{"title":"All-Day, All-Weather Desalination Using a Contactless Evaporator with Antisalt Fouling Property.","authors":"Higgins M Wilson, Tawseef A Wani, Sang J Lee","doi":"10.1021/acsami.4c17002","DOIUrl":null,"url":null,"abstract":"<p><p>Interfacial solar steam generation (ISSG) technology provides a promising solution to the global issue of freshwater scarcity. However, its practical application is hindered by salt fouling and inconsistent solar illumination. In this work, a novel interfacial solar steam generator is proposed that integrates contactless design with low-voltage joule heating to provide all-day, all-weather freshwater generation. The contactless design utilizes a solar-reduced graphene oxide coated carbon fabric (SRGO-CF) as a heat generator and super hydrophilic paper walls as water transport channels. The contactless device can generate steam at the maximum rate of 4.27 kg m<sup>-2</sup> h<sup>-1</sup> under 1 sun solar illumination and small input voltage due to the excellent photothermal and electrothermal capabilities of SRGO-CF. At an input voltage of 2.5 V, the SRGO-CF evaporator exhibits an evaporation rate of 3.52 kg m<sup>-2</sup> h<sup>-1</sup> and 2.32 kg m<sup>-2</sup> h<sup>-1</sup> for 3.5 wt % salt water respectively with and without 1 sun illumination for a long period of time without any salt fouling, demonstrating its all-day, all-weather capability. The proposed contactless ISSG evaporator can resolve the impractical issue of conventional ISSG-based evaporators owing to irregular weather conditions and salt fouling issues while also promoting zero liquid discharge-based salt harvesting.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":" ","pages":"69450-69458"},"PeriodicalIF":8.2000,"publicationDate":"2024-12-18","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.4c17002","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2024/12/4 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Interfacial solar steam generation (ISSG) technology provides a promising solution to the global issue of freshwater scarcity. However, its practical application is hindered by salt fouling and inconsistent solar illumination. In this work, a novel interfacial solar steam generator is proposed that integrates contactless design with low-voltage joule heating to provide all-day, all-weather freshwater generation. The contactless design utilizes a solar-reduced graphene oxide coated carbon fabric (SRGO-CF) as a heat generator and super hydrophilic paper walls as water transport channels. The contactless device can generate steam at the maximum rate of 4.27 kg m-2 h-1 under 1 sun solar illumination and small input voltage due to the excellent photothermal and electrothermal capabilities of SRGO-CF. At an input voltage of 2.5 V, the SRGO-CF evaporator exhibits an evaporation rate of 3.52 kg m-2 h-1 and 2.32 kg m-2 h-1 for 3.5 wt % salt water respectively with and without 1 sun illumination for a long period of time without any salt fouling, demonstrating its all-day, all-weather capability. The proposed contactless ISSG evaporator can resolve the impractical issue of conventional ISSG-based evaporators owing to irregular weather conditions and salt fouling issues while also promoting zero liquid discharge-based salt harvesting.
界面太阳能蒸汽发电(ISSG)技术为解决全球淡水短缺问题提供了一个有希望的解决方案。然而,它的实际应用受到盐污染和不稳定的太阳光照的阻碍。在这项工作中,提出了一种新型的接触式太阳能蒸汽发生器,它将非接触式设计与低压焦耳加热相结合,提供全天候、全天候的淡水发电。非接触式设计利用太阳能还原氧化石墨烯涂层碳织物(SRGO-CF)作为热源,超亲水性纸壁作为水输送通道。由于SRGO-CF优异的光热和电热性能,该非接触式装置在1个太阳光照和小输入电压下产生蒸汽的最大速率为4.27 kg m-2 h-1。在2.5 V的输入电压下,SRGO-CF蒸发器的蒸发速率分别为3.52 kg m-2 h-1和2.32 kg m-2 h-1,在有和没有1个太阳光照的情况下长时间无盐污染,显示出全天候,全天候的能力。提出的非接触式ISSG蒸发器可以解决传统ISSG蒸发器由于不规则天气条件和盐垢问题而不切实际的问题,同时也促进了基于零液体排放的盐收集。
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.