Interfacial Electronic Charge Trapping and Photonic Carrier Excitation Coupling in Solution-Processed Zinc–Tin Oxide Thin-Film Transistors Applied for Logic Gate Design and Quantized Neural Network

IF 8.3 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY ACS Applied Materials & Interfaces Pub Date : 2024-12-18 DOI:10.1021/acsami.4c15102
Pei-Hsuan Chang, Wun-Yun Lin, Ya-Chi Huang, Yu-Chieh Chen, Li-Chung Shih, Jen-Sue Chen
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Abstract

Components needed in Artificial Intelligence with a higher information capacity are critically needed and have garnered significant attention at the forefront of information technology. This study utilizes solution-processed zinc–tin oxide (ZTO) thin-film phototransistors and modulates the values of VG, which allows for the regulation of electron trapping/detrapping at the ZTO/SiO2 interface. By coupling the excited photonic carrier and electronic trapping, logic gates such as “AND,” “OR,” “NAND,” and “NOR” can be achieved. With the exponential growth in data generation, efficient processing and storage solutions are imperative. However, extensive data transfer between computing units and storage limits the level of artificial neural networks (ANNs). Consequently, quantized neural networks (QNNs) have gained interest for their reduced computational resource requirements and lower consumption. In this context, we introduce an optimized ternary logic circuit based on ZTO devices. By utilizing optical modulation to adjust the turn-on voltage of the single device, we demonstrate the achievement of ternary current states, thereby providing three distinct discrete states. This configuration can be extended to QNN computing, demonstrating multilevel quantized current values for in-memory computation. We achieved a handwriting digit recognition rate of 91.6%, thereby demonstrating reliable QNN hardware performance. This robust QNN performance indicates that the metal oxide phototransistor shows significant potential for future ternary computing systems.

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溶液法氧化锌锡薄膜晶体管中的界面电子电荷捕获和光子载流子激发耦合在逻辑门设计和量化神经网络中的应用
人工智能亟需信息容量更高的组件,这在信息技术的前沿领域引起了极大关注。这项研究利用溶液加工的氧化锌锡(ZTO)薄膜光电晶体管,通过调节 VG 值,从而调节 ZTO/SiO2 界面的电子捕获/俘获。通过将激发的光子载流子与电子捕获耦合,可以实现 "AND"、"OR"、"NAND "和 "NOR "等逻辑门。随着数据生成量的指数级增长,高效的处理和存储解决方案势在必行。然而,计算单元和存储之间的大量数据传输限制了人工神经网络(ANN)的水平。因此,量化神经网络(QNN)因其减少计算资源需求和降低消耗而备受关注。在此背景下,我们介绍了一种基于 ZTO 器件的优化三元逻辑电路。通过利用光调制来调整单个器件的开启电压,我们展示了三元电流状态的实现,从而提供了三种不同的离散状态。这种配置可扩展到 QNN 计算,展示了用于内存计算的多级量化电流值。我们实现了 91.6% 的手写数字识别率,从而展示了可靠的 QNN 硬件性能。这种稳健的 QNN 性能表明,金属氧化物光电晶体管在未来的三元计算系统中显示出巨大的潜力。
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来源期刊
ACS Applied Materials & Interfaces
ACS Applied Materials & Interfaces 工程技术-材料科学:综合
CiteScore
16.00
自引率
6.30%
发文量
4978
审稿时长
1.8 months
期刊介绍: ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.
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