4.27 kg m<sup>-2</sup> h<sup>-1</sup> under 1 sun solar illumination and small input voltage due to the excellent photothermal and electrothermal capabilities of SRGO-CF. At an input voltage of 2.5 V, the SRGO-CF evaporator exhibits an evaporation rate of 3.52 kg m<sup>-2</sup> h<sup>-1</sup> and 2.32 kg m<sup>-2</sup> h<sup>-1</sup> for 3.5 wt % salt water respectively with and without 1 sun illumination for a long period of time without any salt fouling, demonstrating its all-day, all-weather capability. The proposed contactless ISSG evaporator can resolve the impractical issue of conventional ISSG-based evaporators owing to irregular weather conditions and salt fouling issues while also promoting zero liquid discharge-based salt harvesting.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":" ","pages":"69450-69458"},"PeriodicalIF":8.3000,"publicationDate":"2024-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.4c17002","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/12/4 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Interfacial solar steam generation (ISSG) technology provides a promising solution to the global issue of freshwater scarcity. However, its practical application is hindered by salt fouling and inconsistent solar illumination. In this work, a novel interfacial solar steam generator is proposed that integrates contactless design with low-voltage joule heating to provide all-day, all-weather freshwater generation. The contactless design utilizes a solar-reduced graphene oxide coated carbon fabric (SRGO-CF) as a heat generator and super hydrophilic paper walls as water transport channels. The contactless device can generate steam at the maximum rate of 4.27 kg m-2 h-1 under 1 sun solar illumination and small input voltage due to the excellent photothermal and electrothermal capabilities of SRGO-CF. At an input voltage of 2.5 V, the SRGO-CF evaporator exhibits an evaporation rate of 3.52 kg m-2 h-1 and 2.32 kg m-2 h-1 for 3.5 wt % salt water respectively with and without 1 sun illumination for a long period of time without any salt fouling, demonstrating its all-day, all-weather capability. The proposed contactless ISSG evaporator can resolve the impractical issue of conventional ISSG-based evaporators owing to irregular weather conditions and salt fouling issues while also promoting zero liquid discharge-based salt harvesting.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.